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We report the simultaneous measurement of the structural and electronic components of the metal-insulator transition of VO$_2$ using electron and photoelectron spectroscopies and microscopies. We show that these evolve over different…

Strongly Correlated Electrons · Physics 2014-11-18 J. Laverock , S. Kittiwatanakul , A. A. Zakharov , Y. R. Niu , B. Chen , S. A. Wolf , J. W. Lu , K. E. Smith

We investigate the structural, vibrational, morphological, and electronic properties of Nb substituted orthovanadate LaV$_{1-x}$Nb$_x$O$_4$ samples prepared by the solid-state reaction method. The x-ray diffraction (XRD) analysis reveals…

Materials Science · Physics 2023-07-04 Ashok Kumar , Anurag Sharma , Madhav Sharma , Vinod Singh , Anita Dhaka , Rajendra S. Dhaka

We report experimental evidence for pressure instabilities in the model multiferroic BiFeO3 and namely reveal two structural phase transitions around 3 GPa and 10 GPa by using diffraction and far-infrared spectroscopy at a synchrotron…

Materials Science · Physics 2011-07-26 R. Haumont , P. Bouvier , A. Pashkin , K. Rabia , S. Frank , B. Dkhil , W. A. Crichton , C. A. Kuntscher , J. Kreisel

We report high-pressure photoluminescence, Raman scattering, and x-ray diffraction measurements on a lead-free halide perovskite $Cs_3Sb_2Br_9$. At about 3 GPa, an electronic transition manifests itself through a broad minimum in linewidth,…

Alkaline-earth metal oxides, in particular MgO and CaO dominate Earths lower mantle, therefore, exploring high pressure behavior of this class of compounds is of significant geophysical research interest. Among all these compounds, BaO…

The temperature (T) dependent x-ray diffraction (XRD) and resistivity measurements of La0.175Pr0.45Ca0.375MnO3 (LPCMO) have been performed down to 2K to understand the structural and transport properties. From room temperature down to 220K,…

Materials Science · Physics 2016-06-22 Shivani Sharma , Aga Shahee , Kiran Singh , N. P. Lalla

We present the structural, electronic, vibrational, and photoluminescence properties of polycrystalline LaV$_{1-x}$Nb$_x$O$_4$ ($x =$ 0--0.2) samples at room temperature. The substitution of Nb at the V site shows the fascinating structural…

Materials Science · Physics 2021-05-19 Hemanshu Dua , Rishabh Shukla , R. S. Dhaka

Compressed S and Se are studied by x-ray diffraction with synchrotron radiation up to 160 GPa. The S-IV phase is shown to have a body-centered monoclinic structure and to be stable between 83 and 150 GPa on pressure increase, where it…

Other Condensed Matter · Physics 2009-11-11 Olga Degtyareva , Eugene Gregoryanz , Maddury Somayazulu , Ho-kwang Mao , Russell J. Hemley

Combining first-principles calculations with a technique for many-body problems, we investigate properties of the transition metal oxide ${\rm Sr_{2}VO_{4}}$ from the microscopic point of view. By using the local density approximation…

Strongly Correlated Electrons · Physics 2007-05-23 Yoshiki Imai , Masatoshi Imada

Structural behavior and equation of state of atomic and molecular crystal phases of dense hydrogen at pressures up to 3.5 TPa are systematically investigated with density functional theory. The results indicate that the Vinet EOS model that…

Other Condensed Matter · Physics 2012-03-27 Hua Y. Geng , Hong X. Song , J. F. Li , Q. Wu

We report studies of in-situ x-ray diffraction (XRD) and electronic properties on the single crystalline of Fe1.05Te compound under high pressure. The results demonstrated that the sample undergoes a pressure-induced lattice collapse in…

Superconductivity · Physics 2009-12-01 Chao Zhang , Wei Yi , Liling Sun , Wei Lu , Xiaoli Dong , Ligang Bai , Jing Liu , Genfu Chen , Nanlin Wang , Zhongxian Zhao

Using ab initio evolutionary structure prediction method in conjunction with density functional theory, we performed a systematic investigation on the structural transition of elemental scandium under pressure up to 250 GPa. Our prediction…

Materials Science · Physics 2019-01-09 Shengcai Zhu , Xiao-Zhi Yan , Scott Fredericks , Yan-Ling Li , Qiang Zhu

The physicochemical behavior of elements and compounds is heavily altered by high pressure. The occurrence of pressure-induced reactions and phase transitions can be revealed by crystal structure prediction approaches. In this work, we…

Materials Science · Physics 2016-03-09 Gabriele Saleh , Artem R. Oganov

Optical conductivity spectra of single crystals of Ca_1-xSr_xVO_3 have been studied to elucidate how the electronic behavior depends on the strength of the electron correlation without changing the nominal number of electrons per vanadium…

Strongly Correlated Electrons · Physics 2009-10-31 H. Makino , I. H. Inoue , M. J. Rozenberg , Y. Aiura , I. Hase , S. Onari

Results of X-ray diffraction experiments on solid oxygen at low temperature and at pressures up to 10 GPa are presented.A careful sample preparation and annealing around 240 K allowed to obtain very good diffraction patterns in the…

Materials Science · Physics 2009-11-07 Federico A. Gorelli , Mario Santoro , Lorenzo Ulivi , Michael Hanfland

We report pressure-dependent reflection and transmission measurements on ZnCr$_2$Se$_4$, HgCr$_2$S$_4$, and CdCr$_2$O$_4$ single crystals at room temperature over a broad spectral range 200-24000 cm$^{-1}$. The pressure dependence of the…

Materials Science · Physics 2018-02-02 K. Rabia , L. Baldassarre , J. Deisenhofer , V. Tsurkan , C. A. Kuntscher

The superconducting and structural properties of elemental strontium metal were investigated under pressures up to 60 GPa while maintaining cryogenic conditions during pressure application. Applying pressure at low temperatures reveals…

We have performed ab initio calculations for new high-pressure phase of Ca-VI between 158-180 GPa. The study includes elastic parameters of mono- and poly-crystalline aggregates, electronic band structure, lattice dynamics and…

Superconductivity · Physics 2015-05-19 M. Aftabuzzaman , A. K. M. A. Islam

Two dimensional ferroic materials exhibit a variety of functional properties that can be tuned by temperature and pressure. CuInP2S6 is a layered material that is ferrielectric at room temperature and whose properties are a result of the…

Materials Science · Physics 2023-06-14 R. Rao , B. S. Conner , J. Jiang , R. Pachter , M. A. Susner

The first-principles periodic linear combination of atomic orbitals method within the framework of density functional theory implemented in the CRYSTAL06 code has been applied to explore effect of pressure on the Compton profiles and…

Materials Science · Physics 2012-07-24 K. B. Joshi , B. K. Sharma , U. Paliwal , B. Barbiellini