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We investigate the chemical reactivity of molecular populations confined inside a nanofluidic Fabry-P{\'e}rot cavity. Due to strong light-matter interactions developing between a resonant electromagnetic cavity-mode and the electric dipole…

Mesoscale and Nanoscale Physics · Physics 2021-04-21 L Mauro , K Caicedo , G Jonusauskas , Rémi Avriller

Experimental studies indicate that optical cavities can affect chemical reactions, through either vibrational or electronic strong coupling and the quantized cavity modes. However, the current understanding of the interplay between…

We experimentally and theoretically study collective emission of a dense atomic ensemble coupled to a single mode in a nanophotonic microring resonator. Because many cold atoms are localized in a small volume, these trapped atoms…

Quantum Physics · Physics 2025-09-12 Xinchao Zhou , Deepak A. Suresh , F. Robicheaux , Chen-Lung Hung

We study strong light-mediated resonant dipole-dipole interactions in two-dimensional planar lattices of cold atoms. We provide a detailed analysis for the description of the dipolar point emitter lattice plane as a "super-atom", whose…

Atomic Physics · Physics 2018-02-26 G. Facchinetti , J. Ruostekoski

Nanocavities formed by ultrathin metallic gaps, such as the nanoparticle-on-mirror geometry, permit the reproducible engineering and enhancement of light-matter interaction thanks to mode volumes reaching the smallest values allowed by…

Recent experiments of chemical reactions in optical cavities have shown great promise to alter and steer chemical reactions but still remain poorly understood theoretically. In particular the origin of resonant effects between the cavity…

Chemical Physics · Physics 2022-12-21 Derek S. Wang , Johannes Flick , Susanne F. Yelin

The coupling of individual atoms to a high-finesse optical cavity is precisely controlled and adjusted using a standing-wave dipole-force trap, a challenge for strong atom-cavity coupling. Ultracold Rubidium atoms are first loaded into…

Quantum Physics · Physics 2015-06-26 Stefan Nussmann , Markus Hijlkema , Bernhard Weber , Felix Rohde , Gerhard Rempe , Axel Kuhn

We consider a simple cubic array of metallic nanoparticles supporting extended collective plasmons that arise from the near-field dipolar interaction between localized surface plasmons in each nanoparticle. We develop a fully analytical…

Mesoscale and Nanoscale Physics · Physics 2015-01-12 Guillaume Weick , Eros Mariani

We investigate the radiative coupling between two two-level atoms with arbitrarily polarized dipoles in the vicinity of a nanofiber. We present a systematic derivation for the master equation, the single- and cross-atom decay coefficients,…

Quantum Physics · Physics 2016-12-15 Fam Le Kien , Arno Rauschenbeutel

Strong light-matter interactions facilitate not only emerging applications in quantum and non-linear optics but also modifications of materials properties. In particular the latter possibility has spurred the development of advanced…

Mesoscale and Nanoscale Physics · Physics 2021-08-17 Jakub Fojt , Tuomas P. Rossi , Tomasz J. Antosiewicz , Mikael Kuisma , Paul Erhart

The interaction between molecular (atomic) electron(s) and the vacuum field of a reflective cavity generates a significant interest thanks to the rapid developments in nanophotonics. Such interaction which lies within the realm of cavity…

Chemical Physics · Physics 2019-05-22 Alexander Semenov , Abraham Nitzan

We predict plasmonic mediated nucleation of pancake shaped resonant nano-cavities in metallic layers that are penetrable to laser fields. The underlying physics is that the cavity provides a narrow plasmonic resonance that maximizes its…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 V. G. Karpov , M. Nardone , A. V. Subashiev

The collective absorption and emission of light by an ensemble of atoms is at the heart of many fundamental quantum optical effects and the basis for numerous applications. However, beyond weak excitation, both experiment and theory become…

Nanoscale quantum dots in microwave cavities can be used as a laboratory for exploring electron-electron interactions and their spin in the presence of quantized light and a magnetic field. We show how a simple theoretical model of this…

Mesoscale and Nanoscale Physics · Physics 2023-11-16 S. S. Beltrán-Romero , F. J. Rodríguez , L. Quiroga , N. F. Johnson

We introduce a theory of chemical equilibrium in optical microcavities, which allows us to relate equilibrium reaction quotients in different electromagnetic environments. Our theory shows that in planar microcavities under strong coupling…

Chemical Physics · Physics 2023-05-02 Kaihong Sun , Raphael F. Ribeiro

Strong coupling of organic molecules to the vacuum field of a nanoscale cavity can be used to modify their chemical and physical properties. We extend the Tavis-Cummings model for molecular ensembles and show that the often neglected…

Chemical Physics · Physics 2024-08-01 Lucas Borges , Thomas Schnappinger , Markus Kowalewski

Strongly interacting atom-cavity systems within a network with many nodes constitute a possible realization for a quantum internet which allows for quantum communication and computation on the same platform. To implement such large-scale…

Atomic Physics · Physics 2016-11-23 Ralf Ritter , Nico Gruhler , Wolfram Pernice , Harald Kübler , Tilman Pfau , Robert Löw

Near-field and resonance effects have a strong influence on the nanoscale electromagnetic energy transfer, and detailed understanding of these effects is required for the design of new, optimized nano-optical devices. We provide a…

Mesoscale and Nanoscale Physics · Physics 2014-04-03 K. Sääskilahti , J. Oksanen , J. Tulkki

Atoms interact with each other through the electromagnetic field, creating collective states that can radiate faster or slower than a single atom, i.e. super- and sub-radiance. The generation and control of such states by engineering the…

Arrays of optically trapped nanoparticles have emerged as a promising platform for the study of complex non-equilibrium phenomena. Analogous to atomic many-body systems, one of the crucial ingredients is the ability to precisely control the…