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The electrocaloric effect (ECE) offers a promising alternative to the traditional gas compressing refrigeration due to its high efficiency and environmental friendliness. The unusual negative electrocaloric effect refers to the adiabatic…

Materials Science · Physics 2023-07-14 Xingyue Ma , Mingxing Chen , Jun-Ming Liu , Di Wu , Yurong Yang

The giant electro- and elasto-caloric effects in spin chain materials are predicted. The theory is based on the exact quantum mechanical solution of the problem. It is shown that the giant jumps in the entropy and the temperature caused by…

Quantum Physics · Physics 2024-06-27 A. A. Zvyagin , V. V. Slavin

In acceptor doped ferroelectrics and in ferroelectric films and nanocomposites, defect dipoles, strain gradients, and the electric boundary conditions at interfaces and surfaces often impose internal bias fields. In this work we delicately…

Materials Science · Physics 2018-09-05 Yang-Bin Ma , Bai-Xiang Xu , Karsten Albe , Anna Grünebohm

We use molecular dynamics with a first-principles-based shell model potential to study the electrocaloric effect (ECE) in lithium niobate, LiNbO$_3$, and find a giant electrocaloric effect along a line passing through the ferroelectric…

Materials Science · Physics 2012-11-08 Maimon C. Rose , R. E. Cohen

Giant electrocaloric (EC) effect is observed in BaTiO3 multilayer thick film structure. The temperature change is as high as 4.0 oC under an applied electric field of 352 kV/cm. Most importantly, the EC effect is found to depend on the…

Materials Science · Physics 2015-05-18 Yang Bai , Guang-Ping Zheng , San-Qiang Shi

An atomistic effective Hamiltonian is used to investigate electrocaloric (EC) effects of Pb(Mg$_{1/3}$Nb$_{2/3}$)O$_{3}$ (PMN) relaxor ferroelectrics in its ergodic regime, and subject to electric fields applied along the pseudocubic [111]…

Materials Science · Physics 2018-04-03 Zhijun Jiang , Y. Nahas , S. Prokhorenko , S. Prosandeev , D. Wang , Jorge Íñiguez , L. Bellaiche

The electrocaloric effect (ECE) in normal and relaxor ferroelectrics is investigated in the framework of a thermodynamic approach based on the Maxwell relation and a Landau-type free energy model. The static dielectric response of relaxors…

Disordered Systems and Neural Networks · Physics 2015-05-20 R. Pirc , Z. Kutnjak , R. Blinc , Q. M. Zhang

A material with reversible temperature change capability under an external electric field, known as the electrocaloric effect (ECE), has long been considered as a promising solid-state cooling solution. However, electrocaloric (EC)…

We show that the electrocaloric (EC) effect -- e.g., the temperature change experienced by an insulator upon application of an electric bias -- lends itself to a straightforward interpretation when expressed as a Taylor series in the…

Materials Science · Physics 2020-12-09 Mónica Graf , Jorge Íñiguez

There is a surge of interest in developing environmentally friendly cooling technology based on the solid--state electrocaloric effect (ECE). Here, we point out that negative ECE with a fast cooling rate ($\approx$10$^{11}$ K/s) can be…

Materials Science · Physics 2018-02-07 Yubo Qi , Shi Liu , Aaron M. Lindenberg , Andrew M. Rappe

The electrocaloric (EC) effect is the reversible change in temperature and/or entropy of a material when it is subjected to an adiabatic electric field change. Our tight-binding calculations linked to Fermi statistics, show that the EC…

Mesoscale and Nanoscale Physics · Physics 2021-01-11 Natalia Cortés , Oscar Negrete , Francisco J. Peña , Patricio Vargas

Physical nature of "giant" magnetocaloric and electrocaloric effects, MCE and ECE, is explained in terms of the new fundamentals of phase transitions, ferromagnetism and ferroelectricity. It is the latent heat of structural…

Materials Science · Physics 2013-06-04 Vitaly J. Vodyanoy , Yuri Mnyukh

Recent progress on caloric effects are reviewed. The application of external stimuli such as magnetic field, hydrostatic pressure, uniaxial stress and electric field give rise respectively to magnetocaloric, barocaloric, elastocaloric and…

Materials Science · Physics 2013-03-18 Lluis Manosa , Antoni Planes , Mehmet Acet

The electrocaloric effect (ECE) in BaTiO3 is simulated using two different first-principles based effective Hamiltonian molecular dynamics methods. The calculations are performed for a wide range of temperatures (30--900 K) and external…

Materials Science · Physics 2013-11-12 Takeshi Nishimatsu , Jordan A. Barr , Scott P. Beckman

The magneto-caloric effect (MCE), which is the refrigeration based on the variation of the magnetic entropy, is of great interest in both technological applications and fundamental research. The MCE is quantified by the magnetic Gr\"uneisen…

Strongly Correlated Electrons · Physics 2019-09-04 Gabriel Gomes , Lucas Squillante , A. C. Seridonio , Andreas Ney , Roberto E. Lagos , Mariano de Souza

Anomalous electrocaloric effect (ECE) with decreasing temperature upon application of an electric field is known to occur in antiferroelectrics (AFEs), and previous understanding refers to the field-induced canting of electric dipoles if…

Materials Science · Physics 2022-12-28 Ningbo Fan , Jorge Íñiguez , L. Bellaiche , Bin Xu

\textit{Ab initio} quantum Monte Carlo (QMC) methods in principle allow for the calculation of exact properties of correlated many-electron systems, but are in general limited to the simulation of a finite number of electrons $N$ in…

Statistical Mechanics · Physics 2021-04-21 Tobias Dornheim , Jan Vorberger

Solid-state cooling applications based on the electrocaloric (EC) effect are particularly promising from a technological point of view due to their downsize scalability and natural implementation in circuitry. However, EC effects typically…

Materials Science · Physics 2023-07-19 César Menéndez , Claudio Cazorla

We describe magneto-, baro- and elastocaloric effects (MCEs, BCEs and eCEs) in materials which possess both discontinuous (first-order) and continuous (second-order) magnetic phase transitions. Our ab initio theory of the interacting…

Materials Science · Physics 2020-06-03 Eduardo Mendive-Tapia , Julie B. Staunton

In the framework of solid-state cooling technology, four kinds of caloric effects, magnetocaloric (MC), electrocaloric (EC), barocaloric (BC) and elastocaloric (eC) effects, are compared in view of environment discussion and application…

Materials Science · Physics 2016-04-21 Zhongjian Xie , Gael Sebald , Daniel Guyomar
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