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The optical spectra of CdSe nanocrystals up to 55 A in diameter are analyzed in a wide range of energies from the fine structure of the low-energy excitations to the so-called high-energy transitions. We apply a symmetry-based method in two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Perez-Conde , A. K. Bhattacharjee

Exciton luminescence of a CdSe quantum dot (QD) inserted in a ZnSe nanowire is strongly influenced by the dark exciton states. Because of the small size of these QDs (2-5nm), exchange interaction between hole and electron is highly enhanced…

The influence of ligands on the low frequency vibration of different thicknesses cadmium selenide colloidal nanoplatelets is investigated using resonant low frequency Raman scattering. The strong vibration frequency shifts induced by ligand…

We demonstrate high quantum yield broad photoluminescence emission of ultrathin sub-nanometer CdSe nanoplatelets (two-monolayer). They also exhibit polarization-characterized lateral size dependent anomalous heavy hole and light/split-off…

Colloidal semiconductor nanoplatelets (NPLs) with electronic structure as quantum wells have recently emerged as exciting materials for optoelectronic applications. Here we investigate how morphology affects important photoluminescence (PL)…

Mesoscale and Nanoscale Physics · Physics 2018-03-23 Zhongjian Hu , Ajay Singh , Serguei V. Goupalov , Jennifer A. Hollingsworth , Han Htoon

Quantum Stark effect in semiconductor nanocrystals is theoretically investigated, using the effective mass formalism within a $4\times 4$ Baldereschi-Lipari Hamiltonian model for the hole states. General expressions are reported for the…

Materials Science · Physics 2009-11-10 Eduardo Ariel Menendez Proupin , Carlos Trallero Giner

We measured the intrinsic ground-state exciton dephasing and population dynamics in colloidal quasi two-dimensional (2D) CdSe nanoplatelets at low temperature (5-50K) using transient resonant four-wave mixing in heterodyne detection. Our…

Mesoscale and Nanoscale Physics · Physics 2015-05-05 Ali Naeem , Francesco Masia , Sotirios Christodoulou , Iwan Moreels , Paola Borri , Wolfgang Langbein

We experimentally investigated for the first time the lowest four band structure of Cd Se nanoplatelets at the r point of Brillouin zone [heavy-hole (hh), light-hole (lh) and two spin-orbital bands] and its modification due to the changing…

We compute exciton binding energies and fine-structure splittings in CdSe nanoplatelets with two zincblende geometries and one wurtzite geometry, finding that the wurtzite structure exhibits the largest bright-bright splitting due to its…

Materials Science · Physics 2026-02-11 Sumanti Patra , Gabriel Bester

This paper reports how CdSe core-only nanoplatelets coupled with plasmonic Al nanoparticle lattices can exhibit exciton-polariton lasing. By improving a procedure to synthesize monodisperse 4-monolayer CdSe nanoplatelets, we could resolve…

Although both epitaxial quantum dots (QDs) and colloidal nanocrystals (NCs) are quantum-confined semiconductor nanostructures, so far they have demonstrated dramatically-different exciton fine structure splittings (FSSs) at the cryogenic…

Mesoscale and Nanoscale Physics · Physics 2017-07-19 Chunyang Yin , Liyang Chen , Yan Lv , Fengrui Hu , Chun Sun , William W. Yu , Chunfeng Zhang , Xiaoyong Wang , Yu Zhang , Min Xiao

We discuss photo-luminescence characteristics of CdSe core/shell quantum dots at cryogenic temperatures using a hybrid system of a single quantum dot and an optical nanofiber. The key point is to control the emission species of quantum dot…

Mesoscale and Nanoscale Physics · Physics 2022-06-27 K. Muhammed Shafi , Kazunori Iida , Emi Tsutsumi , Akiharu Miyanaga , Kohzo Hakuta

Excitons, Coulomb-bound electron and hole pairs, are elementary photo-excitations in semiconductors, that can couple directly to light through radiative relaxation. In contrast to these bright excitons, dark excitons X$\rm{_D}$ with…

Materials Science · Physics 2018-02-14 Kyoung-Duck Park , Tao Jiang , Genevieve Clark , Xiaodong Xu , Markus B. Raschke

The quasiparticle band structure and optical properties of single-walled zigzag and armchair SiC nanotubes (SiC-NTs) as well as single SiC sheet are investigated by ab initio many-body calculations using the GW and the GW plus…

Mesoscale and Nanoscale Physics · Physics 2011-08-23 H. C. Hsueh , G. Y. Guo , Steven G. Louie

We report a combined experimental and computational study of the optical properties of individual silicon telluride (Si2Te3) nanoplates. The p-type semiconductor Si2Te3 has a unique layered crystal structure with hexagonal closed-packed Te…

Materials Science · Physics 2020-06-23 Jiyang Chen , Romakanta Bhattarai , Jingbiao Cui , Xiao Shen , Thang Hoang

Two-dimensional excitons formed in quantum materials such as monolayer transition-metal dichalcogenides and their strong light-matter interaction have attracted unrivalled attention by the research community due to their extraordinarily…

Mesoscale and Nanoscale Physics · Physics 2018-12-31 Lorenz Maximilian Schneider , Shanece Esdaille , Daniel Rhodes , Katayun Barmak , James Hone , Arash Rahimi-Iman

Engineering semiconductors to enhance carrier multiplication (CM) could lead to increased photovoltaic cell performance and a significant widening of the materials range suitable for future solar technologies. Semiconductor nanocrystals…

Mesoscale and Nanoscale Physics · Physics 2007-08-30 Gautham Nair , Moungi G Bawendi

Studies of photoluminescence (PL) can provide fundamental insight into the optical properties of semiconductor nanoparticles (NPs) but the same is being limited by NP size distribution and low luminescence yield. Inorganic semiconductor…

Materials Science · Physics 2010-05-04 A. M. P. Hussain , S. N. Sarangi , S. N. Sahu

We report excited state emission from p-states at excitation fluences well below ground state saturation in CdSe nanoplatelets. Size dependent exciton ground state-excited state energies and dynamics are determined by three independent…

Semiconductor nanoplatelets present reduced Auger recombination, giving rise to enhanced multiexciton emission. This virtue makes them good candidates to investigate higher-order carrier dynamics, allowing to extract important excitonic…

Mesoscale and Nanoscale Physics · Physics 2025-08-26 Daniel Amgar , Nadav Frenkel , Dekel Nakar , Dan Oron