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We examine anharmonic contributions to the optical phonon modes in bulk $T_d$-MoTe$_2$ through temperature-dependent Raman spectroscopy. At temperatures ranging from 100 K to 200 K, we find that all modes redshift linearly with temperature…

Materials Science · Physics 2016-07-20 Jaydeep Joshi , Iris Stone , Ryan Beams , Sergiy Krylyuk , Irina Kalish , Albert Davydov , Patrick Vora

Temperature-dependent FAR-infrared reflectivity spectra of partially ordered magnetodielectric La2CoMnO6 is presented, from room temperature up to 675 K. A clear first-ordered structural phase transition (SPT) from a monoclinic structure…

Materials Science · Physics 2018-02-22 R. X. Silva , A. Nonato , R. L. Moreira , R. M. Almeida , C. W. A. Paschoal

Guided modes in anisotropic two-dimensional van der Waals materials are experimentally investigated and their refractive indices in visible wavelengths are extracted. Our method involves near-field scanning optical microscopy of waveguide…

Polarized Raman scattering spectra of superconducting K$_x$Fe$_{2-y}$Se$_2$ and nonsuperconducting K$_{0.8}$Fe$_{1.8}$Co$_{0.2}$Se$_2$ single crystals were measured in a temperature range from 10 K up to 300 K. Two Raman active modes from…

Materials Science · Physics 2016-09-20 M. Opačić , N. Lazarević , M. Šćepanović , Hyejin Ryu , Hechang Lei , C. Petrovic , Z. V. Popović

The two-dimensional silicon allotrope, silicene, could spur the development of new and original concepts in Si-based nanotechnology. Up to now silicene can only be epitaxially synthesized on a supporting substrate such as Ag(111). Even…

Materials Science · Physics 2016-05-06 Dmytro Solonenko , Ovidiu D. Gordan , Guy Le Lay , Dietrich R. T. Zahn , Patrick Vogt

We investigate the long-wavelength dispersion of longitudinal and transverse optical phonon modes in polar two-dimensional materials, multilayers, and their heterostructures. Using analytical models and density-functional perturbation…

Materials Science · Physics 2017-08-02 Thibault Sohier , Marco Gibertini , Matteo Calandra , Francesco Mauri , Nicola Marzari

In this work, we performed temperature-dependent Raman spectroscopy studies on three layered metal thiophosphates: CuInP2S6, CuCrP2S6, and CuInP2S6-In4/3P2S6 heterostructures. These materials are emerging multiferroics, with CuInP2S6 and…

Materials Science · Physics 2022-12-29 Rahul Rao , Michael A. Susner

We have performed polarized Raman scattering measurements on WTe$_2$, for which an extremely large positive magnetoresistance has been reported recently. We observe 5 A$_1$ phonon modes and 2 A$_2$ phonon modes out of 33 Raman active modes,…

Materials Science · Physics 2015-02-27 W. -D. Kong , S. -F. Wu , P. Richard , C. -S. Lian , J. -T. Wang , C. -L. Yang , Y. -G. Shi , H. Ding

Despite their puzzling vibrational characteristics that include strong signatures of anharmonicity and thermal disorder already around room temperature, halide perovskites exhibit favorable optoelectronic properties for applications in…

Materials Science · Physics 2022-02-08 Christian Gehrmann , Sebastián Caicedo-Dávila , Xiangzhou Zhu , David A. Egger

Black phosphorus (P), a layered material that can be isolated down to individual 2D crystalline sheets, exhibits highly anisotropic mechanical properties due to its corrugated crystal structure in each atomic layer, which are intriguing for…

Mesoscale and Nanoscale Physics · Physics 2015-04-07 Zenghui Wang , Philip X. -L. Feng

Mixed-halide perovskites offer a route to enhance phase stability and modify optoelectronic properties. Here, we use large-scale molecular dynamics simulations with a reactive force field to investigate defects in…

Materials Science · Physics 2026-05-12 Konrad Wilke , Mike Pols , Titus S. van Erp , Geert Brocks , Shuxia Tao

Perovskite oxynitrides are a promising class of material for photocatalytic water-splitting due to their small band gaps and suitably aligned band edges. Recently, epitaxially strained oxynitrides started to attract interest due to the…

Materials Science · Physics 2018-10-17 Nathalie Vonrüti , Ulrich Aschauer

We employ a combined experimental-theoretical study of the first- and second-order Raman modes of monoclinic $\beta$-Ga$_{2}$O$_{3}$. The investigated materials is of particular interest due to its deep-UV bandgap paired with a high…

Materials Science · Physics 2022-01-19 Benjamin M. Janzen , Roland Gillen , Zbigniew Galazka , Janina Maultzsch , Markus R. Wagner

The selection rule for angle-resolved polarized Raman (ARPR) intensity of phonons from standard group-theoretical method in isotropic materials would break down in anisotropic layered materials (ALMs) due to birefringence and linear…

New approach on interpretation and processing of Raman spectra of complex perovskites is suggested. Raman spectra of $PbMg_{1/3}Nb_{2/3}O_{3}$ and $% PbSc_{1/2}Ta_{1/2}O_{3}$ are successfully described on the basis of the phonon-confinement…

Materials Science · Physics 2007-05-23 E. A. Rogacheva

Two-dimensional (2D) perovskites or Ruddleson Popper (RP) perovskites have emerged as a class of material inheriting the superior optoelectronic properties of two different materials: perovskites and 2D materials. The large exciton binding…

A Raman spectroscopy study was carried out for ZnGeN2 with direction of propagation along the (0001) crystallographic direction on hexagonal single crystal platelets obtained by reaction of gaseous ammonia with a Zn-Ge-Sn liquid alloy at…

Materials Science · Physics 2017-03-08 Eric W. Blanton , Mark Hagemann , Keliang He , Jie Shan , Walter R. L. Lambrecht , Kathleen Kash

Borophene, an atomically thin, corrugated, crystalline two-dimensional boron sheet, has been recently synthesized. We investigate mechanical properties and lattice thermal conductivity of borophene via reactive molecular dynamics…

Materials Science · Physics 2017-07-05 Bohayra Mortazavi , Minh-Quy Le , Timon Rabczuk , Luiz Felipe C. Pereira

We investigated 10 to 200 nm thick black phosphorus flakes on SiO2/Si and polyimide substrates by Angle-resolved Polarized Raman spectra (ARPRS) using 442 nm excitation wavelength. The results revealed that ARPRS with 442 nm excitation can…

Materials Science · Physics 2016-10-12 Weijun Luo , Qian Song , Guangnan Zhou , David Tuschel , Guangrui Xia

Ba2YIrO6, a Mott insulator, with four valence electrons in Ir5+ d-shell (5d4) is supposed to be non-magnetic, with Jeff = 0, within the atomic physics picture. However, recent suggestions of non-zero magnetism have raised some fundamental…

Strongly Correlated Electrons · Physics 2019-01-03 Birender Singh , G. A. Cansever , T. Dey , A. Maljuk , S. Wurmehl , B. Büchner , Pradeep Kumar