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The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…

We report the realization and characterization of parametric amplification in high harmonic generation around 100 eV using He gas in a double gas jet arrangement. The delay of the seed XUV pulse with respect to the amplifier gas jet was…

We present a scheme for amplifying an extreme-ultraviolet (XUV) seed isolated attosecond pulse via stimulated Raman scattering of a pulse-train pump. At sufficient seed and pump intensity, the amplification is nonlinear, and the amplitude…

Plasma Physics · Physics 2022-10-24 Andréas Sundström , Mickael Grech , István Pusztai , Caterina Riconda

Attosecond science promises to reveal the most fundamental electronic dynamics occurring in matter and it can develop further by meeting two linked technological goals related to high-order harmonic sources: higher photon flux (permitting…

We suggest a technique to amplify a train of attosecond pulses, produced by high-harmonic generation (HHG) of an infrared (IR) laser field, in an active medium of a plasma-based X-ray laser. This technique is based on modulation of…

The field of attosecond physics has expanded significantly in recent years, yet experimental facilities supporting attosecond pump attosecond probe spectroscopy remain rare. Here, we present a newly constructed beamline for the generation…

High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…

We study the generation of attosecond XUV pulses via high-order frequency mixing (HFM) of two intense generating fields, and compare this process with the more common high-order harmonic generation (HHG) process. We calculate the…

Optics · Physics 2023-08-07 V. A. Birulia , M. A. Khokhlova , V. V. Strelkov

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to…

The interaction of high-intensity laser pulses and solid targets provides a promising way to create compact, tunable and bright XUV attosecond sources that can become a unique tool for a variety of applications. However, it is important to…

Plasma Physics · Physics 2018-10-17 M. Blanco , M. T. Flores-Arias , A. Gonoskov

Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…

Paraxial light skyrmions are topological configurations that map a spatial domain of the field onto the full Poincar\'e sphere of polarization states. While optical skyrmions have been explored in continuous-wave regimes, their realization…

Optics · Physics 2025-10-17 David Marco , Luis Plaja , Carlos Hernández-García

Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…

Atomic Physics · Physics 2016-06-08 S. M. Teichmann , F. Silva , S. L. Cousin , M. Hemmer , J. Biegert

We present the first direct experimental confirmation of attosecond pulse generation in the hard X-ray regime with a free-electron laser. Our experiment is based on measurements of a nonlinear optical phenomenon known as amplified…

We study high-order harmonic generation (HHG) driven by seeded plasmonic-enhanced fields. On one hand, plasmonic-enhanced fields have shown a great potential to extend the HHG cutoff, an instrumental pre-requisite for the generation of…

Atomic Physics · Physics 2018-12-12 Irfana N. Ansari , M. S. Mrudul , Marcelo F. Ciappina , Maciej Lewenstein , Gopal Dixit

We study theoretically the effect of the giant resonance in Xe on the phase difference between the consecutive high order resonantly-enhanced harmonics and calculate the duration of the attosecond pulses produced by these harmonics. For…

Atomic Physics · Physics 2016-12-28 V. V. Strelkov

Lasers capable of generating attosecond X-ray pulses in the water window (282 to 533 eV) through high-order harmonic generation are normally based on inefficient, multi-stage optical parametric amplifiers or optical parametric chirped pulse…

We investigate the production of an isolated attosecond pulse~(IAP) via the phase-matching gating of high-harmonic generation by intense laser pulses. Our study is based on the integration of the propagation equation for the fundamental and…

Optics · Physics 2023-09-12 Vasily V. Strelkov , Margarita A. Khokhlova

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso
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