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We combine the results of magnetic and transport measurements with neutron diffraction data to construct the structural and magnetic phase diagram of the entire family of SrMn$_{1-x}$Ru$_{x}$O$_3$ ($0 \leqslant x \leqslant 1$) perovskites.…

Materials Science · Physics 2009-11-13 S. Kolesnik , B. Dabrowski , O. Chmaissem

Comprehensive muon spin rotation/relaxation (muSR) and neutron powder diffraction (NPD) studies supported via bulk measurements have been performed on the ordered double perovskite Sr2YbRuO6 to investigate the nature of the magnetic ground…

We use \textit{ab initio} calculations to systematically study the phase diagram of multiferroic Sr$_{1-x}$Ba$_x$MnO$_3$ ($0 \leq x \leq 1$) as a function of chemical doping, epitaxial strain and external pressure. We find that by replacing…

Materials Science · Physics 2016-11-03 Hanghui Chen , Andrew J. Millis

With the motivation to study how non-magnetic ion site disorder affects the quantum magnetism of Ba3CoSb2O9, a spin-1/2 equilateral triangular lattice antiferromagnet, we performed DC and AC susceptibility, specific heat, elastic and…

Strongly Correlated Electrons · Physics 2022-03-30 Q. Huang , R. Rawl , W. W. Xie , E. S. Chou , V. S. Zapf , X. X. Ding , C. Mauws , C. R. Wiebe , E. X. Feng , H. B. Cao , W. Tian , J. Ma , Y. Qiu , N. Butch , H. D. Zhou

Density functional theory (DFT) calculations are used to study the magnetic and ferroelectric properties of Sr$_{1-x}$Ba$_{x}$MnO$_3$, with focus on $x=0.5$, under isotropic volume expansion/compression and biaxial strain. Our results…

Materials Science · Physics 2020-11-11 Alexander Edström , Claude Ederer

We have investigated the Mn-site substitution effect in Nd$_{0.45}$Sr$_{0.55}$MnO$_3$ single crystal, which has an $A$-type layered antiferromagnetic ($A$-AFM) phase with the 3$d_{x^2-y^2}$-type orbital-order. Substitution of Fe or Ga for…

Strongly Correlated Electrons · Physics 2014-02-17 Y. Izuchi , M. Akaki , D. Akahoshi , H. Kuwahara

The structural, magnetic, magnetocaloric and Griffiths phase (GP) disorder of non-stoichiometric perovskite manganites La_(0.8-x) Sr_(0.2-y) Mn_(1+x+y) O_3 are reported here. Determination of valence states and structural phases evidenced…

Materials Science · Physics 2021-12-10 Sagar Ghorai , Vitalii Shtender , Petter Ström , Ridha Skini , Peter Svedlindh

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

Strongly Correlated Electrons · Physics 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

The magnetic structure and electronic groundstate of the layered perovskite Ba2IrO4 have been investigated using x-ray resonant magnetic scattering (XRMS). Our results are compared with those for Sr2IrO4, for which we provide supplementary…

Strongly Correlated Electrons · Physics 2013-03-19 S. Boseggia , R. Springell , H. C. Walker , Ch. Rüegg , H. Okabe , M. Isobe , R. S. Perry , S. P. Collins , D. F. McMorrow

In the Fe-Mo based B-site ordered double-perovskite, A2FeMoO6.0, with iron in the mixed-valence II/III state, the valence value of Fe is not precisely fixed at 2.5 but may be fine-tuned by means of applying chemical pressure at the A-cation…

Strongly Correlated Electrons · Physics 2009-11-10 Y. Yasukawa , M. Karppinen , J. Linden , T. S. Chan , R. S. Liu , H. Yamauchi

Ga for Mn substitution in multiferroic TbMnO$_{3}$ has been performed in order to study the influence of Mn-magnetic ordering on the Tb-magnetic sublattice. Complete characterization of TbMn$_{1-x}$Ga$_x$O$_{3}$ ($x$ = 0, 0.04, 0.1)…

Strongly Correlated Electrons · Physics 2015-05-14 O. Prokhnenko , N. Aliouane , R. Feyerherm , E. Dudzik , A. U. B. Wolter , A. Maljuk , K. Kiefer , D. N. Argyriou

Disorder induced by chemical inhomogeneity and Jahn-Teller (JT) distortions is often observed in mixed valence perovskite manganites. The main reasons for the evolution of this disorder are connected with the cationic size differences and…

Materials Science · Physics 2021-11-30 Sagar Ghorai , Sergey A. Ivanov , Ridha Skini , Petter Ström , Peter Svedlindh

Powder neutron diffraction experiments have been employed to establish the effects of site-selective magnetic dilution in the Sm2MnMnMn4-x Tix O12 A-site columnar ordered quadruple perovskite manganites (x = 1, x = 2 and x = 3). We show…

Strongly Correlated Electrons · Physics 2021-01-04 Anuradha M. Vibhakar , Dmitry D. Khalyavin , Pascal Manuel , Ran Liu , Kazunari Yamaura , Alexei A. Belik , Roger D. Johnson

The perovskite ruthenates (ARuO3, A = Ca, Ba, or Sr) exhibit unique properties owing to a subtle interplay of crystal structure and electronic-spin degrees of freedom. Here, we demonstrate an intriguing continuous tuning of crystal symmetry…

Using a Dirac-Heisenberg Hamiltonian with biquadratic exchange interactions, we study the effect of iron disproportionation on the magnetic ordering, and describe the first-order magnetic transition occurring in the perovskite…

Strongly Correlated Electrons · Physics 2009-10-30 H. Kachkachi , P. Kornilovitch , Y. Meurdesoif , J. -C. Grenier , F. Zhou

Cation ordering is most common process detected in A$_{3}$B'B"$_{2}$O$_{9}$-based complex perovskites. Some important physical features of this system are due to the B-site ordering at long and short range. For microwave applications as…

Materials Science · Physics 2017-04-05 J. E. Rodrigues , D. M. Bezerra , A. C. Hernandes

In this study, the magnetic ground state of iridium perovskites (Sr$_{n+1}$Ir$_{n}$O$_{3n+1}$, where $n=1$, 2, and $\infty$) was considered using muon spin spectroscopy ($\mu$SR). When probed by muons in Sr$_2$IrO$_4$ and Sr$_3$Ir$_2$O$_7$…

Strongly Correlated Electrons · Physics 2015-04-13 M. Miyazaki , R. Kadono , M. Hiraishi , A. Koda , K. M. Kojima , K. Ohashi , T. Takayama , H. Takagi

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

Detailed structural measurements were conducted on a new perovskite, ScMnO3, and on orthorhombic LuMnO3. Complementary density functional theory (DFT) calculations were carried out, and predict that ScMnO3 possesses E-phase magnetic order…

Strongly Correlated Electrons · Physics 2015-06-19 T. Yu , T. A. Tyson , H. Y. Chen , A. M. M. Abeykoon , Y. -S. Chen , K. H. Ahn

The spin order in cubic perovskite SrFeO3 and BaFeO3 under high pressure is studied by density functional theory (DFT) calculation with local spin density approximation plus Hubbard U (LSDA+U). At ambient pressure, A-type and G-type helical…

Strongly Correlated Electrons · Physics 2015-06-11 Zhi Li , Toshiaki Iitaka , Takami Tohyama
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