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Lead-halide perovskite nanocrystals such as CsPbBr$_3$, exhibit efficient photoluminescence (PL) up-conversion, also referred to as anti-Stokes photoluminescence (ASPL). This is a phenomenon where irradiating nanocrystals up to 100 meV…

Mesoscale and Nanoscale Physics · Physics 2024-02-29 Zhuoming Zhang , Sushrut Ghonge , Yang Ding , Shubin Zhang , Mona Berciu , Richard D. Schaller , Boldizsár Jankó , Masaru Kuno

Heating of charged particles via collisionless shocks, while ubiquitous in the universe, is an intriguing yet puzzling plasma phenomenon. One outstanding question is how electrons and ions approach an equilibrium after they were heated to…

High Energy Astrophysical Phenomena · Physics 2024-05-16 Masahiro Ichihashi , Aya Bamba , Yuichi Kato , Satoru Katsuda , Hiromasa Suzuki , Tomoaki Kasuga , Hirokazu Odaka , Kazuhiro Nakazawa

Plasmonic nanoapertures generate strong field gradients enabling efficient optical trapping of nano-objects. However, because the infrared laser used for trapping is also partly absorbed into the metal leading to Joule heating, plasmonic…

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

We report on time-resolved measurements of electron number density by continuous-wave laser absorption in a low-energy nanosecond-scale laser-produced spark in atmospheric pressure air. Laser absorption is a result of free-free and…

Plasma Physics · Physics 2021-05-19 T. Yong , A. I. Abdalla , M. A. Cappelli

We report the studies of ultrafast electron nanocrystallography on size-selected Au nanoparticles (2-20 nm) supported on a molecular interface. Reversible surface melting, melting, and recrystallization were investigated with dynamical…

Materials Science · Physics 2015-05-13 Chong-Yu Ruan , Yoshie Murooka , Ramani K. Raman , Ryan A. Murdick

The temperature of a nonneutral plasma confined in a Penning-Malmberg trap can be determined by slowly lowering one side of the trap's electrostatic axial confinement barrier; the temperature is inferred from the rate at which particles…

Instrumentation and Detectors · Physics 2020-10-26 E. D. Hunter , J. Fajans , N. A. Lewis , A. P. Povilus , C. Sierra , C. So , D. Zimmer

The study of parametric instabilities has played a crucial role in understanding energy transfer to plasma and, with that, the development of key applications such as inertial confinement fusion. When the densities are between…

Above-threshold light emission from plasmonic tunnel junctions, when emitted photons have energies significantly higher than the energy scale of the incident electrons, has attracted much recent interest in nano-optics, while the underlying…

Mesoscale and Nanoscale Physics · Physics 2020-12-08 Longji Cui , Yunxuan Zhu , Mahdiyeh Abbasi , Arash Ahmadivand , Burak Gerislioglu , Peter Nordlander , Douglas Natelson

One of the goals of pump/probe spectroscopies is to determine how electrons relax after they have been driven out of equilibrium. It is challenging to determine how close electrons are to a thermal state solely by fitting their distribution…

Strongly Correlated Electrons · Physics 2019-06-26 O. P. Matveev , A. M. Shvaika , T. P. Devereaux , J. K. Freericks

Spintronic terahertz emitters (STEs) pumped by femtosecond lasers have become a widely used source of broadband terahertz radiation. However, the strength of the emitted field is limited in part by the optical damage threshold at the pump…

Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…

Photoluminescence (PL) is a fundamental light-matter interaction, which conventionally involves the absorption of energetic photon, thermalization and the emission of a red-shifted photon. Conversely, in optical-refrigeration the absorption…

Optics · Physics 2014-12-23 Assaf Manor , Leopoldo L. Martin , Carmel Rotschild

Warm-dense matter (WDM) is a highly-excited state that lies at the confluence of solids, plasmas, and liquids and that cannot be described by equilibrium theories. The transient nature of this state when created in a laboratory, as well as…

We demonstrate that in confined plasmonic metal structures subject to ultra-fast laser excitation electron thermal diffusion can provide relaxation faster than the energy transfer to the lattice. This relaxation occurs due to excitation of…

Direct measurements of photoexcited carrier dynamics in nickel are made using few-femtosecond extreme ultraviolet (XUV) transient absorption spectroscopy at the nickel M$_{2,3}$ edge. It is observed that the core-level absorption lineshape…

Controlling the temperature in architectures involving nanoparticles and substrates is a key issue for applications involving micro and nanoscale heat transfer. We study the thermal behavior of a single nanoparticle interacting with a flat…

Optics · Physics 2017-03-03 Houssem Kallel , Rémi Carminati , Karl Joulain

Recently [3] predicted the existence of an intriguing new phenomenon. It was shown that if temperature is suddenly raised at the surface of a sphere the temperature in the interior initially decreases. The authors of [3] gave a thorough…

Soft Condensed Matter · Physics 2011-05-11 J. J. Papini

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…