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Magnetic circular dichroism (MCD) is a widely used spectroscopic technique which reveals valuable information about molecular geometry and electronic structure. However, the weak signal and the necessary strong magnets impose major…

Chemical Physics · Physics 2022-11-16 Jiaan Cao , Lyuzhou Ye , Dawei He , Xiao Zheng , Shaul Mukamel

In this manuscript, we outline a reliable procedure to manufacture photonic nanostructures from single-crystal diamond (SCD). Photonic nanostructures, in our case SCD nanopillars on thin (< 1$\mu$m) platforms, are highly relevant for…

Materials Science · Physics 2019-10-25 Mariusz Radtke , Richard Nelz , Abdallah Slablab , Elke Neu

Progress in electron-beam spectroscopies has recently enabled the study of optical excitations with combined space, energy and time resolution in the nanometer, millielectronvolt and femtosecond domain, thus providing unique access into…

Optics · Physics 2019-11-13 Albert Polman , Mathieu Kociak , F. Javier García de Abajo

Light-sheet microscopes must compromise between field of view, optical sectioning, resolution, and detection efficiency. High-numerical-aperture (NA) detection objective lenses provide high resolution but their narrow depth of field fails…

Energy-loss magnetic chiral dichroism (EMCD) is a versatile method for studying magnetic properties on the nanoscale. However, the classical EMCD technique is notorious for its low signal to noise ratio (SNR). Here, we study the theoretical…

Instrumentation and Detectors · Physics 2019-03-12 Stefan Löffler , Walid Hetaba

We report on strong field ionization of S- and R-propylene oxide in circularly polarized two-color laser fields. We find that the relative helicity of the two single color laser fields affects the photoelectron circular dichroism (PECD).…

Recent progress in the application of color centers to nanoscale spin sensing makes the combined use of noise spectroscopy and scanning probe imaging an attractive route for the characterization of arbitrary material systems. Unfortunately,…

Prospects of using metal hole arrays for the enhanced optical detection of molecular chirality in nanosize volumes are investigated. Light transmission through the holes filled with an optically active material is modeled and the activity…

Optical dielectric resonances have the ability to modulate optical energy, and by coupling multiple resonators into photonic molecules, new opportunities emerge in spectral engineering. Using electron-beam spectroscopy, in a 300-keV…

Optics · Physics 2021-10-07 Martin Couillard

The detection of individual photons is an inherently binary mechanism, revealing either their absence or presence while concealing their spectral information. For multi-color imaging techniques, such as single photon spectroscopy,…

Instrumentation and Detectors · Physics 2016-09-27 O. Kahl , S. Ferrari , V. Kovalyuk , A. Vetter , G. Lewes-Malandrakis , C. Nebel , A. Korneev , G. Goltsman , W. Pernice

Photoelectron circular dichroism (PECD) is a method where randomly oriented chiral molecules are photoionized due to irradiation by circularly-polarized lasers, yielding large chiral signals in the photoelectron momentum distribution.…

Optics · Physics 2025-12-16 Gal Bouskila , Avner Fleischer , Ofer Neufeld

Si$_3$N$_4$ waveguides, pumped at 1550 nm, can provide spectrally smooth, broadband light for gas spectroscopy in the important 2 ${\mathrm{\mu}}$m to 2.5 ${\mathrm{\mu}}$m atmospheric water window, which is only partially accessible with…

Extreme field localization and giant field enhancement are often achieved by using plasmonic nanostructures and metamaterials such as strongly coupled silver nanoparticles.Dielectric particles and structures can focus light beyond the…

We present the first photoelectron circular dichroism (PECD) measurements of chiral alcohols, and in particular 1-Phenylethanol, using multiphoton ionization at 400 nm. Observed PECD values were rather small at $\sim2$%, but could be…

Optical chirality (OC) is a fundamental property of electromagnetic waves that plays a key role in governing chiral light-matter interaction. Here, we demonstrate how to obtain superchiral surface lattice resonances (SLRs), which arise from…

Optics · Physics 2022-03-23 Joshua T. Y. Tse , H. C. Ong

High-numerical-aperture (NA) oblique plane microscopy enables noninvasive fluorescence imaging of subcellular dynamics without requiring radical sample modification. However, performance degrades at depth in multicellular specimens as…

Cavity ring-down spectroscopy is a ubiquitous optical method used to study light-matter interactions with high resolution, sensitivity and accuracy. However, it has never been performed with the multiplexing advantages of direct frequency…

Open subwavelength cylindrical resonators of finite height are widely used in various photonics applications. Circular cylindrical resonators are particularly important in nanophotonics, since they are relatively easy to fabricate and can…

Optics · Physics 2019-07-24 Hualiang Shi , Ya Yan Lu

Chirality is an intriguing property of certain molecules, materials or artificial nanostructures, which allows them to interact with the spin angular momentum of the impinging light field. Due to their chiral geometry, they can distinguish…

Optics · Physics 2016-11-03 Peter Banzer , Pawel Wozniak , Uwe Mick , Israel De Leon , Robert W. Boyd

Controlling scattering and routing of chiral light at the nanoscale is important for optical information processing and imaging, quantum technologies as well as optical manipulation. Here, we introduce a concept of rotating chiral dipoles…

Optics · Physics 2025-09-25 Yuanyang Xie , Alexey V. Krasavin , Diane J. Roth , Anatoly V. Zayats
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