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We have used the convergent close-coupling method and a unitarized first-order many-body theory to calculate integral cross sections for elastic scattering and momentum transfer, for excitation of the 5d^2 ^1S, 6s6p^1P_1, 6s7p^1P_1,…

Atomic Physics · Physics 2009-10-31 D. V. Fursa , S. Trajmar , I. Bray , I. Kanik , G. Csanak , R. E. H. Clark , J. Abdallah

We consider the nonequilibrium quantum vibrations of a molecule clamped between two macroscopic leads in a current-carrying state at finite voltages. Our approach is based on the nonequilibrium Green function technique and the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 D. A. Ryndyk , M. Hartung , G. Cuniberti

Differential cross sections are computed for the title polar molecule using static interaction, exchange forces and correlation-polarisation effects as described in detail in the main text. The dipole effect is also reported via the dipole…

Chemical Physics · Physics 2009-11-13 F. A. Gianturco , T. Stoecklin

A phenomenological optical potential is generalized to include the Coulomb and nuclear interactions caused by the dynamical deformation of its surface. In the high-energy approach analytical expressions for elastic and inelastic scattering…

Nuclear Theory · Physics 2009-11-11 V. K. Lukyanov , Z. Metawei , E. V. Zemlyanaya

We report first ns-resolved absorption measurements of the ro-vibrational excitation of CO$_2$. The high temporal resolution of 8 ns is made possible by a fast detector (rise-time 5 ns), sensitive in the mid-infrared region. The resolution…

Plasma Physics · Physics 2021-07-02 Yanjun Du , Tsanko V Tsankov , Dirk Luggenhölscher , Uwe Czarnetzki

A general theory of electronic excitations in aggregates of molecules coupled to intramolecular vibrations and the harmonic environment is developed for simulation of the third-order nonlinear spectroscopy signals. The model is applied in…

Chemical Physics · Physics 2014-01-17 Vytautas Butkus , Leonas Valkunas , Darius Abramavicius

The cross section for dissociative recombination of BeH^+ is calculated by solution of the time-dependent Schrodinger equation in the local complex potential approximation. The effects of couplings between resonant states and the Rydberg…

Atomic Physics · Physics 2009-04-02 J. B. Roos , M. Larsson , AA. Larson , A. E Orel

The influence of dispersion on the differential scattering cross section in the vicinity of the first diffraction minimum is revisited for collision energies between 200 and 450 MeV. Transient nuclear excitations in the giant resonance…

Nuclear Theory · Physics 2026-03-12 D. H. Jakubassa-Amundsen

New cross sections for the rotational excitation of H$_3^+$ by electrons are calculated {\it ab initio} at low impact energies. The validity of the adiabatic-nuclei-rotation (ANR) approximation, combined with $R$-matrix wavefunctions, is…

Atomic Physics · Physics 2009-11-13 A. Faure , V. Kokoouline , Chris H. Greene , Jonathan Tennyson

We consider the excitation of single-electron wave packets by means of a time dependent voltage applied to the ballistic edge channels of the integer quantum Hall effect at filling factor $\nu=2$. Due to electron-electron interactions,…

Mesoscale and Nanoscale Physics · Physics 2018-07-23 Matteo Acciai , Matteo Carrega , Jérôme Rech , Thibaut Jonckheere , Thierry Martin , Maura Sassetti

Long-term simulations of energetic electron fluxes in many space plasma systems require accounting for two groups of processes with well separated time-scales: microphysics of electron resonant scattering by electromagnetic waves and…

Plasma Physics · Physics 2021-10-04 A. S. Lukin , A. V. Artemyev , A. A. Petrukovich

The article reports electron-impact excitation cross-sections and rate coefficients for neutral tungsten for three transitions (400.87 nm, 429.46 nm, and 430.21 nm) using the relativistic distorted wave approach within the flexible atomic…

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

Atomic Physics · Physics 2017-11-21 V. Mosert , D. Bauer

Differential cross sections for electromagnetic dissociation in nucleus-nucleus collisions are calculated. The kinetic energy distribution is parameterized with a Boltzmann distribution and the angular distribution is assumed isotropic in…

Nuclear Theory · Physics 2008-11-26 John W. Norbury , Anne Adamczyk

Molecular adsorbates on metal surfaces exchange energy with substrate phonons and low-lying electron-hole pair excitations. In the limit of weak coupling, electron-hole pair excitations can be seen as exerting frictional forces on…

Materials Science · Physics 2016-09-28 Reinhard J. Maurer , Mikhail Askerka , Victor S. Batista , John C. Tully

One of the most important parameters in a collision is the 'miss distance' or impact parameter, which in quantum mechanics is described by quantized partial waves. Usually, the collision outcome is the result of unavoidable averaging over…

Non-equilibrium vibrational dissociation of CO$_2$ at low translational-rotational temperatures $T$ is investigated computationally for conditions of microwave induced plasmas. Semi-analytic treatment of vibrational relaxation in CO$_2$ in…

Plasma Physics · Physics 2022-09-08 Vladislav Kotov

We propose a semi-empirical formula for the cross section of ionization by electron impact. The formula involves adjustable parameters which are determined by comparison with measured or numerically calculated cross sections. In the latter…

Atomic Physics · Physics 2024-04-09 Djamel Benredjem , Jean-Christophe Pain

We present a perturbation approach rooted in time-dependent density-functional theory to calculate electron hole (eh)-pair excitation spectra during the non-adiabatic vibrational damping of adsorbates on metal surfaces. Our analysis for the…

Chemical Physics · Physics 2017-11-22 Simon P. Rittmeyer , Jörg Meyer , Karsten Reuter

In this article, we propose a generalized model for nonequilibrium vibrational energy distribution functions. The model can be used, in place of equilibrium (Boltzmann) distribution functions, when deriving reaction rate constants for…

Chemical Physics · Physics 2020-07-15 Narendra Singh , Thomas Schwartzentruber