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Kohn-Sham density functional theory is one of the most widely used electronic structure theories. The recently developed adaptive local basis functions form an accurate and systematically improvable basis set for solving Kohn-Sham density…

Numerical Analysis · Mathematics 2021-08-03 Jason Kaye , Lin Lin , Chao Yang

We present a multigrid algorithm for self consistent solution of the Kohn-Sham equations in real space. The entire problem is discretized on a real space mesh with a high order finite difference representation. The resulting self consistent…

Materials Science · Physics 2009-10-31 Jian Wang , Thomas L. Beck

We propose accurate computable error bounds for quantities of interest in plane-wave electronic structure calculations, in particular ground-state density matrices and energies, and interatomic forces. These bounds are based on an…

Numerical Analysis · Mathematics 2022-10-20 Eric Cancès , Geneviève Dusson , Gaspard Kemlin , Antoine Levitt

The gas of the interacted electrons is usually described within Kohn-Sham approximation by the set of Poisson and Schr\"{o}dinger equations with an effective potential for the single-particle wave functions. The solution of these equations…

Materials Science · Physics 2007-05-23 A. Ya. Shul'man , D. V. Posvyanskii

In this paper, we study finite dimensional approximations of Kohn-Sham models, which are widely used in electronic structure calculations. We prove the convergence of the finite dimensional approximations and derive the a priori error…

Numerical Analysis · Mathematics 2011-08-10 Huajie Chen , Xingao Gong , Lianhua He , Zhang Yang , Aihui Zhou

In this article, we derive fully guaranteed error bounds for the energy of convex nonlinear mean-field models. These results apply in particular to Kohn-Sham equations with convex density functionals, which includes the reduced Hartree-Fock…

Starting from the observation that one of the most successful methods for solving the Kohn-Sham equations for periodic systems -- the plane-wave method -- is a spectral method based on eigenfunction expansion, we formulate a spectral method…

Computational Physics · Physics 2016-03-08 Amartya S. Banerjee , Ryan S. Elliott , Richard D. James

We propose a novel numerical algorithm for computing the electronic structure related eigenvalue problem of incommensurate systems. Unlike the conventional practice that approximates the system by a large commensurate supercell, our…

Numerical Analysis · Mathematics 2019-03-27 Yuzhi Zhou , Huajie Chen , Aihui Zhou

We introduce a practical and efficient approach for calculating the all-electron full potential bandstructure in real space, employing a finite element basis. As an alternative to the k-space method, the method involves the self-consistent…

Materials Science · Physics 2023-07-25 Dongming Li , James Kestyn , Eric Polizzi

This paper considers the finite element solution of the boundary value problem of Poisson's equation and proposes a guaranteed em a posteriori local error estimation based on the hypercircle method. Compared to the existing literature on…

Numerical Analysis · Mathematics 2021-12-17 Taiga Nakano , Xuefeng Liu

The density functional approach in the Kohn-Sham approximation is widely used to study properties of many-electron systems. Due to the nonlinearity of the Kohn-Sham equations, the general self-consistence searching method involves…

Materials Science · Physics 2015-05-13 D. V. Posvyanskii , A. Ya. Shul'man

In the present work, we derive functional upper bounds for the potential error arising from finite-element boundary-element coupling formulations for a nonlinear Poisson-type transmission problem. The proposed a posteriori error estimates…

Numerical Analysis · Mathematics 2026-02-17 Alexander Freiszlinger , Dirk Pauly , Dirk Praetorius , Michael Schomburg

For the pure biharmonic equation and a biharmonic singular perturbation problem, a residual-based error estimator is introduced which applies to many existing nonconforming finite elements. The error estimator involves the local…

Numerical Analysis · Mathematics 2024-10-18 Dietmar Gallistl , Shudan Tian

We obtain non-symmetric upper and lower bounds on the rate of convergence of general monotone approximation/numerical schemes for parabolic Hamilton Jacobi Bellman Equations by introducing a new notion of consistency. We apply our general…

Analysis of PDEs · Mathematics 2009-11-11 Guy Barles , Espen R. Jakobsen

We propose an adaptive planewave method for eigenvalue problems in electronic structure calculations. The method combines a priori convergence rates and accurate a posteriori error estimates into an effective way of updating the energy…

Computational Physics · Physics 2021-07-30 Beilei Liu , Huajie Chen , Geneviève Dusson , Jun Fang , Xingyu Gao

This paper is concerned with the derivation of conforming and non-conforming functional a posteriori error estimates for elliptic boundary value problems in exterior domains. These estimates provide computable and guaranteed upper and lower…

Numerical Analysis · Mathematics 2014-07-22 Olli Mali , Alexey Muzalevskiy , Dirk Pauly

In this work, a method for obtaining pixel-wise error bounds in Bayesian regularization of inverse imaging problems is introduced. The proposed method employs estimates of the posterior variance together with techniques from conformal…

Computer Vision and Pattern Recognition · Computer Science 2024-08-01 Dominik Narnhofer , Andreas Habring , Martin Holler , Thomas Pock

Projection-based model order reduction of dynamical systems usually introduces an error between the high-fidelity model and its counterpart of lower dimension. This unknown error can be bounded by residual-based methods, which are typically…

Numerical Analysis · Mathematics 2023-03-31 Johannes Rettberg , Dominik Wittwar , Patrick Buchfink , Robin Herkert , Jörg Fehr , Bernard Haasdonk

This paper considers a probabilistic model for floating-point computation in which the roundoff errors are represented by bounded random variables with mean zero. Using this model, a probabilistic bound is derived for the forward error of…

Numerical Analysis · Mathematics 2021-04-15 Eric Hallman

We present some new and explicit error bounds for the approximation of distributions. The approximation error is quantified by the maximal density ratio of the distribution $Q$ to be approximated and its proxy $P$. This non-symmetric…

Statistics Theory · Mathematics 2022-09-02 Lutz Duembgen , Richard Samworth , Jon Wellner
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