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Circular dichroism, arising from interactions with light fields of opposite spin angular momentum, has become a fundamental tool for molecular characterization. Meanwhile, helical dichroism (HD) - the dichroic response to vortex beams…

The optical properties of rod-like two-layer nanoparticles are studied using the notions of equivalent prolate spheroid. The calculations are presented for frequency dependencies for polarizability and the absorption and scattering…

Optics · Physics 2024-07-02 Ya. V. Karandas

Van der Waals interactions are ubiquitous and they play an important role for the stability of materials. Current understanding of this type of coupling is based on linear response theory, while optical nonlinearities are rarely considered…

Materials Science · Physics 2024-08-27 Dai-Nam Le , Pablo Rodriguez-Lopez , Lilia M. Woods

In some respects, a cluster consisting of many atoms may be regarded as a single large atom. Knowing the dielectric properties of such a cluster permits one to evaluate the form of the van der Waals (dispersion) interactions between two…

Soft Condensed Matter · Physics 2009-11-07 M. M. Calbi , S. M. Gatica , D. Velegol , M. W. Cole

Chiral crystals show promise for spintronic technologies on account of their high spin selectivity, which has led to significant recent interest in quantitative characterization and first-principles prediction of their spin-optoelectronics…

Materials Science · Physics 2023-12-05 Christian Multunas , Andrew Grieder , Junqing Xu , Yuan Ping , Ravishankar Sundararaman

We present a simple model of collective plasmons in a dimerized chain of spherical metallic nanoparticles, an elementary example of a topologically nontrivial nanoplasmonic system. Taking into account long-range quasistatic dipolar…

Mesoscale and Nanoscale Physics · Physics 2018-10-23 Charles A. Downing , Guillaume Weick

We develop a general quantum theory of the coupled plasmonic modes resulting from the near-field interaction between localized surface plasmons in a heterogeneous metallic nanoparticle dimer. In particular, we provide analytical expressions…

Mesoscale and Nanoscale Physics · Physics 2016-03-02 Adam Brandstetter-Kunc , Guillaume Weick , Dietmar Weinmann , Rodolfo A. Jalabert

Circular dichroism is a technologically important phenomenon contrasting the absorption and resultant emission properties between left- and right-handed circularly polarized light. While the chiral handedness of systems mainly determines…

Optics · Physics 2023-03-21 Xiuhu Zhao , Jinxing Li , Mingjun Huang , Satoshi Aya

The optical properties of nanoparticle clusters vary with the spatial arrangement of the constituent particles, but also the overall orientation of the cluster with respect to the incident light. This is particularly important in the…

Optics · Physics 2021-11-02 Atefeh Fazel-Najafabadi , Baptiste Auguié

Self-organized monocrystalline Au nanoparticles with potential applications in plasmonics are grown in a SrTiO$_3$ matrix by a novel two-step deposition process. The crystalline preferred orientation of these Au nanoparticles is…

Mesoscale and Nanoscale Physics · Physics 2015-07-02 Davide Pincini , Claudio Mazzoli , Hendrik Bernhardt , Christian Katzer , Frank Schimdl , Ingo Uschmann , Carsten Detlefs

Polarons can control carrier mobility and can also be used in the design of quantum devices. Although much effort has been directed into investigating the nature of polarons, observation of defect-related polarons is challenging due to…

Materials Science · Physics 2024-09-11 Takuto Ichikawa , Junjie Guo , Paul Fons , Dwi Prananto , Toshu An , Muneaki Hase

Unidirectional backward and forward scattering of electromagnetic waves by nanoparticles are usually interpreted as the interference of conventional multipole moments (i.e., electric and magnetic dipole, electric quadrupole, etc.). The role…

Optics · Physics 2017-05-24 Lixin Ge , Liang Liu , Shiwei Dai , Jiwang Chai , Qianju Song , Hong Xiang , Dezhuan Han

Plasmonic nanocrystals with hot spots are able to localize optical energy in small spaces. In such physical systems, near-field interactions between molecules and plasmons can become especially strong. This paper considers the case of a…

Mesoscale and Nanoscale Physics · Physics 2017-04-19 Lucas V. Besteiro , Hui Zhang , Jérôme Plain , Gil Markovich , Zhiming Wang , Alexander O. Govorov

We experimentally demonstrate the coupling of far-field light to highly confined plasmonic gap modes via connected nanoantennas. The excitation of plasmonic gap modes is shown to depend on the polarization, position and wavelength of the…

Strong light-matter interactions facilitate not only emerging applications in quantum and non-linear optics but also modifications of materials properties. In particular the latter possibility has spurred the development of advanced…

Mesoscale and Nanoscale Physics · Physics 2021-08-17 Jakub Fojt , Tuomas P. Rossi , Tomasz J. Antosiewicz , Mikael Kuisma , Paul Erhart

Light interaction with rotating nanostructures gives rise to phenemona as varied as optical torques and quantum friction. Here we reveal that circular dichroism of rotating optically-isotropic particles has an unexpectedly strong dependence…

Mesoscale and Nanoscale Physics · Physics 2019-08-14 Deng Pan , Hongxing Xu , F. Javier García de Abajo

The near-field interaction of plasmonic nanostructures and chiral molecules induces circular dichroism in achiral nanostructure. The induced circular dichroism (ICD) strength is several orders greater than the molecular inherent CD (MCD),…

The albedo and dichroic polarization of spheroidal particles are studied. For the description of the phase function two asymmetry parameters $g_{||}$ and $g_{\bot}$ characterizing the anisotropy in forward/backward and left/right directions…

Astrophysics · Physics 2007-05-23 Nikolai V. Voshchinnikov

A light beam can carry both spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is commonly evidenced by circular dichroism (CD) experiments {\em i. e.} differential absorption of left and right-handed circularly polarized…

Photoelectron circular dichroism in the one-photon detachment of a model methane-like chiral anionic system is studied theoretically by the single center method. The computed chiral asymmetry, characterized by the dichroic parameter…

Atomic and Molecular Clusters · Physics 2022-02-02 Anton N. Artemyev , Eric Kutscher , Philipp V. Demekhin