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We investigate the influence of light-matter interactions on correlated quantum matter by studying the paradigmatic Ising model subject to a quantum Rabi coupling. This type of coupling to a confined, spatially delocalized bosonic light…

Strongly Correlated Electrons · Physics 2020-05-13 J. Rohn , M. Hörmann , Claudiu Genes , K. P. Schmidt

The propagation of light in strongly coupled atomic media takes place through the formation of polaritons - hybrid quasi-particles resulting from a superposition of an atomic and a photonic excitation. Here we consider the propagation under…

Quantum Gases · Physics 2020-09-30 Johannes Lang , Darrick E. Chang , Francesco Piazza

Recent experiments have demonstrated that molecular polaritons, hybrid states of light and matter formed by the strong coupling between molecular electronic or vibrational excitations and an optical cavity, can substantially modify the…

Chemical Physics · Physics 2021-07-08 Nguyen Thanh Phuc

The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…

We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

Mesoscale and Nanoscale Physics · Physics 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

The polariton, a quasiparticle formed by strong coupling of a photon to a matter excitation, is a fundamental ingredient of emergent photonic quantum systems ranging from semiconductor nanophotonics to circuit quantum electrodynamics.…

Quantum Gases · Physics 2024-03-21 Joonhyuk Kwon , Youngshin Kim , Alfonso Lanuza , Dominik Schneble

Light and matter can intertwine to create entirely new quantum states in the so-called strong-coupling regime, allowing unprecedented control over electromagnetic waves. In this work, strong-coupling mediated polaritonic states are…

We present a new methodology to calculate the strong light-matter coupling between photonic modes in microcavities and large molecular aggregates that consist of hundreds of molecular fragments. To this end, we combine our fragment…

Chemical Physics · Physics 2024-07-30 Richard Einsele , Luca Nils Philipp , Roland Mitrić

Bose condensed light can form new phases [1] in a dye filled cavity due to the presence of the orientational disorder created by dye molecules which are essentially frozen on the time scale of the photonic thermalization (few ps). At longer…

Quantum Gases · Physics 2020-05-06 Victor Fleurov , Anatoly B. Kuklov

This paper presents a nonperturbative treatment of strong-coupling induced effects in atom-field systems which cannot be seen in traditional perturbative treatments invoking compromising assumptions such as the Born-Markov, rotating wave or…

Quantum Physics · Physics 2020-02-25 Jen-Tsung Hsiang , Bei-Lok Hu

The interaction between light and matter can give rise to novel topological states. This principle was recently exemplified in Floquet topological insulators, where \emph{classical} light was used to induce a topological electronic band…

Quantum Gases · Physics 2015-07-08 Torsten Karzig , Charles-Edouard Bardyn , Netanel Lindner , Gil Refael

Light-matter systems allow to realize a strongly correlated phase where photons are present. In these systems strong correlations are achieved by optical nonlinearities, which appear due to the coupling of photons to atomic-like structures.…

Mesoscale and Nanoscale Physics · Physics 2011-06-10 Michael Knap , Enrico Arrigoni , Wolfgang von der Linden

Despite the potential paradigm breaking capability of microcavities to control chemical processes, the extent to which photonic devices change properties of molecular materials is still unclear, in part due to challenges in modeling hybrid…

Chemical Physics · Physics 2021-12-30 Raphael F. Ribeiro

Confined electromagnetic modes strongly couple to collective excitations in ensembles of quantum emitters, producing light-matter hybrid states known as polaritons. Under such conditions, the discrete multilevel spectrum of molecular…

Quantum Physics · Physics 2022-06-01 Jorge A. Campos-Gonzalez-Angulo , Joel Yuen-Zhou

The interaction of organic molecules and molecular aggregates with electromagnetic fields that are strongly confined inside optical cavities within nanoscale volumes, has allowed the observation of exotic quantum regimes of light-matter…

Quantum Physics · Physics 2018-01-30 Felipe Herrera , Frank C. Spano

We analyze the properties of strongly coupled excitons and photons in systems made of semiconducting two-dimensional transition-metal dichalcogenides embedded in optical cavities. Through a detailed microscopic analysis of the coupling we…

Mesoscale and Nanoscale Physics · Physics 2018-10-03 Á. Gutiérrez-Rubio , L. Chirolli , L. Martín-Moreno , F. J. García-Vidal , F. Guinea

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling,…

We observe natural exceptional points in the excitation spectrum of an exciton-polariton system by optically tuning the light-matter interactions. The observed exceptional points do not require any spatial or polarization degrees of freedom…

The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this…

We consider an ensemble of homonuclear diatomic molecules coupled to the two polarization directions of a Fabry-P\'erot cavity via fully quantum simulations. Accompanied by analytical results, we identify a coupling mechanism mediated…

Chemical Physics · Physics 2024-01-22 Niclas Krupp , Oriol Vendrell