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Related papers: X-ray spectroscopy of rare-earth nickelate LuNiO$_…

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With the advancement of synchrotron radiation and free-electron laser, X-ray quantum optics has emerged as a novel frontier for exploring light-matter interactions at high photon energies. A significant challenge in this field is achieving…

Quantum Physics · Physics 2026-03-11 Zheqian Zhao , Shuxing Wang , Xiyuan Wang , Yang Su , Ziru Ma , Xinchao Huang , Linfan Zhu

The energy spectrum of topological semimetals contains protected degeneracies in reciprocal space that correspond to Weyl, Dirac, or multifold fermionic states. To exploit the unconventional properties of these states, one has to access the…

Ultrashort x-ray pulses can be used to disentangle magnetic and structural dynamics and are accordingly utilized here to study the photoexcitation of NdNiO$_3$ (NNO), a model nickelate exhibiting structural and magnetic dynamics that…

The theoretical calculation of the interaction of electromagnetic radiation with matter remains a challenging problem for contemporary $ab$ $initio$ electronic structure methods, in particular for x-ray spectroscopies. This is not only due…

Strongly Correlated Electrons · Physics 2024-01-09 Felix Sorgenfrei , Mébarek Alouani , Johan Schött , H. Johan M. Jönsson , Olle Eriksson , Patrik Thunström

Results of resonant inelastic X-ray scattering (RIXS) measurements at Fe L-edges and electronic structure calculations of LiFeAs and NaFeAs are presented. Both experiment and theory show that in the vicinity of the Fermi energy, the density…

The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic x-ray scattering (RIXS) at the forefront of photon science. Here we develop the scattering theory for RIXS…

Superconductivity · Physics 2015-04-10 Pasquale Marra , Steffen Sykora , Krzysztof Wohlfeld , Jeroen van den Brink

We determine how the elementary excitations of iridium-oxide materials, which are dominated by a strong relativistic spin-orbit coupling, appear in Resonant Inelastic X-ray Scattering (RIXS). Whereas the RIXS spectral weight at the L2 x-ray…

Strongly Correlated Electrons · Physics 2012-12-03 Luuk J. P. Ament , Giniyat Khaliullin , Jeroen van den Brink

Resonant inelastic X-ray scattering (RIXS) is used increasingly for characterizing low-energy collective excitations in materials. RIXS is a powerful probe, which often requires sophisticated theoretical descriptions to interpret the data.…

Strongly Correlated Electrons · Physics 2021-09-22 Krzysztof Bieniasz , Steven Johnston , Mona Berciu

Using a combination of spectroscopic ellipsometry and DC transport measurements, we determine the temperature dependence of the optical conductivity of NdNiO$_3$ and SmNiO$_{3}$ films. The optical spectra show the appearance of a…

Strongly Correlated Electrons · Physics 2015-10-01 J. Ruppen , J. Teyssier , O. E. Peil , S. Catalano , M. Gibert , J. Mravlje , J. -M. Triscone , A. Georges , D. van der Marel

Epitaxial strain, layer confinement and inversion symmetry breaking have emerged as powerful new approaches to control the electronic and atomic-scale structural properties in complex metal oxides. Nickelate heterostructures, based on…

Results of model calculations using exact diagonalization reveal the orbital character of states associated with different Raman loss peaks in Cu $K$-edge resonant inelastic X-ray scattering (RIXS) from La$_{2}$CuO$_{4}$. The model includes…

While defects such as oxygen vacancies in correlated materials can modify their electronic properties dramatically, understanding the microscopic origin of electronic correlations in materials with defects has been elusive. Lanthanum…

Strongly Correlated Electrons · Physics 2021-02-24 Xingyu Liao , Vijay Singh , Hyowon Park

Resonant Inelastic X-Ray Scattering (RIXS) is a well-established tool for probing excitations in a wide range of materials. The measured spectra strongly depend on the scattering geometry, via its influence on the polarization of the…

Strongly Correlated Electrons · Physics 2026-05-18 Michelangelo Tagliavini , Fabian Wenzel , Maurits W. Haverkort

Resonant Inelastic X-ray Scattering (RIXS) was used to measure the local electronic structure in few-layer exfoliated flakes of the van der Waals antiferromagnet NiPS$_3$. The resulting spectra show a systematic softening and broadening of…

Strongly Correlated Electrons · Physics 2024-02-09 M. F. DiScala , D. Staros , A. de la Torre , A. Lopez , D. Wong , C. Schulz , M. Bartkowiak , B. Rubenstein , K. W. Plumb

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

Materials Science · Physics 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We present an ab initio theory of core- and valence resonant inelastic x-ray scattering (RIXS) based on a real-space multiple scattering Green's function formalism and a quasi-boson model Hamiltonian. Simplifying assumptions are made which…

Materials Science · Physics 2011-01-25 J. J. Kas , J. J. Rehr , J. A. Soininen , P. Glatzel

The transition metal K-edge x-ray absorption near edge structure (XANES) studies have been carried on LaBO3 (B=Mn, Fe, Co, Ni), La2CuO4 and SrMnO3 compounds. The theoretical spectra have been calculated using transition metal (TM) 4p…

Strongly Correlated Electrons · Physics 2007-05-23 S. K. Pandey , S. Khalid , A. V. Pimpale

We develop a theory of resonant inelastic x-ray scattering (RIXS) at the $K$ edge in La$_2$CuO$_4$ on the basis of the Keldysh Green's function formalism. In our previous analysis (Phys. Rev. B 71, 035110 (2005)), the scattering by the…

Strongly Correlated Electrons · Physics 2015-06-25 Jun-ichi Igarashi , Takuji Nomura , Manabu Takahashi

We have revisited the valence band electronic structure of NiO by means of hard x-ray photoemission spectroscopy (HAXPES) together with theoretical calculations using both the GW method and the local density approximation + dynamical…

X-ray absorption and resonant inelastic x-ray scattering measurements are carried out on lithium nitrate LiNO$_3$. The $\sigma$ orbitals around the nitrogen atoms exhibit a large lifetime effect. Experimentally, this is manifest as an…

Materials Science · Physics 2019-09-04 John Vinson , Terrence Jach , Matthias Müller , Rainer Unterumsberger , Burkhard Beckhoff