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When strained beyond the linear regime, soft colloidal glasses yield to steady-state plastic flow in a way that is similar to the deformation of conventional amorphous solids. Due to the much larger size of the colloidal particles with…

Soft Condensed Matter · Physics 2017-04-12 Antina Ghosh , Zoe Budrikis , Vijayakumar Chikkadi , Alessandro Sellerio , Stefano Zapperi , Peter Schall

Inelastic deformation of metallic glasses occurs via slip events with avalanche dynamics similar to those of earthquakes. For the first time in these materials, measurements have been obtained with sufficiently high temporal resolution to…

Colloidal model systems allow for a flexible tuning of particle sizes, particle spacings and mutual interactions at constant temperature. Colloidal suspensions typically crystallize as soon as the interactions get sufficiently strong and…

Nanoparticle surface structural dynamics is believed to play a significant role in regulating functionalities such as diffusion, reactivity, and catalysis but the atomic-level processes are not well understood. Atomic resolution…

We use theory and simulations to investigate the existence of amorphous glassy states in ultrasoft colloids. We combine the hyper-netted chain approximation with mode-coupling theory to study the dynamic phase diagram of soft repulsive…

Soft Condensed Matter · Physics 2010-12-16 Ludovic Berthier , Angel J. Moreno , Grzegorz Szamel

Freezing is a fundamental physical phenomenon that has been studied over many decades; yet the role played by surfaces in determining nucleation has remained elusive. Here we report direct computational evidence of surface induced…

Statistical Mechanics · Physics 2015-05-13 T. Li , D. Donadio , L. M. Ghiringhelli , G. Galli

Surface plasmon resonances of metallic nanostructures offer great opportunities to guide and manipulate light on the nanoscale. In the design of novel plasmonic devices, a central topic is to clarify the intricate relationship between the…

Optics · Physics 2019-09-11 Sanghyeon Yu , Habib Ammari

Organisms in nature can alter the short-range order of an amorphous precursor phase, thereby controlling the resulting crystalline structure. This phenomenon inspired an investigation of the effect of modifying the short-range order within…

Materials Science · Physics 2020-01-13 Yael Etinger-Geller , Alex Katsman , Boaz Pokroy

Tribological properties of materials play an important role in engineering applications. Up to now, a number of experimental studies have identified correlations between tribological parameters and the mechanical response. Using molecular…

Computational Physics · Physics 2019-08-30 Karina E. Avila , Stefan Küchemann , Iyad Alabd Alhafez , Herbert M. Urbassek

We introduce a combined Restrained MD/Parallel Tempering approach to study the difference in free energy as a function of a set of collective variables between two states in presence of unknown slow degrees of freedom. We applied this…

Statistical Mechanics · Physics 2015-03-19 Simone Meloni , Sergio Orlandini , Giovanni Ciccotti

The influence of static stress and alternating loading direction on the potential energy and mechanical properties of amorphous alloys is investigated using molecular dynamics simulations. The model glass is represented via a binary mixture…

Soft Condensed Matter · Physics 2021-02-09 Nikolai V. Priezjev

We study the influence of the liquid-vapor surface on the crystallization kinetics of supercooled metal alloys. While a good glass former, $\rm{Cu}_{50}\rm{Zr}_{50}$, shows no evidence of surface enhancement of crystallization,…

Materials Science · Physics 2019-01-17 Chunguang Tang , Peter Harrowell

The durability of passivable metals and alloys is often limited by the stability of the surface oxide film, the passive film, providing self-protection against corrosion in aggressive environments. Improving this stability requires to…

Materials Science · Physics 2019-07-26 Li Ma , Frederic Wiame , Vincent Maurice , Philippe Marcus

We present the viability of obtaining the particle size and surface coverage in a monolayer of polystyrene particles adsorbed on a glass surface from optical coherent reflectance data around the critical angle in an internal reflection…

Systemic symmetry is introduced into our work to investigate the symmetries of different ZnO nanocrystals. Result shows that systemic symmetries obey the law of spontaneous symmetry breaking during the formation of ZnO nanocrystals. A…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Yan Zhou , Junyan Zhang , Jiangong Li , Bin Zhang

Metallic glasses response to the mechanical stress in a complex and inhomogeneous manner with plastic strain highly localized into nanoscale shear bands. Contrary to the well-defined deformation mechanism in crystalline solids,…

Materials Science · Physics 2020-07-01 Baoan Sun , Liping Yu , Gang Wang , Xing Tong , Chuan Geng , Jingtao Wang , Jingli Ren , Weihua Wang

Glasses are featured with a disordered amorphous structure, being opposite to crystals that are constituted by periodic lattices. In this study we report that the exceptional thermodynamic and kinetic stability of an ultra-stable binary…

Disordered Systems and Neural Networks · Physics 2021-11-05 Zhen Lu , Anh Khoa Augustin Lu , Fan Zhang , Yuan Tian , Jing Jiang , Daixiu Wei , Jiuhui Han , Qingyang Gao , Koji Ohara , Hidemi Kato , Akihiko Hirata , Mingwei Chen

This paper develops a general data-driven approach to stochastic elastoplastic modelling that leverages atomistic simulation data directly rather than by fitting parameters. The approach is developed in the context of metallic glasses,…

Statistical Mechanics · Physics 2024-10-02 Bin Xu , Zhao Wu , Jiayin Lu , Michael D. Shields , Chris H. Rycroft , Franz Bamer , Michael L. Falk

The kinetics and thermodynamics of structural transformations under pressure depend strongly on particle size due to the influence of surface free energy. By suitable design of surface structure, composition, and passivation it is possible,…

Materials Science · Physics 2017-04-05 Michael Grünwald , Katie Lutker , A. Paul Alivisatos , Eran Rabani , Phillip L. Geissler

Metallic glasses possess outstanding mechanical and physical properties, making them promising candidates for advanced structural and functional applications; however, the lack of understanding and control over their glass transition and…

Soft Condensed Matter · Physics 2025-06-04 Wei Chu , Zheng Wang , Christopher Ness , Konrad Samwer , Alessio Zaccone , Lina Hu