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Molecular dynamics simulation of a generic polymer model is applied to study melts of polymers with different types of intrinsic stiffness. Important static observables of the single chain such as gyration radius or persistence length are…

Soft Condensed Matter · Physics 2017-09-13 Roland Faller , Alexander Kolb , Florian Müller-Plathe

The interplay of geometrical and topological entanglement in semiflexible knotted polymer rings confined inside a spherical cavity is investigated using advanced numerical methods. By using stringent and robust algorithms for locating…

Soft Condensed Matter · Physics 2011-11-15 Luca Tubiana , Enzo Orlandini , Cristian Micheletti

A tight binding model for scanning tunneling microscopy images of a molecule adsorbed on a metal surface is described. The model is similar in spirit to that used to analyze conduction along molecular wires connecting two metal leads and…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yoel Calev , Hezy Cohen , Gianaurelio Cuniberti , Abraham Nitzan , Danny Porath

We perform Monte Carlo simulations to study the elastic properties of the helix-coil worm-like chain model of alpha-helical polypeptides. In this model the secondary structure enters as a scalar (Ising like) variable that controls the local…

Soft Condensed Matter · Physics 2007-05-23 Buddhapriya Chakrabarti , Alex J. Levine

The spatial correlations of entangled polymer dynamics are examined by molecular dynamics simulations and neutron spin-echo spectroscopy. Due to the soft nature of topological constraints, the initial spatial decays of intermediate…

We calculate correlation functions in matrix models modified by trace-squared terms. First we study scaling operators in modified one-matrix models and find that their correlation functions satisfy modified Virasoro constraints. Then we…

High Energy Physics - Theory · Physics 2016-09-06 J. L. F. Barbón , K. Demeterfi , I. ~R. Klebanov , C. Schmidhuber

We present a new simulation technique to study systems of polymers functionalized by reactive sites that bind/unbind forming reversible linkages. Functionalized polymers feature self-assembly and responsive properties that are unmatched by…

Soft Condensed Matter · Physics 2018-04-18 Bernardo Oyarzún , Bortolo Matteo Mognetti

Loop formation between monomers in the interior of semiflexible chains describes elementary events in biomolecular folding and DNA bending. We calculate analytically the interior distance distribution function for semiflexible chains using…

Soft Condensed Matter · Physics 2009-11-11 Changbong Hyeon , D. Thirumalai

We consider a fully directed self-avoiding walk model on a cubic lattice to mimic the conformations of an infinitely long confined flexible polymer chain; and the confinement condition is achieved by two parallel athermal plates. The…

Soft Condensed Matter · Physics 2021-06-21 P K Mishra

We study the conformations of a semiflexible chain, confined in nano-scaled spherical cavities, under two distinct processes of confinement. Radial contraction and packaging are employed as two confining procedures. The former method is…

Soft Condensed Matter · Physics 2014-09-29 Arman Fathizadeh , Maziar Heidari , Behrouz Eslami-Mossallam , Mohammad Reza Ejtehadi

Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

The correlations in the motion of reptating polymers in their melt are investigated by means of kinetic Monte Carlo simulations of the three dimensional slithering snake version of the bond-fluctuation model. Surprisingly, the slithering…

Statistical Mechanics · Physics 2009-11-07 L. Mattioni , J. P. Wittmer , J. Baschnagel , J. -L. Barrat , E. Luijten

If a semiflexible polymer confined to a narrow channel bends around by 180 degrees, the polymer is said to exhibit a hairpin. The equilibrium extension statistics of the confined polymer are well understood when hairpins are vanishingly…

We investigate theoretically the effect of polymer tension on the collective behavior of reversibly binding cross-links. For this purpose, we employ a model of two weakly bending wormlike chains aligned in parallel by a tensile force, with…

Biological Physics · Physics 2015-02-10 Panayotis Benetatos , Alice von der Heydt , Annette Zippelius

Spin correlation functions (up to the 3-site one) of disordered Ising model with the nearest neighbour interaction are calculated and investigated within a two-site cluster approximation for both quenched and annealed cases. The approach…

Condensed Matter · Physics 2007-05-23 R. R. Levitskii , S. I. Sorokov

I propose a variation of the standard worm--like chain model to account for internal order parameter (helix/coil) fields on the polymer chain. This internal order parameter field influences polymer conformational statistics by locally…

Soft Condensed Matter · Physics 2007-05-23 Alex J. Levine

A formula is derived for stiffness of a polymer chain in terms of the distribution function of end-to-end vectors. This relationship is applied to calculate the stiffness of Gaussian chains (neutral and carrying electric charges at the…

Statistical Mechanics · Physics 2007-05-23 A. D. Drozdov

Analytical relations for the mechanical response of single polymer chains are valuable for modeling purposes, on both the molecular and the continuum scale. These relations can be obtained using statistical thermodynamics and an idealized…

Statistical Mechanics · Physics 2023-10-02 Michael R. Buche , Meredith N. Silberstein , Scott J. Grutzik

Single-chain elasticity of polyethylene at $\theta$ point up to 90% of stretching with respect to its contour length is computed by Monte-Carlo simulation of an atomistic model in continuous space. The elasticity law together with the…

Soft Condensed Matter · Physics 2009-11-07 John T. Titantah , Carlo Pierleoni , Jean-Paul Ryckaert

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis
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