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We perform molecular dynamics simulations of ionic liquids confined between graphene walls under a large variety of conditions (pure ionic liquids, mixtures with water and alcohols, mixtures with lithium salts and defective graphene walls).…

The electrified solid-liquid interface plays an essential role in many renewable energy-related applications, including hydrogen production and utilization. Limitations in computational modelling of the electrified solid-liquid interface…

We study the competition between the electron liquid and solid phases, such as Wigner crystal and bubbles, in partially filled Landau levels (LLs) of multilayer graphene. Graphene systems offer a versatile platform for controlling band…

Mesoscale and Nanoscale Physics · Physics 2023-12-21 Rakesh K. Dora , Ajit C. Balram

The interactions of ionic liquids (ILs) with organic solutes are of interest to many applications involving the use of ILs as task-specific solvents, such as in sensing devices or catalysis. However, currently little is known about these…

Chemical Physics · Physics 2023-11-06 Clare Xie Yijia , Julian Becker , Tom Welton , Patricia Hunt

Graphene-water interaction has been under scrutiny ever since graphene discovery and realization of its exceptional properties. Several computational and experimental reports exist that have tried to look into the interactions involved,…

Materials Science · Physics 2020-02-19 Priyanka Solanky , Vidushi Sharma , Kamalika Ghatak , Jatin Kashyap , Dibakar Datta

We formulate a general mean-field theory of a flat electric double layer in ionic liquids and electrolyte solutions with ions possessing static polarizability and a permanent dipole moment on a charged electrode. We establish a new…

Statistical Mechanics · Physics 2021-08-17 Yu. A. Budkov , S. V. Zavarzin , A. L. Kolesnikov

A Dirac-Fermi liquid (DFL)--a doped system with Dirac spectrum--is an important example of a non-Galilean-invariant Fermi liquid (FL). Real-life realizations of a DFL include, e.g., doped graphene, surface states of three-dimensional (3D)…

Strongly Correlated Electrons · Physics 2021-07-28 Prachi Sharma , Alessandro Principi , Dmitrii L. Maslov

The interaction between graphene and copper (111) surface have been investigated using the molecular dynamics simulations. We have shown that it is possible to fit Lennard-Jones potential leading to the correct values of the binding energy…

Mesoscale and Nanoscale Physics · Physics 2016-11-03 A. V. Sidorenkov , S. V. Kolesnikov , A. M. Saletsky

We present a theory of the hydrodynamic forces in the drainage flow of an electrolyte between a sphere and a plane with charged surfaces. Our theory considers a thin electrolyte film which is at all times in local equilibrium across its…

Soft Condensed Matter · Physics 2025-04-01 C. Cramail , R. Lhermerout , E. Charlaix

Using a scanning electron microscope, we observed a reproducible, discrete distribution of secondary electron intensity stemming from an atomically thick graphene film on a thick insulating substrate. The discrete distribution made it…

Materials Science · Physics 2010-09-29 Hidefumi Hiura , Hisao Miyazaki , Kazuhito Tsukagoshi

Room temperature ionic liquids (ILs) at solid surfaces have been recognized for their significant interfacial properties in electrochemical and electronic devices. To ascertain the interface effects, we investigate dynamical and structural…

Chemical Physics · Physics 2017-10-27 Tamisra Pal , Constantin Beck , Dominik Lessnich , Michael Vogel

The vertical integration of multiple two-dimensional (2D) materials in heterostructures, held together by van der Waals forces, has opened unprecedented possibilities for modifying the (opto-)electronic properties of nanodevices. Graphene,…

Graphene flakes were produced by nanosecond plasma discharge at atmospheric pressure between an electrode and the surface of distilled water, in which were placed graphite flakes. The discharge ionizes the gas and forms free radicals on the…

Atomically thin crystals have recently been the focus of attention in particular after the synthesis of graphene, a monolayer hexagonal crystal structure of carbon. In this novel material class the chemically derived graphenes have…

Materials Science · Physics 2015-02-23 H. Sahin , O. Leenaerts , S. K. Singh , F. M. Peeters

Evidence is accumulating for the crucial role of a solid's free electrons in the dynamics of solid-liquid interfaces. Liquids induce electronic polarization and drive electric currents as they flow; electronic excitations, in turn,…

Mesoscale and Nanoscale Physics · Physics 2023-06-27 Xiaoqing Yu , Alessandro Principi , Klaas-Jan Tielrooij , Mischa Bonn , Nikita Kavokine

Climate emergency has led to the investigation of CO$_{2}$ valorization routes. A competitive process included in this framework is the catalytic CO$_{2}$ cycloaddition to epoxides, to produce cyclic carbonates. Halide-based Ionic liquids…

Soft Condensed Matter · Physics 2025-03-17 Sergio Dorado-Alfaro , Elisa Hernández , Jesús Algaba , Pablo Navarro , Felipe J. Blas , José Palomar

We theoretically investigate the three-dimensional (3D) electron dynamics of graphene in real space under strong laser fields using time-dependent density functional theory (TDDFT). We successfully reproduce the reversal of current…

Mesoscale and Nanoscale Physics · Physics 2026-02-11 S. Li , M. Tani , A. Hashmi , K. L. Ishikawa

Diffraction patterns produced by grazing scattering of fast atoms from insulator surfaces are used to examine the atom-surface interaction. The method is applied to He atoms colliding with a LiF(001) surface along axial crystallographic…

Other Condensed Matter · Physics 2009-10-07 A. Schuller , H. Winter , M. S. Gravielle , J. M. Pruneda , J. E. Miraglia

Graphene, the one-atom-thick sp2 hybridized carbon crystal, displays unique electronic, structural and mechanical properties, which promise a large number of interesting applications in diverse high tech fields. Many of these applications…

Mesoscale and Nanoscale Physics · Physics 2016-09-27 Tommaso Cavallucci , Khatuna Kakhiani , Riccardo Farchioni , Valentina Tozzini

The wettability of monolayer and multilayer graphene remains a topic of longstanding debate. Here, we combined first-principles molecular dynamics simulations accelerated with the atomic cluster expansion machine learning interatomic…

Chemical Physics · Physics 2026-04-15 Dianwei Hou , Yevhen Horbatenko , Stefan Ringe , Minhaeng Cho