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Pulse generation often requires a stabilized cavity and its corresponding mode structure for initial phase-locking. Contrastingly, modeless cavity-free random lasers provide new possibilities for high quantum efficiency lasing that could…

A technique to measure the decoherence time of optical phonons in a solid is presented. Phonons are excited with a pair of time delayed 80 fs, near infrared pulses via spontaneous, transient Raman scattering. The fringe visibility of the…

We describe a simple and efficient setup to generate and characterize femtosecond quadrature-entangled pulses. Quantum correlations equivalent to about 2.5 dB squeezing are efficiently and easily reached using the non-degenerate parametric…

Quantum Physics · Physics 2009-11-10 Jerome Wenger , Alexei Ourjoumtsev , Rosa Tualle-Brouri , Philippe Grangier

We address a problem of generating a robust entangling gate between electronic and nuclear spins in the system of a single nitrogen-vacany centre coupled to a nearest Carbon-13 atom in diamond against certain types of systematic errors such…

Quantum Physics · Physics 2010-07-14 R. S. Said , J. Twamley

We employed femtosecond pump probe technique to investigate the dynamics of coherent optical phonons in iron garnet. A phenomenological symmetry-based consideration reveals that oscillations of the terahertz T2g mode are excited. Selective…

We experimentally demonstrate over two orders of magnitude increase in the coherence time of nitrogen vacancy centres in diamond by implementing decoupling techniques. We show that equal pulse spacing decoupling performs just as well as…

Quantum Physics · Physics 2010-12-08 C. A. Ryan , J. S. Hodges , D. G. Cory

We show theoretically that polariton pairs with a high degree of polarization entanglement can be produced through parametric scattering. We demonstrate that it can emerge in coincidence experiments, even at low excitation densities where…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 S. Portolan , O. Di Stefano , S. Savasta , V. Savona

Nitrogen-vacancy (NV) centers in diamond have emerged as quantum sensors capable of detecting nuclear magnetic resonance (NMR) signals at unprecedented length scales, ranging from picoliter sample volumes down to single spins at the diamond…

Chemical Physics · Physics 2025-01-07 Nick R. von Grafenstein , Karl D. Briegel , Jorge Casanova , Dominik B. Bucher

We demonstrate stimulated Raman gain using a broadband LED Stokes source to measure vibrational spectra of aqueous glucose solutions. This versatile and cost-effective method increases Raman signal for a variety of applications. We measured…

Applied Physics · Physics 2018-09-14 Peter Bullen , Ioannis Kymissis , Adler Perotte

The chaotic nature of x-ray free-electron-laser pulses is a major bottleneck that has limited the joint temporal and spectral resolution of spectroscopic measurements. We show how to use the stochastic x-ray field statistics to overcome…

Optics · Physics 2021-02-15 Stefano M. Cavaletto , Daniel Keefer , Shaul Mukamel

We show that coherent anti-Stokes Raman lineshapes do not follow known spectral profiles if the time asymmetry of realistic laser pulses is taken into account. Examples are given for nanosecond and picosecond laser pulses commonly employed…

Optics · Physics 2015-06-22 Michele Marrocco , Emil Nordström , Per-Erik Bengtsson

An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

We demonstrate an efficient nonlinear process in which Stokes and anti-Stokes components are generated spontaneously in a Raman-like, near resonant media driven by low power counter-propagating fields. Oscillation of this kind does not…

Quantum Physics · Physics 2009-01-23 A. S. Zibrov , M. D. Lukin , M. O. Scully

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…

We study the influence of nuclei-induced frequency focusing on the mode locking of spin coherence in quantum dots subjected to a periodic train of optical pulses. In particular, we address the question whether or not nuclei-induced…

Mesoscale and Nanoscale Physics · Physics 2020-09-09 Philipp Schering , Philipp W. Scherer , Götz S. Uhrig

Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…

Quantum Physics · Physics 2023-07-18 Valeria Vento , Santiago Tarrago Velez , Anna Pogrebna , Christophe Galland

Nuclear spins nearby nitrogen-vacancy (NV) centers in diamond are excellent quantum memory for quantum computing and quantum sensing, but are difficult to be initialized due to their weak interactions with the environment. Here we propose…

Quantum Physics · Physics 2019-09-04 Nanyang Xu , Yu Tian , Bing Chen , Jianpei Geng , Xiaoxiong He , Ya Wang , Jiangfeng Du

We investigate the polarization state dynamics of single photon pulse for optical fiber quantum communication channels. On the basis of a birefringence vector model in which amplitude and direction are both stochastic variables, Jones…

Quantum Physics · Physics 2009-09-01 Chang-hua Zhu , Chang-xing Pei , Dong-xiao Quan , Nan Chen , Yun-hui Yi