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Quantum spin liquid (QSL) phases exist in theory, but real candidate QSL materials are often extraordinarily sensitive to structural defects which disrupt the ground state. Here, we investigate candidate triangular QSL material…

The spiral spin liquid (SSL) is a highly degenerate state characterized by a continuous contour or surface in reciprocal space spanned by a spiral propagation vector. Although the SSL state has been predicted in a number of various…

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

Strongly Correlated Electrons · Physics 2013-07-19 Tian-Heng Han , Joel S. Helton , Shaoyan Chu , Daniel G. Nocera , Jose A. Rodriguez-Rivera , Collin Broholm , Young S. Lee

We report proximate quantum spin liquid behavior in K$_2$Co$_2$(SO$_4$)$_3$ with the magnetic Co$^{2+}$ ions embedded on a highly frustrated three-dimensional double trillium lattice. Single-crystal and high-resolution synchrotron powder…

Motivated by recent experiments on Ba3NiSb2O9, we investigate possible quantum spin liquid ground states for spin S=1 Heisenberg models on the triangular lattice. We use Variational Monte Carlo techniques to calculate the energies of…

Strongly Correlated Electrons · Physics 2012-12-27 Samuel Bieri , Maksym Serbyn , T. Senthil , Patrick A. Lee

Quantum spin liquid (QSL), a state characterized by exotic low energy fractionalized excitations and statistics is still elusive experimentally and may be gauged via indirect experimental signatures. Remnant of QSL phase may reflect in the…

Strongly Correlated Electrons · Physics 2023-03-29 Vivek Kumar , Deepu Kumar , Birender Singh , Yuliia Shemerliuk , Mahdi Behnami , Bernd Buchner , Saicharan Aswartham , Pradeep Kumar

Quantum spin liquids are materials that feature quantum entangled spin correlations and avoid magnetic long-range order at T = 0 K. Particularly interesting are two-dimensional honeycomb spin lattices where a plethora of exotic quantum spin…

Strongly Correlated Electrons · Physics 2020-11-20 C. Wessler , B. Roessli , K. W. Krämer , B. Delley , O. Waldmann , L. Keller , D. Cheptiakov , H. B. Braun , M. Kenzelmann

On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

The honeycomb-lattice cobaltate Na$_3$Co$_2$SbO$_6$ has recently been proposed to be a proximate Kitaev quantum spin liquid~(QSL) candidate. However, non-Kitaev terms in the Hamiltonian lead to a zigzag-type antiferromagnetic~(AFM) order at…

A key characteristic of quantum spin liquids(QSL) is the presence of fractional excitations related to their entanglement properties, yet experimental verification of their statistics is missing. For example, in the potential Kitaev spin…

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

Very recently we revealed a large family of triangular lattice quantum spin liquid candidates named rare-earth chalcogenides, which features a high-symmetry structure without structural/charge disorders and spin impurities, and may serve as…

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K2Co(SeO3)2. Despite the presence of quasi-2D "supersolid" magnetic order, the…

Strongly Correlated Electrons · Physics 2024-11-04 M. Zhu , V. Romerio , N. Steiger , S. D. Nabi , N. Murai , S. Ohira-Kawamura , K. Yu. Povarov , Y. Skourski , R. Sibille , L. Keller , Z. Yan , S. Gvasaliya , A. Zheludev

Quantum spin liquid (QSL) is a novel state of matter with exotic excitations and was theoretically predicted to be realized most possibly in an S=1/2 kagome antiferromagnet. Experimentally searching for the candidate materials is a big…

Strongly Correlated Electrons · Physics 2014-09-15 Yuesheng Li , Bingying Pan , Shiyan Li , Wei Tong , Langsheng Ling , Zhaorong Yang , Junfeng Wang , Zhongjun Chen , Zhonghua Wu , Qingming Zhang

The kagome lattice, with its unique geometric structure, has emerged as a leading platform for exploring quantum many-body physics, particularly in the study of quantum spin liquids (QSLs) and unconventional superconductivity. This review…

Strongly Correlated Electrons · Physics 2025-12-19 Li-Wei He , Shun-Li Yu , Jian-Xin Li

A primary goal at the interface of theoretical and experimental quantum magnetism is the investigation of exotic spin states, most notably quantum spin liquids (QSLs). Magnetic rare-earth ions go beyond the straightforward paradigm of…

Strongly Correlated Electrons · Physics 2022-01-11 Christopher A. Pocs , Peter E. Siegfried , Jie Xing , Athena S. Sefat , Michael Hermele , Bruce Normand , Minhyea Lee

We probed the local electronic properties of the mixed-valent Co(+4-x) triangular-lattice in Na{x}CoO{2}-yH{2}O by 59-Co NMR. We observed two distinct types of Co sites for x>=1/2, but the valence seems averaged out for x~1/3. Local spin…

Strongly Correlated Electrons · Physics 2009-11-10 F. L. Ning , T. Imai , B. W. Statt , F. C. Chou

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

Since strong quantum fluctuations are essential for the emergence of quantum spin liquids, there have been extensive exploration and identification of spin liquid candidates in spin-$1/2$ systems, while such activities are rare in higher…

Strongly Correlated Electrons · Physics 2023-07-26 Wei-Wei Luo , Yixuan Huang , D. N. Sheng , W. Zhu
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