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Exciton and polaron pair dissociation is a key functional aspect of photovoltaic devices. To improve upon the current state of interfacial transport models, we augment the existing classical models of dielectric interfaces by incorporating…

Materials Science · Physics 2017-05-08 Michael J. Waters , Daniel Hashemi , John Kieffer

Efficient energy transport is highly desirable for organic semiconductor (OSC) devices such as photovoltaics, photodetectors, and photocatalytic systems. However, photo-generated excitons in OSC films mostly occupy highly localized states…

We present here a formalism based on time-dependent density-functional theory (TDDFT) to describe characteristics of both intra- and inter-valley excitons in semiconductors, the latter of which had remained a challenge. Through the usage of…

Materials Science · Physics 2023-05-10 Jia Shi , Volodymyr Turkowski , Duy Le , Talat S. Rahman

We study theoretically fundamental Coulomb-correlated complexes: neutral and charged excitons, also known as trions, in transition metal dichalogenides monolayers. We focus on the situation where one of the electrons occupies excited,…

Mesoscale and Nanoscale Physics · Physics 2023-03-23 M. A. Semina , J. V. Mamedov , M. M. Glazov

Two dimensional (2D) van der Waals heterostructures from transition metal dichalcogenide (TMDC) semiconductors show a new class of spatially separate excitons with extraordinary properties. The interlayer excitons (XI) have been studied…

Materials Science · Physics 2021-03-02 Jaehoon Ji , Jong Hyun Choi

This work quantifies the effect of misfit and threading dislocations on the surface energies of PbTe-PbSe interfaces, with the defect structures of the interfaces being obtained from atomistic and multiscale simulations of their…

Materials Science · Physics 2026-03-05 Emir Bilgili , Nicholas Taormina , Yang Li , Adrian Diaz , Simon R. Phillpot , Youping Chen

We study the refraction effect of electronic wave in hole-doped lateral heterojunctions of metallic and semiconducting transition-metal dichalcogenide monolayers. This effect is theoretically investigated in 2$H$-type MoSe$_2$-NbS$_2$ and…

Mesoscale and Nanoscale Physics · Physics 2019-10-01 Tetsuro Habe

We have theoretically investigated the spin- and valley-dependent superfluidity properties of indirect momentum space dark dipolar excitons in double layers with massive anisotropic tilted semi-Dirac bands in the presence of circularly…

Mesoscale and Nanoscale Physics · Physics 2024-01-23 A. Nafis Arafat , Oleg L. Berman , Godfrey Gumbs

Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic…

Optics · Physics 2022-03-11 J. S. Duan

Because of the reduced dielectric screening and enhanced Coulomb interactions, two-dimensional (2D) materials like phosphorene and transition metal dichalcogenides (TMDs) exhibit strong excitonic effects, resulting in fascinating…

Materials Science · Physics 2019-11-04 Xiaoyang Zheng , Xian Zhang

We carry out a detailed theoretical study of the electronic and optical properties of bulk and monolayer bismuth triiodide (BiI$_{3}$), a layered metal halide, using the ab initio GW+BSE scheme with a full spinorial formulation. We discuss…

We report that dark excitons can have a large contribution to the emission intensity in carbon nanotubes due to an efficient exciton conversion from a dark state to a bright state. Time-resolved photoluminescence measurements are used to…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 A. Ishii , H. Machiya , Y. K. Kato

Oxide heterointerfaces are ideal for investigating strong correlation effects to electron transport, relevant for oxide-electronics. Using hot-electrons, we probe electron transport perpendicular to the La$_{0.7}$Sr$_{0.3}$MnO$_{3}$ (LSMO)-…

When transition-metal dichalcogenide monolayers lack inversion symmetry, their low-energy single particle spectrum can described by tilted massive Dirac Hamiltonians. The so-called Janus materials fall into that category. Inversion symmetry…

Mesoscale and Nanoscale Physics · Physics 2022-09-15 M. F. C. Martins Quintela , A. T. Costa , N. M. R. Peres

We investigate the two-pulse photon echo response of excitons in the mixed lead halide perovskite crystal \sample in dependence on the excitation intensity and polarization of the incident laser pulses. Using spectrally narrow picosecond…

Exciton dissociation plays a crucial role in the performance of optoelectronic devices based on two-dimensional (2D) transition metal dichalcogenides (TMDs). In this work, we investigate the effect of an in-plane electric field on the…

Materials Science · Physics 2024-10-11 Tao Zhu , Chenhang Zheng , Lei Xu , Ming Yang

The gas of interacting excitons in quantum wells is studied. We obtain the Hamiltonian of this gas by the projection of the electron-hole plasma Hamiltonian to exciton states and an expansion in a small density. Matrix elements of the…

Condensed Matter · Physics 2009-10-31 S. Ben-Tabou de-Leon , B. Laikhtman

Heterostructures made from 2D transition-metal dichalcogenides are known as ideal platforms to explore excitonic phenomena ranging from correlated moir\'e excitons to degenerate interlayer exciton ensembles. So far, it is assumed that the…

The multivalley band structure of monolayer transition metal dichalcogenides (TMDs) gives rise to intravalley and intervalley excitons. Much knowledge of these excitons has been gained, but fundamental questions remain, such as how to…

Mesoscale and Nanoscale Physics · Physics 2021-12-08 Ngoc-Cam Hoang , Thanh-Phuc Nguyen , Vladimir A. Osipov

The optical orientation and alignment of excitons in semiconductor indirect gap quantum dots have been studied theoretically. A special regime is analyzed in which the energy of the hyperfine interaction of an electron with lattice nuclei…

Mesoscale and Nanoscale Physics · Physics 2024-05-27 D. S. Smirnov , E. L. Ivchenko
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