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The competition between interactions in frustrated magnets allows a wide variety of new ground states, often exhibiting emergent physics and unique excitations. Expanding the suite of lattices available for study enhances our chances of…
Atomic-scale computational modeling of technologically relevant permanent magnetic materials faces two key challenges. First, a material's magnetic properties depend sensitively on temperature, so the calculations must account for thermally…
We report a combined study of transport and thermodynamic measurements on the layered pnictide material SrAg4As2. Upon cooling, a drop in electrical and Hall resistivity, a jump in heat capacity and an increase in susceptibility and…
We present theoretical results for the underscreened Kondo lattice model with localized S=1 spins coupled to a conduction band through a Kondo coupling, $J_K$, and interacting among them ferromagnetically. We use a fermionic representation…
It is shown that the large-N approach yields two energy scales for the Kondo lattice model. The single-impurity Kondo temperature, $T_K$, signals the onset of local singlet formation, while Fermi liquid coherence sets in only below a lower…
Many tetragonal compounds LnIr$_2$Si$_2$ (Ln = lanthanoid) occur in two polymorphous phases and are therefore well suited to study the relationship between crystal structure and magnetic properties. We have grown GdIr$_2$Si$_2$ single…
We studied the crystal and magnetic structure of the La$_{1-x}$Ca$_{x}$MnO$_{3}$ compound for $(0.11\leq x\leq 0.175)$ using stoichiometric samples. For $x<0.13$ the system's ground state is insulating canted antiferromagnetic. For $0.13\le…
We report on structural, magnetic and electronic properties of Co-implanted TiO2 rutile single crystals for different implantation doses. Strong ferromagnetism at room temperature and above is observed in TiO2 rutile plates after cobalt ion…
Room-temperature ferromagnetism has been recently discovered in Co-doped TiO$_2$ rutile. Our $ab$ $initio$ density-functional theory investigations show that the substitutional Co ions incorporated into TiO$_2$ rutile tend to cluster and…
Chirality in crystals arises from the exclusive presence of proper symmetry operations, such as rotations and screw axes, while lacking improper operations like inversion, mirror planes, and roto-inversions. Crystallographic chirality is…
We report a thorough study of Y$_{0.7}$La$_{0.3}$VO$_3$ single crystals by measuring magnetic properties, specific heat, thermal conductivity, x-ray and neutron diffraction with the motivation of revealing the lattice response to the…
The structural, electronic and magnetic properties of the Kondo-lattice system CeRuSi2 are experimentally investigated and analyzed in the series of other ternary cerium compounds. This system is shown to be an excellent model system…
We report 7Li NMR, magnetic susceptibility, and heat capacity measurements on the triangular lattice Heisenberg antiferromagnet compound LiCrO2. We find that in contrast to NaCrO2, magnetic properties of LiCrO2 have a more pronounced three…
Single crystals of the new compound CeCu0.18Al0.24Si1.58 have been grown by high-temperature solution growth method using a eutectic Al-Si mixture as flux. This compound is derived from the binary CeSi2 (tetragonal ThSi2-type, Pearson…
We report the experimental observation of spin reorientation in the double perovskite Ho$_2$FeCoO$_6$. The magnetic phase transitions in this compound are characterized and studied through magnetization and specific heat, and the magnetic…
Single crystals of the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$ have been studied to determine low-temperature bulk properties, structure and the magnetic ground state. Refinements of x-ray diffraction data show that the low…
We study theoretically the lattice instability in the spin gap systems under magnetic field. With the magnetic field larger than a critical value h_{c1}, the spin gap is collapsed and the magnetization arises. We found that the lattice…
The domain structure of a MnSb$_2$Te$_4$ single crystal with a Curie temperature $T_C \approx 45~K$ was studied using the high-resolution Bitter decoration technique. Magnetotransport measurements confirm a soft ferromagnetic ordering with…
The magnetic properties of GdBaMn_{2}O_{5.0}, which exhibits charge ordering, are studied from 2 to 400 K using single crystals. In a small magnetic field applied along the easy axis, the magnetization M shows a temperature-induced reversal…
Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…