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Related papers: On the ice-nucleating potential of warm hydrometeo…

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The formation of ice in mixed phase clouds greatly impacts Earths hydrologic cycle. The intensity, distribution and frequency of precipitation as well as radiative properties of clouds in the mid latitudes are strongly influenced by the…

Atmospheric and Oceanic Physics · Physics 2019-06-17 Prasanth Prabhakaran , Gregory Kinney , Will Cantrell , Raymond A. Shaw , Eberhard Bodenschatz

Accurate estimate of nucleation rate is crucial for the study of ice nucleation and ice-promoting/anti-freeze strategies. Within the framework of Classical Nucleation Theory (CNT), the estimate of ice nucleation rate is very sensitive to…

Soft Condensed Matter · Physics 2021-07-07 Chaohong Wang , Hao Wang , Jianyang Wu , Zhisen Zhang

The study of atmospheric ice nuclei is vital for understanding the formation of precipitation and the development of cloud systems as it reveals how these tiny particles grow. A mechanism of such growth when the nuclei are in a mixed…

Materials Science · Physics 2023-03-10 M. Boström , Y. Li , I. Brevik , C. Persson , S. Carretero-Palacios , O. I. Malyi

Acoustic cavitation is known to trigger ice nucleation in supercooled water. Several competing and still debatable mechanisms have been proposed in the literature and are related to the pressure field in the vicinity of the bubble at the…

Chemical Physics · Physics 2018-10-22 Olivier Louisnard , Fabienne Espitalier

Ice nucleation is greatly important in areas as diverse as climate change, cryobiology, geology or food industry. Predicting the ability of a substrate to induce the nucleation of ice from supercooled water is a difficult problem. Here, we…

Materials Science · Physics 2026-01-12 Miguel Camarillo , Javier Oller-Iscar , María M. Conde , Jorge Ramírez , Eduardo Sanz

The prevalence of heterogeneous nucleation in nature was explained qualitatively by the classical theory for heterogeneous nucleation established over more than 60 years ago, but the quantitative validity and the key conclusions of the…

Chemical Physics · Physics 2015-06-11 Raffaela Cabriolu , Tianshu Li

Estimating the homogeneous ice nucleation rate from undercooled liquid water is at the same time crucial for understanding many important physical phenomena and technological applications, and challenging for both experiments and theory.…

Statistical Mechanics · Physics 2025-10-06 Bingqing Cheng , Christoph Dellago , Michele Ceriotti

Ice nucleation is a process of great relevance in physics, chemistry, technology and environmental sciences, much theoretical and experimental efforts have been devoted to its understanding, but still it remains a topic of intense research.…

Soft Condensed Matter · Physics 2019-06-26 Haiyang Niu , Yi Isaac Yang , Michele Parrinello

Molecular simulations have provided valuable insight into the microscopic mechanisms underlying homogeneous ice nucleation. While empirical models have been used extensively to study this phenomenon, simulations based on first-principles…

It is surprisingly difficult to freeze water. Almost all ice that forms under "mild" conditions (temperatures > -40 degrees Celsius) requires the presence of a nucleating agent - a solid particle that facilitates the freezing process - such…

Statistical Mechanics · Physics 2014-04-25 Stephen J. Cox , Zamaan Raza , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

Despite the simplicity of the water molecule, the kinetics of ice nucleation under natural conditions can be complex. We investigated spontaneously grown ice nuclei using all-atom molecular dynamics simulations and found significant…

Soft Condensed Matter · Physics 2025-04-28 Maodong Li , Yupeng Huang , Yijie Xia , Dechin Chen , Cheng Fan , Lijiang Yang , Yi Qin Gao , Yi Isaac Yang

Among all the freezing transitions, that of water into ice is probably the most relevant to biology, physics, geology or atmospheric science. In this work we investigate homogeneous ice nucleation by means of computer simulations. We…

Soft Condensed Matter · Physics 2013-12-04 E. Sanz , C. Vega , J. R. Espinosa , R. Caballero-Bernal , J. L. F. Abascal , C. Valeriani

Coarse grained molecular dynamics simulations are presented in which the sensitivity of the ice nucleation rate to the hydrophilicity of a graphene nanoflake is investigated. We find that an optimal interaction strength for promoting ice…

Materials Science · Physics 2015-06-01 Stephen J. Cox , Shawn M. Kathmann , Ben Slater , Angelos Michaelides

The avoidance of water freezing is the holy grail in the cryopreservation of biological samples, food, and organs. Fast cooling rates are used to beat ice nucleation and avoid cell damage. This strategy can be enhanced by applying high…

We examine ice crystal growth from water vapor at temperatures near the melting point, when surface premelting creates a quasiliquid layer at the solid/vapor interface. Recent ice growth measurements as a function of vapor supersaturation…

Materials Science · Physics 2014-07-04 Kenneth G. Libbrecht

Nucleation in small volumes of water has garnered renewed interest due to the relevance of pore condensation and freezing under conditions of low partial pressures of water, such as in the upper troposphere. Molecular simulations can in…

Chemical Physics · Physics 2023-06-23 John A. Hayton , Michael B. Davies , Thomas F. Whale , Angelos Michaelides , Stephen J. Cox

To predict the radiative forcing of clouds it is necessary to know the rate with which ice homogeneously nucleates in supercooled water. Such rate is often measured in drops to avoid the presence of impurities. At large supercooling small…

Soft Condensed Matter · Physics 2020-03-06 Jorge R. Espinosa , Carlos Vega , Eduardo Sanz

In principle, the answer to the posed titular question is undoubtedly 'yes.' But in practice, requisite reference data for homogeneous systems have been obtained with a treatment of intermolecular interactions that is different from that…

Statistical Mechanics · Physics 2022-05-02 Dominic Atherton , Angelos Michaelides , Stephen J. Cox

What makes a material a good ice nucleating agent? Despite the importance of heterogeneous ice nucleation to a variety of fields, from cloud science to microbiology, major gaps in our understanding of this ubiquitous process still prevent…

Chemical Physics · Physics 2016-11-29 Martin Fitzner , Gabriele C Sosso , Stephen J Cox , Angelos Michaelides

The formation mechanism of ice banding in the system of freezing colloidal suspensions, which is of significance in frost heaving, ice-templating porous materials and biological materials, still remains a mystery. Recently, the theory of…

Materials Science · Physics 2016-12-21 Jiaxue You , Jincheng Wang , Lilin Wang , Zhijun Wang , Junjie Li , Xin Lin
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