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High-order harmonic generation (HHG), characterized by its highly nonlinear nature, often exhibits a complex spatio-temporal profile that poses challenges for practical applications. In this study, we unveil a method for manipulating the…

Optics · Physics 2024-12-10 Qi Zeng , Yimin Deng , Xinyue Yang , Wei Cao , Peixiang Lu

We report on the development of a high-order harmonic generation (HHG)-based ultrafast high-repetition-rate (250 kHz) monochromatic extreme ultraviolet (21.6 eV) source with polarization tunability, specifically designed for multi-modal…

High harmonic generation (HHG) is a crucial technology for compact, high-brightness extreme ultraviolet (XUV) and soft X-ray sources, which are key to advancing both fundamental and applied sciences. The availability of advanced driving…

Optics · Physics 2025-10-07 Robert Klas , Martin Gebhardt , Jan Rothhardt , Jens Limpert

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

Effects of the laser pulse wavelength and intensity on the HHG production from the \textit{ionic} and \textit{homolytic} pre-ionization transient states of the two-electron H$_{2}$ system exposed to ultrashort intense laser pulses are…

Atomic Physics · Physics 2015-06-17 Behnaz Buzari , Mohsen Vafaee , Hassan Sabzyan

High harmonic generation (HHG) from gas phase atoms (or molecules) has opened up a new frontier in ultrafast optics, where attosecond time resolution and Angstrom spatial resolution are accessible. The fundamental physical pictures of HHG…

Optics · Physics 2023-04-26 Liang Li , Pengfei Lan , Xiaosong Zhu , Peixiang Lu

High harmonic generation (HHG) in gaseous media provides a robust method for producing coherent extreme-ultraviolet (EUV) radiation and attosecond pulses. However, the spectral and temporal properties of these pulses -- such as bandwidth…

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

Atomic Physics · Physics 2016-12-28 Néstor F. Aguirre , Fernando Martín

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

We demonstrate a High-Harmonic-Generation scheme which offers control over the bandwidth of the spectral peaks. The scheme uses a vectorial two-color driver with close central frequencies, generated by spectrally splitting a…

Optics · Physics 2024-02-26 Eldar Ragonis , Eran Ben Arosh , Lev Merensky , Avner Fleischer

The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , B. R. Avchyan , G. F. Mkrtchian

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

High harmonic generation (HHG) has become a multipurpose source of coherent XUV radiation used in various applications. One of the notable aspects of HHG is its wide spectrum consisting of many harmonic orders. This might represent a…

We introduce two-color counterrotating circularly polarized laser fields as a new way to spectrally control high harmonic generation (HHG) from relativistic plasma mirrors. Through particle-in-cell simulations, we show that only a selected…

Plasma Physics · Physics 2018-04-13 Zi-Yu Chen

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

In the past two decades high-harmonic generation (HHG) has become a key process in ultra-fast science due to the extremely short time-structure of the underlying electron dynamics being imprinted in the emitted harmonic light bursts. After…

Atomic Physics · Physics 2012-01-25 Markus C. Kohler , Thomas Pfeifer , Karen Z. Hatsagortsyan , Christoph H. Keitel