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We develop a microscopic theory for nonlinear optical response of moir\'e exciton-polaritons in bilayers of transition metal dichalcogenides (TMDs). Our theory allows to study the tunnel-coupled intralayer and interlayer excitonic modes for…

Mesoscale and Nanoscale Physics · Physics 2025-07-16 Kok Wee Song , Oleksandr Kyriienko

Realizing strong nonlinear optical responses is a long-standing goal of both fundamental and technological importance. Recently significant efforts have focused on exploring excitons in solids as a pathway to achieving nonlinearities even…

Mesoscale and Nanoscale Physics · Physics 2023-06-21 Liuxin Gu , Lifu Zhang , Ruihao Ni , Ming Xie , Dominik S. Wild , Suji Park , Houk Jang , Takashi Taniguchi , Kenji Watanabe , Mohammad Hafezi , You Zhou

Optically generated excitons dictate the absorption and emission spectrum of doped semiconductor transition metal dichalcogenide monolayers. We show that upon increasing the electron density, the elementary optical excitations develop a…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Ovidiu Cotlet , Dominik S. Wild , Mikhail D. Lukin , Atac Imamoglu

Strong optical nonlinearities at the few-photon level are a central goal for quantum photonics, yet they remain difficult to realize in solid-state systems. In doped two-dimensional semiconductors, coupling between excitons and a degenerate…

We present a theoretical study of the optical response of a nonlinear oscillator formed by coupling a metal nanoparticle local surface plasmon resonance to excitonic degrees of freedom in a monolayer transition-metal dichalcogenide. We show…

Mesoscale and Nanoscale Physics · Physics 2019-06-13 Daniel B. S. Soh , Ryotatsu Yanagimoto , Eric Chatterjee , Hideo Mabuchi

Monolayer transition metal dichalcogenides (TMDs) are the first truly two-dimensional (2D) semiconductor, providing an excellent platform to investigate light-matter interaction in the 2D limit. Apart from fundamental scientific…

The strong excitonic effect in monolayer transition metal dichalcogenide (TMD) semiconductors has enabled many fascinating light-matter interaction phenomena. Examples include strongly coupled exciton-polaritons and nearly perfect atomic…

Mesoscale and Nanoscale Physics · Physics 2021-04-13 Hongchao Xie , Shengwei Jiang , Daniel A. Rhodes , James C. Hone , Jie Shan , Kin Fai Mak

We develop a theoretical description of Coulomb interactions between trions (charged excitons) that define a nonlinear optical response in doped two-dimensional semiconductors. First, we formulate a microscopic theory of trion-trion…

Mesoscale and Nanoscale Physics · Physics 2022-07-07 Kok Wee Song , Salvatore Chiavazzo , Ivan A. Shelykh , Oleksandr Kyriienko

We present a quantitative study of the nonlinear optical response of layered perovskites placed inside planar photonic microcavities in the regime of strong light matter coupling, when excitonic and photonic modes hybridize and give rise to…

Mesoscale and Nanoscale Physics · Physics 2022-11-15 A. D. Belogur , D. A. Baghdasaryan , I. V. Iorsh , I. A. Shelykh , V. Shahnazaryan

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs.…

Optics · Physics 2021-12-07 Wei Li , Ming Xin , Wenze Lan , Qinghu Bai , Shuo Du , Gang Wang , Baoli Liu , Changzhi Gu

We develop a microscopic theory for excitons and cavity exciton polaritons in transition metal dichalcogenide (TMD) monolayers under a perpendicular static magnetic field. We obtain numerically exact solutions for the ground and excited…

Mesoscale and Nanoscale Physics · Physics 2025-01-27 D. de la Fuente Pico , J. Levinsen , E. Laird , M. M. Parish , F. M. Marchetti

We theoretically investigate the corrections of exciton binding energy in monolayer transition metal dichalcogenides (TMDs) due to the exciton-optical phonon coupling in the Fr$\ddot{o}$hlich interaction model by using the linear operator…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Zi-Wu Wang , Yao Xiao , Wei-Ping Li , Run-Ze Li , Zhi-Qing Li

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…

Mesoscale and Nanoscale Physics · Physics 2022-11-02 Raul Perea-Causin , Daniel Erkensten , Jamie M. Fitzgerald , Joshua J. P. Thompson , Roberto Rosati , Samuel Brem , Ermin Malic

We study a doped transition metal dichalcogenide (TMDC) monolayer in an optical microcavity. Using the microscopic theory, we simulate spectra of quasiparticles emerging due to the interaction of material excitations and a high-finesse…

Materials Science · Physics 2024-07-23 Y. V. Zhumagulov , S. Chiavazzo , D. R. Gulevich , V. Perebeinos , I. A. Shelykh , O. Kyriienko

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

We study theoretically the Coulomb interaction between excitons in transition metal dichalcogenide (TMD) monolayers. We calculate direct and exchange interaction for both ground and excited states of excitons. The screening of the Coulomb…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 V. Shahnazaryan , I. Iorsh , I. A. Shelykh , O. Kyriienko

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

Active control over strong optical nonlinearity in solid-state systems is central to unlocking exotic many-body phenomena and scalable photonic devices. While exciton-polaritons in transition metal dichalcogenides (TMDs) offer a promising…

Strong optical nonlinearities play a central role in realizing quantum photonic technologies. In solid state systems, exciton-polaritons, which result from the hybridization of material excitations and cavity photons, are an attractive…

Monolayer transition metal dichalcogenide (TMD) semiconductors such as MoSe$_2$ host strongly bound excitons which are known to exhibit a strong resonant third-order nonlinear response. Although there have been numerous studies of the…

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