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Related papers: Adsorption of H$_2$ on Amorphous Solid Water Studi…

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Accurate modeling of physical and chemical processes in the interstellar medium requires detailed knowledge of how atoms and molecule adsorb on dust grains. However, the sticking coefficient, a number between 0 and 1 that measures the first…

Instrumentation and Methods for Astrophysics · Physics 2016-06-01 Jiao He , Kinsuk Acharyya , Gianfranco Vidali

Gas-grain and gas-phase reactions dominate the formation of molecules in the interstellar medium (ISM). Gas-grain reactions require a substrate (e.g. a dust or ice grain) on which the reaction is able to occur. The formation of molecular…

Astrophysics of Galaxies · Physics 2016-11-09 John L. Dupuy , Steven P. Lewis , P. C. Stancil

Nonthermal desorption of molecules from icy grain surfaces is required to explain molecular line observations in the cold gas of star-forming regions. Chemical desorption is one of the nonthermal desorption processes and is driven by the…

Astrophysics of Galaxies · Physics 2022-03-02 Kenji Furuya , Yasuhiro Oba , Takashi Shimonishi

We present a computational study into the adsorption properties of CO$_2$ on amorphous and crystalline water surfaces under astrophysically relevant conditions. Water and carbon dioxide are two of the most dominant species in the icy…

Astrophysics of Galaxies · Physics 2017-09-13 L. J. Karssemeijer , G. A. de Wijs , H. M. Cuppen

Dynamics of adsorption and desorption of (4S)-N on amorphous solid water are analyzed using molecular dynamics simulations. The underlying potential energy surface was provided by machine-learned interatomic potentials. Binding energies…

Astrophysics of Galaxies · Physics 2020-09-22 Germán Molpeceres , Viktor Zaverkin , Johannes Kästner

Using the King & Wells method, we present experimental data on the dependence of the sticking of molecular hydrogen and deuterium on the beam temperature onto non- porous amorphous solid water (ASW) ice surfaces of interstellar interest. A…

Chemical Physics · Physics 2015-05-19 E. Matar , H. Bergeron , F. Dulieu , H. Chaabouni , M. Accolla , J. L. Lemaire

Interstellar ices are mainly composed of amorphous solid water (ASW) containing small amounts of hypervolatiles, such as O2, whose diffusion-limited reactions play a key role in space chemistry. Although O2 is an important precursor…

Astrophysics of Galaxies · Physics 2026-03-13 Lina Coulaud , Julia C. Santos , Ko-Ju Chuang

In the quest to understand the formation of the building blocks of life, amorphous solid water (ASW) is one of the most widely studied molecular systems. Indeed, ASW is ubiquitous in the cold interstellar medium (ISM), where ASW-coated dust…

Chemical Physics · Physics 2014-02-17 Jennifer A Noble , Céline Martin , Helen J. Fraser , Pascale Roubin , Stéphane Coussan

Water (H2O) ice is an important solid constituent of many astrophysical environments. To comprehend the role of such ices in the chemistry and evolution of dense molecular clouds and comets, it is necessary to understand the freeze-out,…

The ultraviolet (UV) photodissociation of amorphous water ice at different ice temperatures is investigated using molecular dynamics (MD) simulations and analytical potentials. Previous MD calculations of UV photodissociation of amorphous…

Chemical Physics · Physics 2010-05-21 C. Arasa , S. Andersson , H. M. Cuppen , E. F. van Dishoweck , G. -J. Kroes

Absorption of ultraviolet radiation by water ice coating interstellar grains can lead to dissociation and desorption of the ice molecules. These processes are thought to be important in the gas-grain chemistry in molecular clouds and…

Astrophysics · Physics 2009-11-13 S. Andersson , E. F. van Dishoeck

We present results of classical dynamics calculations, performed to study the photodissociation of water in crystalline and amorphous ice surfaces at a surface temperature of 10 K. Dissociation in the top six monolayers is considered.…

Astrophysics · Physics 2009-11-11 Stefan Andersson , Ayman Al-Halabi , Geert-Jan Kroes , Ewine F. van Dishoeck

The diffusion of atoms and molecules in ices covering dust grains in dense clouds in interstellar space is an important but poorly characterized step in the formation of complex molecules in space. Here we report the measurement of…

Instrumentation and Methods for Astrophysics · Physics 2018-08-29 Jiao He , SM Emtiaz , Gianfranco Vidali

The knowledge of the binding energy of molecules on astrophysically relevant ices can help to obtain an estimate of the desorption rate, i.e. the molecules residence time on the surface. This represents an important parameter for…

Aims. Interstellar dust grains, because of their catalytic properties, are crucial to the formation of H2, the most abundant molecule in the Universe. The formation of molecular hydrogen strongly depends on the ability of H atoms to stick…

Solar and Stellar Astrophysics · Physics 2015-05-28 S. Cazaux , S. Morisset , M. Spaans , A. Allouche

Sticking of H and D atoms on interstellar dust grains is the first step in molecular hydrogen formation, which is a key reaction in the InterStellar Medium (ISM). After studying the sticking coefficients of H2 and D2 molecules on amorphous…

Instrumentation and Methods for Astrophysics · Physics 2012-02-14 H. Chaabouni , H. Bergeron , S. Baouche , F. Dulieu , E. Matar , E. Congiu , L. Gavilan , J. L. Lemaire

Abundances and partitioning of ices and gases produced by gas-grain chemistry are governed by adsorption and desorption on grains. Understanding astrophysical observations rely on laboratory measurements of adsorption and desorption rates…

Astrophysics of Galaxies · Physics 2021-02-22 Carine Laffon , Daniel Ferry , Olivier Grauby , Philippe Parent

The morphology of water ice in the interstellar medium is still an open question. Although accretion of gaseous water could not be the only possible origin of the observed icy mantles covering dust grains in cold molecular clouds, it is…

Solid O2 has been proposed as a possible reservoir for oxygen in dense clouds through freeze-out processes. The aim of this work is to characterize quantitatively the physical processes that are involved in the desorption kinetics of CO-O2…

Astrophysics · Physics 2009-11-13 K. Acharyya , G. W. Fuchs , H. J. Fraser , E. F. van Dishoeck , H. Linnartz

The abundance of interstellar ice constituents is usually expressed with respect to the water ice because, in denser regions, a significant portion of the interstellar grain surface would be covered by water ice. The binding energy (BE), or…

Astrophysics of Galaxies · Physics 2021-06-01 Ankan Das , Milan Sil , Rana Ghosh , Prasanta Gorai , Soutan Adak , Subhankar Samanta , Sandip K. Chakrabarti
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