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Related papers: Spin-wave gap collapse in Rh-doped Sr2IrO4

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The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

The simultaneous presence of sizable spin-orbit interactions and electron correlations in iridium oxides has led to predictions of novel ground states including Dirac semimetals, Kitaev spin liquids, and superconductivity. Electron and hole…

Strongly Correlated Electrons · Physics 2017-02-22 S. Chikara , G. Fabbris , J. Terzic , G. Cao , D. Khomskii , D. Haskel

The dispersive magnetic excitations in Sr2IrO4 have previously been well described within an isospin-1/2 Heisenberg model on a square lattice that revealed parallels with La2CuO4. Here we investigate the inelastic spectra of Sr2Ir0.8Ru0.2O4…

Strongly Correlated Electrons · Physics 2017-01-04 S. Calder , J. W. Kim , A. E. Taylor , M. H. Upton , D. Casa , Guixin Cao , M. D. Lumsden , A. D. Christianson

We have used a combination of resonant magnetic x-ray scattering (RMXS) and x-ray absorption spectroscopy (XAS) to investigate the properties of the doped spin-orbital Mott insulator Sr2Ir(1-x)Rh(x)O4 (0.07 < x < 0.70). We show that…

Strongly Correlated Electrons · Physics 2014-02-12 J. P. Clancy , A. Lupascu , H. Gretarsson , Z. Islam , Y. F. Hu , D. Casa , C. S. Nelson , S. C. Lamarra , G. Cao , Young-June Kim

Sr$_2$IrO$_4$ is the archetype of the spin-orbit Mott insulator, but the nature of the metallic states that may emerge from this type of insulator is still not very well known. We study with angle-resolved photoemission the…

Strongly Correlated Electrons · Physics 2018-04-30 Alex Louat , Fabrice Bert , Lise Serrier-Garcia , François Bertran , Patrick Le Fèvre , Julien Rault , Véronique Brouet

The electron-doping-driven collapse of the charge gap and staggered magnetization of the spin-orbit-assisted Mott insulator Sr$_{3}$Ir$_{2}$O$_{7}$ is explored via first-principles computational methods. In the antiferromagnetic phase, the…

Strongly Correlated Electrons · Physics 2018-08-15 Michael W. Swift , Zach Porter , Stephen D. Wilson , Chris G. Van de Walle

We have investigated the electronic structure of Sr2IrO4 within the density-functional theory using the generalized gradient approximation while taking into account strong Coulomb correlations in the framework of the fully relativistic…

Strongly Correlated Electrons · Physics 2023-10-13 V. N. Antonov , D. A. Kukusta , L. V. Bekenov

Materials that exhibit both strong spin orbit coupling and electron correlation effects are predicted to host numerous new electronic states. One prominent example is the Jeff =1/2 Mott state in Sr2IrO4, where introducing carriers is…

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

Strongly Correlated Electrons · Physics 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson

We study the effects of dilute La and Rh doping on the electronic structure of the relativistic Mott insulator Sr$_2$IrO$_4$ using fully relativistic and magnetically non-collinear density functional theory with the inclusion of an on-site…

Strongly Correlated Electrons · Physics 2016-12-07 Peitao Liu , Michele Reticcioli , Bongjae Kim , Alessandra Continenza , Georg Kresse , D. D. Sarma , Xing-Qiu Chen , Cesare Franchini

We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin flop transition from…

One way to induce insulator to metal transitions in the spin-orbit Mott insulator Sr2IrO4 is to substitute iridium with transition metals (Ru, Rh). However, this creates intriguing inhomogeneous metallic states, which cannot be described by…

Strongly Correlated Electrons · Physics 2021-09-08 Véronique Brouet , Paul Foulquier , Alex Louat , François Bertran , Patrick Le Fèvre , Julien E. Rault , Dorothée Colson

The physics of doped Mott insulators remains controversial after decades of active research, hindered by the interplay among possible competing orders and fluctuations. It is thus highly desired to distinguish the intrinsic characters of…

Transformation of Coulomb interaction terms to the pseudo-orbital basis constituted by $J=1/2$ and $3/2$ states arising from spin-orbit coupling provides a versatile tool. This formalism is applied to investigate magnetic anisotropy effects…

Strongly Correlated Electrons · Physics 2019-03-11 Shubhajyoti Mohapatra , Avinash Singh

Electronic excitations near the Fermi energy in the hole doped manganese oxides (La1-xSrxMnO3, x=0.2 and 0.4) have been elucidated by using the resonant inelastic x-ray scattering (RIXS) method. A doping effect in the strongly correlated…

Strongly Correlated Electrons · Physics 2007-05-23 K. Ishii , T. Inami , K. Ohwada , K. Kuzushita , J. Mizuki , Y. Murakami , S. Ishihara , Y. Endoh , S. Maekawa , K. Hirota , Y. Moritomo

We performed resonant x-ray diffraction experiments at the $L$ absorption edges for the post-perovskite-type compound CaIrO$_{3}$ with $(t_{2g})^5$ electronic configuration. By observing the magnetic signals, we could clearly see that the…

Dynamical correlations of Jeff = 1/2 isospins in the paramagnetic state of spin-orbital Mott insu- lator Sr2IrO4 was revealed by resonant magnetic x-ray diffuse scattering. We found two-dimensional antiferromagnetic fluctuation with a large…

Strongly Correlated Electrons · Physics 2015-06-04 S. Fujiyama , H. Ohsumi , T. Komesu , J. Matsuno , B. J. Kim , M. Takata , T. Arima , H. Takagi

We report high-resolution resonant inelastic x-ray scattering (RIXS) measurements of the collective spin fluctuations in three compositions of the superconducting cuprate system La2-xSrxCuO4. We have mapped out the excitations throughout…

Superconductivity · Physics 2020-02-14 H. C. Robarts , M. Barthelemy , M. Garcia-Fernandez , J. Li , A. Nag , A. C. Walters , K. J. Zhou , S. M. Hayden

In Sr2IrO4 and Sr3Ir2O7, correlations, magnetism and spin-orbit coupling compete on similar energy scales, creating a new context to study metal-insulator transitions (MIT). We use here Angle-Resolved photoemission to investigate the MIT as…

Strongly Correlated Electrons · Physics 2018-12-13 V. Brouet , L. Serrier-Garcia , A. Louat , L. Fruchter , F. Bertran , P. Le Fevre , J. Rault , A Forget , D. Colson

Momentum resolved inelastic resonant x-ray scattering is used to map the evolution of charge excitations over a large range of energies, momenta and doping levels in the electron doped Mott insulator class Nd$_{2-x}$Ce$_x$CuO$_4$. As the…

Strongly Correlated Electrons · Physics 2008-12-11 Y. W. Li , D. Qian , L. Wray , D. Hsieh , Y. Kaga , T. Sasagawa , H. Takagi , R. S. Markiewicz , A. Bansil , H. Eisaki , S. Uchida , M. Z. Hasan
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