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Dual-comb spectroscopy (DCS) utilizes a pair of broadband mutually coherent laser frequency combs to enable high-resolution, high-accuracy spectroscopic measurements with atomic-clock-level frequency referencing, and rapid, multiplexed…

Optics · Physics 2025-10-01 D. Konnov , A. Muraviev , K. L. Vodopyanov

Laser spectroscopy and interferometry have provided an unparalleled view into the fundamental nature of matter and the universe through ultra-precise measurements of atomic transition frequencies and gravitational waves. Optical frequency…

Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…

Quantum cascade lasers (QCLs) facilitate compact optical frequency comb sources that operate in the mid-infrared and terahertz spectral regions, where many molecules have their fundamental absorption lines. Enhancing the optical bandwidth…

Optical ranging is a key technology in metrology. Optical frequency combs are shown to provide several advantages in light ranging, offering high precision with high acquisition rate. However, performance of traditional ranging systems…

The broad and equidistant spectrum of frequency combs has had a profound impact on spectroscopic studies. Particularly, experiments involving the coupling of frequency combs to cavities have already enabled unprecedented broadband and…

Optics · Physics 2024-12-10 Andrei Diakonov , Konstantin Khrizman , Eliran Zano , Liron Stern

We propose a new approach to near-infrared molecular spectroscopy, harnessing advanced concepts of optical telecommunications and supercontinuum photonics. We generate, without mode-locked lasers, two frequency combs of slightly different…

A theoretical analysis is carried out for the recently developed three-pulse photon echo spectroscopy employing dual frequency combs (DFC) as the light sources. In this method, the molecular sample interacts with three pulse trains derived…

Chemical Physics · Physics 2020-01-08 Jonggu Jeon , JunWoo Kim , Tai Hyun Yoon , Minhaeng Cho

Spectroscopy in the molecular fingerprint spectral region (6.5-20 $\mu$m) yields critical information on material structure for physical, chemical and biological sciences. Despite decades of interest and effort, this portion of the…

We demonstrate simple optical frequency combs based on semiconductor quantum well laser diodes. The frequency comb spectrum can be tailored by choice of material properties and quantum-well widths, providing spectral flexibility. Finally,…

Optics · Physics 2020-07-21 Mark Dong , Matthew W. Day , Herbert G. Winful , Steven T. Cundiff

Optical frequency combs are an essential tool for precision metrology experiments ranging in application from remote spectroscopic sensing of trace gases to the characterization and comparison of optical atomic clocks for precision…

We perform dual-comb spectroscopy in two UV bands: 325-342 nm and 372-410 nm, corresponding to the 7th and 6th harmonics of a dual-comb 2.35-{\mu}m laser source, and simultaneously resolve ~500,000 and ~1,000,000 comb lines spaced by 80 MHz…

Frequency combs, spectra of evenly-spaced narrow phase-coherent laser lines, have revolutionized precision measurements. On-chip frequency comb generators hold much promise for fully-integrated instruments of time and frequency metrology.…

In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…

Measuring the spectral properties of an optical frequency comb is among the most fundamental tasks of precision metrology. In contrast to general single-parameter measurement schemes, we demonstrate here single shot multiparameter…

Quantum Physics · Physics 2020-03-16 Y. Cai , J. Roslund , V. Thiel , C. Fabre , N. Treps

Infrared spectroscopy in the spectral fingerprint region from 6-12 um accesses the largest molecular absorption cross-sections, permitting sensitive, quantitative and species-specific measurements. Here, we show how dual-comb…

Optics · Physics 2023-06-26 O. Kara , L. Maidment , T. Gardiner , P. G. Schunemann , D. T. Reid

We present a new representation of light curves, which is quite different from the binning method. Instead of choosing uniform bins, the reciprocal of interval between two successive photons is adopted to represent the counting rate. A…

High Energy Astrophysical Phenomena · Physics 2014-01-14 Jun Tian , Yuan-Chuan Zou

We have built a frequency chain which enables to measure the absolute frequency of a laser emitting in the 28-31 THz frequency range and stabilized onto a molecular absorption line. The set-up uses an optical frequency comb and an…

We generate a 200-nm optical frequency comb at 1.5 microns by injecting two single-frequency lasers into a highly nonlinear fiber, and explore its spectral phase properties and high power to demonstrate full nonlinear conversion into its…

It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…

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