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We describe the behavior of an Ising model with orthogonal dynamics, where changes in energy and changes in alignment never occur during the same Monte Carlo (MC) step. This orthogonal Ising model (OIM) allows conservation of energy and…

Soft Condensed Matter · Physics 2022-10-26 Ralph V. Chamberlin

Directional solidification occurs in industrial and natural processes, such as freeze-casting, metal processing, biological cryopreservation and freezing of soils. Translational temperature gradient stage allows to control the process of…

Applied Physics · Physics 2020-11-10 Michael Chasnitsky , Victor Yashunsky , Ido Braslavsky

Sympathetic cooling is the process of energy exchange between a system and a colder bath. We investigate this fundamental process in an atom-ion experiment where the system is composed of a single ion, trapped in a radio-frequency Paul…

Atomic Physics · Physics 2018-08-08 Ziv Meir , Meirav Pinkas , Tomas Sikorsky , Ruti Ben-shlomi , Nitzan Akerman , Roee Ozeri

We investigate the temperature dependence of thermodynamic (density, isobaric heat capacity), dynamical (self-diffusion coefficient, shear viscosity), and dielectric properties of several water models, the commonly employed TIP3P water…

Soft Condensed Matter · Physics 2022-04-13 Tatiana I. Morozova , Nicolas A. Garcia , Jean-Louis Barrat

We study a two-dimensional fluid of particles interacting through a spherically-symmetric and marginally soft two-body repulsion. This model can exist in three different crystal phases, one of them with square symmetry and the other two…

Soft Condensed Matter · Physics 2012-09-13 Santi Prestipino , Franz Saija , Paolo V. Giaquinta

Standard density functionals without van der Waals interactions yield an unsatisfactory description of ice phases, specifically, high density phases occurring under pressure are too unstable compared to the common low density phase I$_h$…

Chemical Physics · Physics 2014-05-16 Markus Macher , Jiří Klimeš , Cesare Franchini , Georg Kresse

Water is the main component of interstellar ice mantles, is abundant in the solar system and is a crucial ingredient for life. The formation of this molecule in the interstellar medium cannot be explained by gas-phase chemistry only and its…

Solar and Stellar Astrophysics · Physics 2017-08-23 S. Ioppolo , H. M. Cuppen , C. Romanzin , E. F. van Dishoeck , H. Linnartz

Using numerical simulations that mimic recent experiments on hexagonal colloidal ice, we show that colloidal hexagonal artificial spin ice exhibits an inner phase within its ice state that has not been observed previously. Under increasing…

Statistical Mechanics · Physics 2018-01-17 A. Libal , C. Nisoli , C. J. O. Reichhardt , C. Reichhardt

The potential energy landscape (PEL) formalism is a statistical mechanical approach to describe supercooled liquids and glasses. Here we use the PEL formalism to study the pressure-induced transformations between low-density amorphous ice…

Statistical Mechanics · Physics 2019-07-24 Philip H. Handle , Francesco Sciortino , Nicolas Giovambattista

We examine the shape of a an isolated, dislocation-free ice crystal when it is in equilibrium with the vapor phase in an isothermal closed environment, as a function of temperature. From our analysis we draw the following conclusions: 1)…

Materials Science · Physics 2012-05-08 Kenneth G. Libbrecht

Water ice is abundant both astrophysically, for example in molecular clouds, and in planetary systems. The Kuiper belt objects, many satellites of the outer solar system, the nuclei of comets and some planetary rings are all known to be…

Astrophysics · Physics 2009-11-13 Weijun Zheng , David Jewitt , Ralf I. Kaiser

We perform molecular dynamics simulations of a well-known water model (the TIP5P pair potential) and a simple liquid model (a two-scale repulsive ramp potential) to compare the regions of anomalous behavior in their phase diagrams. We…

Soft Condensed Matter · Physics 2007-12-14 Zhenyu Yan , Sergey V. Buldyrev , Pradeep Kumar , Nicolas Giovambattista , H. Eugene Stanley

We present results of classical dynamics calculations, performed to study the photodissociation of water in crystalline and amorphous ice surfaces at a surface temperature of 10 K. Dissociation in the top six monolayers is considered.…

Astrophysics · Physics 2009-11-11 Stefan Andersson , Ayman Al-Halabi , Geert-Jan Kroes , Ewine F. van Dishoeck

An exact integral formula for the Kirkwood correlation factor of isotropic polar fluids $g_K$ is derived from the equilibrium averaged rotational Dean equation, which as compared to previous approaches easily lends itself to further…

We provide a fully analytical microscopic theory for the proton correlations in water ice $I_h$. We compute the full diffuse elastic neutron scattering structure factor, which we find to be in excellent quantitative agreement with Monte…

Statistical Mechanics · Physics 2015-08-19 S. V. Isakov , R. Moessner , S. L. Sondhi , D. A. Tennant

Molecular dynamics simulations are utilized to study the microwave heating of methane hydrate by the five-body rotation coordinate system with the TIP5P-Ewald model. The structure I of methane hydrate is constructed, and the ice and free…

Chemical Physics · Physics 2024-03-01 Motohiko Tanaka

In equilibrium and supercooled liquids, polymorphism is manifested by thermodynamic regions defined in the phase diagram, which are predominantly of different short- and medium-range order (local structure). It is found that on the phase…

Soft Condensed Matter · Physics 2024-03-19 Anatolii V. Mokshin , Roman V. Vlasov

Water has many anomalous properties compared to "simple" liquids, and these anomalies are typically enhanced in supercooled water. While numerous models have been proposed, including the liquid-liquid critical point, the singularity-free…

Chemical Physics · Physics 2020-10-28 Loni Kringle , Wyatt A. Thornley , Bruce D. Kay , Greg A. Kimmel

The paper presents a model for liquid uranium dioxide, obtained by improving a simplified ionic model, previously adopted to describe the equation of state of this substance [1]. A "chemical picture" is used for liquid UO2 of stoichiometric…

A relativistic mean-field model of nuclear matter with arbitrary proton fraction is studied at finite temperature. An analysis is performed of the liquid-gas phase transition in a system with two conserved charges (baryon number and…

Nuclear Theory · Physics 2008-11-26 Horst Mueller , Brian D. Serot