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We investigate the chemical evolution of a collapsing core that starts from a hydrostatic core and finally form a low-mass protostar. New multiphase gas-grain models that include bulk diffusion and photon penetration are simulated by the…

Solar and Stellar Astrophysics · Physics 2018-12-27 Yang Lu , Qiang Chang , Yuri Aikawa

A widely accepted phenomenological rule states that solids with free surfaces cannot be overheated. In this work we discuss this statement critically under the light of the statistical thermodynamics of interfacial roughening transitions.…

Soft Condensed Matter · Physics 2025-01-08 Lukasz Baran , Pablo Llombart , Eva G. Noya , L. G. MacDowell

Understanding the nucleation and growth dynamics of the surface bubbles generated on a heated surface can benefit a wide range of modern technologies, such as the cooling systems of electronics, refrigeration cycles, nuclear reactors and…

Understanding the pathways to crystallization during the deposition of a vapor phase on a cold solid substrate is of great interest in industry, e.g., for the realization of electronic devices made of crystallites-free glassy materials, as…

Soft Condensed Matter · Physics 2023-10-03 Fabio Leoni , Hajime Tanaka , John Russo

Morphological changes in a dry phospholipid film on a solid substrate were studied below and above the main transition temperature, between the gel and liquid-crystalline phases by phase-contrast microscopy and AFM. A Phospholipid film in…

Chemical Physics · Physics 2015-06-26 Mafumi Hishida , Hideki Seto , Kenichi Yoshikawa

Icy pebbles may play an important role in planet formation close to the water ice line of protoplanetary discs. There, dust coagulation is more efficient and re-condensation of vapor on pebbles may enhance their growth outside the ice line.…

Earth and Planetary Astrophysics · Physics 2021-11-24 Stefano Spadaccia , Holly L. Capelo , Antoine Pommerol , Philipp Schuetz , Yann Alibert , Katrin Ros , Nicolas Thomas

The present study reports experiments of water droplet impacting on ice or on a cold metallic substrate, with the aim of understanding the effect of phase change on the impingement process. Both liquid and substrate temperatures are varied,…

In this work we measured Surface Energy and Freezing Temperature of supercooled water droplets in air. We find that freezing of water droplets is triggered at the water-air interface and that freezing progresses faster on the surface than…

A broad fundamental understanding of the mechanisms underlying the phenomenology of supercooled liquids has remained elusive, despite decades of intense exploration. When supercooled beneath its characteristic melting temperature, a liquid…

Soft Condensed Matter · Physics 2016-11-10 Nicholas B. Weingartner , Chris Pueblo , Flavio S. Nogueira , K. F. Kelton , Zohar Nussinov

When an ice crystal is born from liquid water two key changes occur: (i) the molecules order; and (ii) the mobility of the molecules drops as they adopt their lattice positions. Most research on ice nucleation (and crystallization in…

Chemical Physics · Physics 2019-03-27 Martin Fitzner , Gabriele C. Sosso , Stephen J. Cox , Angelos Michaelides

(Abridged) Aims & Methods. A two-dimensional, semi-analytical model is presented that follows, for the first time, the chemical evolution from a collapsing molecular cloud (a pre-stellar core) to a protostar and circumstellar disk. The…

Solar and Stellar Astrophysics · Physics 2009-11-13 R. Visser , E. F. van Dishoeck , S. D. Doty , C. P. Dullemond

The coalescence between growing droplets is important for the surface coverage and spatial arrangements of droplets on surfaces. In this work, total internal reflection fluorescence (TIRF) microscopy is utilized to in-situ investigate the…

Soft Condensed Matter · Physics 2018-04-06 Brendan Dyett , Hao Hao , Detlef Lohse , Xuehua Zhang

Hypothesis: As a fluid approaches three phase coexistence, adsorption may take place by the successive formation of two intervening wetting films. The equilibrium thickness of these wetting layers is the result of a delicate balance of…

Chemical Physics · Physics 2021-03-11 Juan Luengo-Márquez , Luis G. MacDowell

Iceberg melting is a critical factor for climate change, contributing to rising sea levels and climate change. However, the shape of an iceberg is an often neglected aspect of its melting process. Our study investigates the influence of…

Fluid Dynamics · Physics 2023-09-12 Rui Yang , Christopher J. Howland , Hao-Ran Liu , Roberto Verzicco , Detlef Lohse

Thin films are usually obtained by depositing atoms with a continuous flux. We show that using a chopped flux changes the growth and the morphology of the film. A simple scaling analysis predicts how the island densities change as a…

Materials Science · Physics 2016-08-16 Pablo Jensen , Bernd Niemeyer

We use molecular simulation to calculate the nucleation free energy barrier for the freezing of a 456 atom gold cluster over a range of temperatures. The results show that the embryo of the solid cluster grows at the vapor-surface interface…

Soft Condensed Matter · Physics 2007-05-23 Eduardo Mendez-Villuendas Richard K. Bowles

Context. The study of the snow line is an important topic in several domains of astrophysics, and particularly for the evolution of proto-stellar environments and the formation of planets. Aims. The formation of the first layer of ice on…

Earth and Planetary Astrophysics · Physics 2015-05-27 M. G. Marseille , S. Cazaux

We present measurements of the growth of long columnar ice crystals from water vapor over a broad range of temperatures and supersaturation levels in air. Starting with thin, c-axis ice needle crystals, we observed their subsequent growth…

Materials Science · Physics 2016-02-09 Kenneth G. Libbrecht

Drops impacting on a surface are ubiquitous in our everyday experience. This impact is understood within a commonly accepted hydrodynamic picture: it is initiated by a rapid shock and a subsequent ejection of a sheet leading to beautiful…

We describe observations of a novel hysteresis behavior in the growth of ice crystals under near-vacuum conditions. Above a threshold supersaturation, we find that the ice growth rate often exhibits a sudden increase that we attribute to an…

Materials Science · Physics 2008-09-30 Kenneth G. Libbrecht
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