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We divide glass and viscous liquid sciences into two major research areas, the first dealing with how to avoid crystals and so access the viscous liquid state, and the second dealing with how liquids behave when no crystals form. We review…

Disordered Systems and Neural Networks · Physics 2009-11-13 C. Austen Angell

Evolutionary crystal structure prediction proved to be a powerful approach for studying a wide range of materials. Here, we present a specifically designed algorithm for the prediction of the structure of complex crystals consisting of…

Materials Science · Physics 2012-05-21 Qiang Zhu , Artem R. Oganov , Colin W. Glass , Harold T. Stokes

We examine the molecular dynamics of crystal growth in the presence of surface melting and surface impurities, and from this propose a detailed microscopic model for the growth of ice from the vapor phase. Our model naturally accounts for…

Materials Science · Physics 2008-10-06 Kenneth G. Libbrecht

We present a kinetic model of crystal growth of polymers of finite molecular weight. Experiments help to classify polymer crystallization broadly into two kinetic regimes. One is observed in melts or in high molar mass polymer solutions and…

Soft Condensed Matter · Physics 2009-11-11 Arindam Kundagrami , M. Muthukumar

Crystallization and vitrification are two different routes to form a solid. Normally these two processes suppress each other, with the glass transition preventing crystallization at high density (or low temperature). This is even true for…

Soft Condensed Matter · Physics 2014-08-26 Ran Ni , Martien A. Cohen Stuart , Marjolein Dijkstra , Peter G. Bolhuis

The competition between crystallization and vitrification in glass-forming materials manifests as a non-monotonic behavior in the time-temperature transformation (TTT) diagrams, which quantify the time scales for crystallization as a…

Statistical Mechanics · Physics 2025-10-16 Muhammad R. Hasyim , Kranthi K. Mandadapu

Finding an optimal match between two different crystal structures underpins many important materials science problems, including describing solid-solid phase transitions, developing models for interface and grain boundary structures. In…

Materials Science · Physics 2020-02-21 Félix Therrien , Peter Graf , Vladan Stevanović

We study a quasi-two-dimensional macroscopic system of magnetic spherical particles settled on a shallow concave dish under a temporally oscillating magnetic field. The system reaches a stationary state where the energy losses from…

Soft Condensed Matter · Physics 2021-10-13 A. Escobar , F. Donado , R. E. Moctezuma , Eric R. Weeks

Efficient heuristics have predicted many functional materials such as high-temperature superconducting hydrides, while inorganic structural chemistry explains why and how the crystal structures are stabilized. Here we develop the paired…

Materials Science · Physics 2024-11-07 Ryotaro Koshoji , Taisuke Ozaki

The nucleation of crystals in liquids is one of nature's most ubiquitous phenomena, playing an important role in areas such as climate change and the production of drugs. As the early stages of nucleation involve exceedingly small time and…

The kinetics and microstructure of solid-phase crystallization under continuous heating conditions and random distribution of nuclei are analyzed. An Arrhenius temperature dependence is assumed for both nucleation and growth rates. Under…

Materials Science · Physics 2017-04-26 J. Farjas , P. Roura

Understanding the growth of quasicrystals poses a challenging problem, not the least because the quasiperiodic order present in idealized mathematical models of quasicrystals prohibit simple local growth algorithms. This can only be…

Disordered Systems and Neural Networks · Physics 2007-05-23 Uwe Grimm , Dieter Joseph

We study a crystal growth Markov model proposed by Gates and Westcott (\cite{Kinetics1}, \cite{Kinetics2}). This is an aggregation process where particles are packed in a square lattice accordingly to prescribed deposition rates. This model…

Probability · Mathematics 2012-11-07 François Ezanno

The growth of quasicrystals, i.e., aperiodic structures with long-range order, seeded from the melt is investigated using a dynamical phase field crystal model. Depending on the thermodynamic conditions, two different growth modes are…

Soft Condensed Matter · Physics 2014-07-31 C. V. Achim , M. Schmiedeberg , H. Löwen

Gaining fundamental understanding of crystal nucleation processes in metal alloys is crucial for the development and design of high-performance materials with targeted properties. Yet, crystallization is a complex non-equilibrium process…

Materials Science · Physics 2022-12-09 Grisell Díaz Leines , Angelos Michaelides , Jutta Rogal

We study the evolution from a liquid to a crystal phase in two-dimensional curved space. At early times, while crystal seeds grow preferentially in regions of low curvature, the lattice frustration produced in regions with high curvature is…

Soft Condensed Matter · Physics 2015-06-16 Nicolas A. Garcia , Richard A. Register , Daniel A. Vega , Leopoldo R. Gomez

We propose a model for the abrupt emergence, below temperatures close to the glass transition, of the ultra-fast (GC) steady mode of spherulitic crystal growth in deeply undercooled liquids. We interpret this phenomenon as controlled by the…

Materials Science · Physics 2015-06-05 Christiane Caroli , Anaël Lemaître

One of water's unsolved puzzles is the question of what determines the lowest temperature to which it can be cooled before freezing to ice. The supercooled liquid has been probed experimentally to near the homogeneous nucleation temperature…

Soft Condensed Matter · Physics 2011-12-08 Emily B. Moore , Valeria Molinero

Recently, a universal relation between the thermal expansion coefficient of glasses $\alpha_g$, their glass-transition temperature Tg, and the so-called fragility index m of the corresponding supercooled liquid state was found to be valid…

Soft Condensed Matter · Physics 2024-10-29 P. Lunkenheimer , K. Samwer , A. Loidl

The phase-field model for the description of the solidification processes with the glass-crystal competition is suggested. The model combines the first-order phase transition model in the phase-field formalism and gauge-field theory of…

Materials Science · Physics 2024-08-07 M. G. Vasin , V. Ankudinov