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A systematic first-principles study has been performed to understand the magnetism of thin film SrRuO$_3$ which lots of research efforts have been devoted to but no clear consensus has been reached about its ground state properties. The…

Strongly Correlated Electrons · Physics 2017-07-07 Siheon Ryee , Myung Joon Han

During the past decades, approximate Kohn-Sham density-functional theory schemes garnered many successes in computational chemistry and physics; yet the performance in the prediction of spin state energetics is often unsatisfactory. By…

Other Condensed Matter · Physics 2023-05-05 Joao Paulo Almeida de Mendonca , Lorenzo A. Mariano , Emilie Devijver , Noel Jakse , Roberta Poloni

An extended around mean field (AMF) functional for less localized $p$ electrons is developed to quantify the influence of electronic correlations in $\alpha$-Ga. Both the local density approximation (LDA) and generalized gradient…

Strongly Correlated Electrons · Physics 2015-06-03 Zhiyong Zhu , Xuhui Wang , Udo Schwingenschlögl

We assess the validity of various exchange-correlation functionals for computing the structural, vibrational, dielectric, and thermodynamical properties of materials in the framework of density-functional perturbation theory (DFPT). We…

Scanning electron microscopy with polarization analysis is a powerful lab-based magnetic imaging technique offering parallel imaging of multiple magnetization components and a very high spatial resolution. However, one drawback of the…

Instrumentation and Detectors · Physics 2018-08-22 Daniel Schönke , Andreas Oelsner , Pascal Krautscheid , Robert M. Reeve , Mathias Kläui

In this contribution we assess the performance of two different exchange-correlation functionals in the first-principle prediction of the lattice thermal conductivity of bulk semiconductors, namely the local density approximation (LDA) and…

Materials Science · Physics 2018-11-16 Marco Arrigoni , Georg K. H. Madsen

Using a linear combination of atomic orbitals approach, we report a systematic comparison of various Density Functional Theory (DFT) and hybrid exchange-correlation functionals for the prediction of the electronic and structural properties…

Materials Science · Physics 2008-05-07 D. I. Bilc , R. Orlando , R. Shaltaf , G. -M. Rignanese , Jorge Íñiguez , Ph. Ghosez

A spin angular gradient approximation for the exchange correlation magnetic field in the density functional formalism is proposed. The usage of such corrections leads to a consistent spin dynamical approach beyond the local approximation.…

Strongly Correlated Electrons · Physics 2009-11-07 M. I. Katsnelson , V. P. Antropov

Magnetic properties of Mn-doped GaAs are re-investigated within a realistic multiband description of the host valence bands. We explicitely demonstrate that the recent Monte Carlo (MC) simulations performed on a large scale supercomputer…

Strongly Correlated Electrons · Physics 2011-07-26 Stefan Barthel , Gerd Czycholl , Georges Bouzerar

One of the standard generalized-gradient approximations (GGAs) in use in modern electronic-structure theory, PBE, and a recently proposed modification designed specifically for solids, PBEsol, are identified as particular members of a…

Materials Science · Physics 2015-05-13 Luana S. Pedroza , Antonio J. R. da Silva , Klaus Capelle

We extend the previously proposed one-parameter double-hybrid density-functional theory [K. Sharkas, J. Toulouse, and A. Savin, J. Chem. Phys. 134, 064113 (2011)] to meta-generalized-gradient-approximation (meta-GGA) exchange-correlation…

Chemical Physics · Physics 2014-02-27 Sidi Ould Souvi , Kamal Sharkas , Julien Toulouse

We present a global hybrid meta-generalized gradient approximation (meta-GGA) with three empirical parameters, as well as its underlying semilocal meta-GGA and a meta-GGA with only one empirical parameter. All of them are based on the new…

We establish sharp inequalities involving the incomplete Beta and Gamma functions. These inequalities arise in the approximation of generalized Bernstein functions by higher order Thorin-Bernstein functions. Furthermore, new properties of a…

Classical Analysis and ODEs · Mathematics 2024-09-05 Stamatis Koumandos , Henrik Laurberg Pedersen

A recent study of Mejia-Rodriguez and Trickey [Phys. Rev. A 96, 052512 (2017)] showed that the deorbitalization procedure (replacing the exact Kohn-Sham kinetic-energy density by an approximate orbital-free expression) applied to…

Materials Science · Physics 2018-10-10 Fabien Tran , Péter Kovács , Leila Kalantari , Georg K. H. Madsen , Peter Blaha

The magnetic ground-state configuration of iron selenide FeSe has been a topic of debate, with experimental evidence suggesting the stripe spin fluctuations as predominant at low temperatures, while density functional theory (DFT)…

Superconductivity · Physics 2025-03-21 Luke Myers , Nigel Hew , Shun-Li Shang , Zi-Kui Liu

We use time-dependent spin-density-functional theory to study dynamical magnetic phenomena. First, we recall that the local-spin-density approximation (LSDA) fails to account correctly for magnetic fluctuations in the paramagnetic state of…

Materials Science · Physics 2009-11-07 K. Capelle , B. L. Gyorffy

The discovery of ferromagnetism in Mn doped GaAs [1] has ignited interest in the development of semiconductor technologies based on electron spin and has led to several proof-of-concept spintronic devices [2-4]. A major hurdle for realistic…

Materials Science · Physics 2009-11-11 Dale Kitchen , Anthony Richardella , Jian-Ming Tang , Michael E. Flatte , Ali Yazdani

The recent TASK meta-GGA density functional [Phys. Rev. Research, 1, 033082 (2019)] is constructed with an enhanced nonlocality in the generalized Kohn-Sham scheme, and therefore harbors great opportunities for band gap prediction. Although…

Materials Science · Physics 2021-06-30 Bimal Neupane , Hong Tang , Niraj K. Nepal , Santosh Adhikari , Adrienn Ruzsinszky

The study of defects in materials is of utmost importance for technological applications and the design of new materials. In this work, we analyze the performance of density functional approximations on two prototypical sets of defective…

A meta generalized gradient level screened range-separated hybrid functional is developed for solid-state electronic structure theory. Assessment of the present range-separated hybrid functional for solid-state lattice constants and band…

Materials Science · Physics 2018-03-13 Subrata Jana , Abhilash Patra , Prasanjit Samal