Related papers: Enhancing second-harmonic generation with electron…
Optical properties of metallic nanoparticles are most often considered in terms of plasmons, the coupled states of light and quasi-free electrons. Here we predict that confinement of electrons inside the nanostructure leads to another, very…
The collective oscillations of surface charges (surface plasmons) induced by light-matter interactions were predicted in the 1950s to influence electrical conduction in 2D noble metals. Primarily two mechanisms were predicted and later by…
With the help of a theoretical model and finite-difference-time-domain simulations based on the hydrodynamic-Maxwell model, we examine the effect of difference frequency generation in an array of L-shaped metal nano-particles characterized…
We study the second-harmonic generation in left-handed metamaterials with a quadratic nonlinear response. We demonstrate a novel type of the exact phase matching between the backward propagating wave of the fundamental frequency and the…
Plasmons facilitate a strong confinement and enhancement of near-field light, offering exciting opportunities to enhance nonlinear optical responses at the nanoscale. However, despite significant advancements, the electrically tunable range…
Second harmonic generation has been applied to study lattice, electronic and magnetic proprieties in atomically thin materials. However, inversion symmetry breaking is usually required for the materials to generate a large signal. In this…
We present a method, based on noncollinear second harmonic generation, to evaluate the non-zero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization…
We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…
Nonlinear nanostructured surfaces provide a paradigm shift in nonlinear optics with new ways to control and manipulate frequency conversion processes at the nanoscale, also offering novel opportunities for applications in photonics,…
To add the detailed information to the existed knowledge of nonlinear optics field, the nonlinear optical processes of the second and third order have been discussed in their respective susceptibility tensors in the presence of degenerate…
Strong second-harmonic generation has recently been experimentally observed from metamaterials consisting of periodic arrays of metal split ring resonators with an effective negative magnetic permeability [Science, 313, 502 (2006)]. To…
We have derived the local electric field inside graded metal-dielectric composite films with weak nonlinearity analytically, which further yields the effective linear dielectric constant and third-order nonlinear susceptibility of the…
The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal…
High quality factor optical nanostructures provide great opportunity to enhance nonlinear optical processes such as third harmonic generation. However, the field enhancement in these high quality factor structures is typically accompanied…
A combined analytical and numerical study of the modes in two distinct plasmonic nanowire systems is presented. The computations are based on a Discontinuous Galerkin Time-Domain approach and a fully nonlinear and nonlocal hydrodynamic…
Generation of even-order optical harmonics requires noncentrosymmetric structures being conventionally observed in crystals lacking the center of inversion. In centrosymmetric systems, even-order harmonics may arise, e.g., at surfaces but…
We develop a microscopic large-$N$ theory of electron-electron interaction corrections to multi-legged Feynman diagrams describing second- and third-order nonlinear response functions. Our theory, which reduces to the well-known random…
Understanding how light interacts at the nanoscale with metals, semiconductors, or ordinary dielectrics is pivotal if one is to properly engineer nano-antennas, filters and, more generally, devices that aim to harness the effects of new…
Nonlinear metasurface holography shows the great potential of metasurfaces to control the phase, amplitude, and polarization of light while simultaneously converting the frequency of the light. The possibility of tailoring the scattering…
We theoretically show the existence of cascaded second-order surface plasmon solitons propagating at the interface between metal and linear dielectric. Nonlocal multipole nonlinearities originating from free conduction electron plasma of a…