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The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

Developing effective methods to measure the enantiomeric excess of the chiral mixture is one of the major topics in chiral molecular researches, yet remains challenging. Enantiodetection method via two-dimensional (2D) spectroscopy based on…

Chemical Physics · Physics 2023-05-05 Mao-Rui Cai , Chong Ye , Yong Li , Hui Dong

We theoretically introduce a scheme to perform Ramsey spectroscopy on a racemic mixture of chiral molecules, simultaneously extracting the transition frequencies of the left- and right-handed molecules, known as enantiomers. By taking the…

Atomic Physics · Physics 2023-11-07 Itay Erez , Eliana Ruth Wallach , Yuval Shagam

We consider a single electron traveling along a strictly one-dimensional quantum wire interacting with another electron in a quantum ring capacitively coupled to the wire. We develop an exact numerical method for treating the scattering…

Mesoscale and Nanoscale Physics · Physics 2016-11-25 M. R. Poniedziałek , B. Szafran

We present a state-space-based path integral method to calculate the rate of electron transfer (ET) in multi-state, multi-electron condensed-phase processes. We employ an exact path integral in discrete electronic states and continuous…

Chemical Physics · Physics 2016-06-07 Jessica Ryan Duke , Nandini Ananth

Coherent control of interfering one- and two-photon processes has for decades been the subject of research to achieve the redirection of photocurrent. The present study develops two-pathway coherent control of ground state helium atom…

Atomic Physics · Physics 2021-06-02 Yimeng Wang , Chris H. Greene

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

We show how to create maximal entanglement between spectrally distinct solid-state emitters embedded in a waveguide interferometer. By revealing the rich underlying structure of multi-photon scattering in emitters, we show that a two-photon…

Quantum Physics · Physics 2019-07-17 David L. Hurst , Kristoffer B. Joanesarson , Jake Iles-Smith , Jesper Mørk , Pieter Kok

Microwave three-wave mixing allows for enantiomer-selective excitation of randomly oriented chiral molecules into rotational states with different energy. The random orientation of molecules is reflected in the degeneracy of the rotational…

Quantum Physics · Physics 2022-08-02 Monika Leibscher , Jonas Kalveram , Christiane P. Koch

Enantio-conversion of chiral mixtures, converting the mixtures composed of left- and right-handed chiral molecules into the homochiral ensembles, has become an important research topic in chemical and biological fields. In previous studies…

Quantum Physics · Physics 2023-12-18 Fen Zou , Chong Ye , Yong Li

We present an optical "enantio-selective switch", that, in two steps, turns a ("racemic") mixture of left-handed and right-handed chiral molecules into the enantiomerically pure state of interest. The optical switch is composed of an…

Quantum Physics · Physics 2009-11-07 Petr Král , Ioannis Thanopulos , Moshe Shapiro , Doron Cohen

We propose a scheme for both distilling and quantifying entanglement, applicable to individual copies of an arbitrary unknown two-qubit state. It is realized in a usual two-qubit interferometry with local filtering. Proper filtering…

Quantum Physics · Physics 2010-06-09 S. -S. B. Lee , H. -S. Sim

The purpose of this paper is to study the interaction between a two-level system and two continuous-mode photons. Two scenarios are investigated: Case 1, how a two-level system changes the pulse shapes of two input photons propagating in a…

Quantum Physics · Physics 2019-10-14 Zhiyuan Dong , Guofeng Zhang , Nina H. Amini

Hydrogen-release by photoexcitation, excited-state- hydrogen-transfer (ESHT), is one of the important photo- chemical processes that occur in aromatic acids and is responsible for photoprotection of biomolecules. The mecha- nism is…

The reliable distribution of high-dimensional entangled quantum states, an important resource in quantum technologies, through optical fibre networks is challenging due to the need to maintain coherence across multiple modes. Here we…

We present an entanglement swapping process for unknown nonmaximally entangled photonic states, where the standard Bell-state measurement is replaced by a three-step quantum walk-like state discrimination process, i.e., the practically…

Quantum Physics · Physics 2017-11-22 Xiao-Man Li , Ming Yang , Nikola Paunkovic , Da-Chuang Li , Zhuo-Liang Cao

Single-loop cyclic three-level ($\Delta$-type) configuration of chiral molecules was used for enantio-separation in many theoretical works. Considering the effect of molecular rotation, this simple single-loop configuration is generally…

Quantum Physics · Physics 2018-12-12 Chong Ye , Quansheng Zhang , Yong Li

Enantioselective photochemistry provides access to unique molecular structures and functions, with deep implications for fundamental science and industrial applications. Current methods for highly enantioselective photochemistry critically…

Chemical Physics · Physics 2025-03-07 Andrés Ordóñez , Patricia Vindel-Zandbergen , David Ayuso

We study the protocol known as quantum state transfer for a strongly coupled antiferromagnetic spin chain or ring (acting as a spin bus), with weakly coupled external qubits. By treating the weak coupling as a perturbation, we find that…

Quantum Physics · Physics 2013-04-25 Sangchul Oh , Lian-Ao Wu , Yun-Pil Shim , Mark Friesen , Xuedong Hu

Dynamically varying system parameters along a path enclosing an exceptional point is known to lead to chiral mode conversion. But is it necessary to include this non-Hermitian degeneracy inside the contour for this process to take place? We…