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Forces between charged silica particles in solutions of multivalent coions are measured with colloidal probe technique based on atomic force microscopy. The concentration of 1:z electrolytes is systematically varied to understand the…

Soft Condensed Matter · Physics 2019-08-08 Biljana Uzelac , Valentina Valmacco , Gregor Trefalt

Explicit molecular dynamics simulations were applied to a pair of amorphous silica nanoparticles in aqueous solution, of diameter 4.4 nm with four different background electrolyte concentrations, to extract the mean force acting between the…

Chemical Physics · Physics 2009-11-13 S. Jenkins , S. R. Kirk , M. Persson , J. Carlen , Z. Abbas

The forces between colloidal particles at a decane-water interface, in the presence of low concentrations of a monovalent salt (NaCl) and of the surfactant sodium dodecylsulfate (SDS) in the aqueous subphase, have been studied using laser…

Soft Condensed Matter · Physics 2008-07-11 B. J. Park , J. P. Pantina , E. Furst , M. Oettel , S. Reynaert , J. Vermant

Experimental measurements of interactions in ionic liquids and concentrated electrolytes over the past decade or so have revealed simultaneous monotonic and oscillatory decay modes. These observations have been hard to interpret using…

Soft Condensed Matter · Physics 2024-02-28 Timothy S. Groves , Susan Perkin

The structure and interactions in electrolytes at high concentration have implications from energy storage to biomolecular interactions. However many experimental observations are yet to be explained in these mixtures, which are far beyond…

Soft Condensed Matter · Physics 2017-04-05 Alexander Smith , Alpha Lee , Susan Perkin

Explicit molecular dynamics simulations were applied to a pair of amorphous silica nanoparticles of diameter 3.2 nm immersed in a background electrolyte. Mean forces acting between the pair of silica nanoparticles were extracted at four…

Chemical Physics · Physics 2007-09-11 S. Jenkins , S. R. Kirk , M. Persson , J. Carlen , Z. Abbas

We consider the interactions between two uncharged planar macroscopic surfaces immersed in an electrolyte solution which are induced by interfacial selectivity. These forces are taken into account by introducing a depletion free-energy…

Soft Condensed Matter · Physics 2009-10-31 M. N. Tamashiro , P. Pincus

Recent experiments and a series of subsequent theoretical studies suggest the occurrence of universal underscreening in highly concentrated electrolyte solutions. We performed a set of systematic Atomic Force Spectroscopy measurements for…

The present article provides an overview of the recent progress in the direct force measurements between individual pairs of colloidal particles in aqueous salt solutions. Results obtained by two different techniques are being highlighted,…

Soft Condensed Matter · Physics 2016-06-02 Gregor Trefalt , Thomas Palberg , Michal Borkovec

Recent reports of surface forces across nanoconfined ionic liquids have revealed the existence of an anomalously long-ranged interaction apparently of electrostatic origin. Ionic liquids are viscous and therefore it is important to inspect…

Soft Condensed Matter · Physics 2018-01-04 Romain Lhermerout , Susan Perkin

We explore the force generation and surface interactions arising when electric fields are applied across fluid films. Using a surface force balance (SFB) we measure directly the force between two electrodes in crossed-cylinder geometry…

Soft Condensed Matter · Physics 2019-04-09 Carla Perez-Martinez , Susan Perkin

We study, using Monte Carlo simulations, the interaction between charged colloidal particles confined to the air-water interface. The dependence of force on ionic strength and counterion valence is explored. For 1:1 electrolyte, we find…

Soft Condensed Matter · Physics 2018-02-05 Matheus Girotto , Alexandre P. dos Santos , Yan Levin

The behavior of polyelectrolytes between charged surfaces immersed in semi-dilute solutions is investigated theoretically. A continuum mean field approach is used for calculating numerically concentration profiles between two electrodes…

Soft Condensed Matter · Physics 2007-05-23 I. Borukhov , D. Andelman , H. Orland

Optical microscopy and multi-particle tracking are used to investigate the spatially correlated motion of weakly charged silica spheres at an air-water interface for different area fraction $n$ occupied by the particles. When the area…

Soft Condensed Matter · Physics 2012-04-11 Wei Zhang , Wei Chen , Penger Tong

The interaction between charged objects in solution is generally expected to recapitulate two central principles of electromagnetics: (i) like-charged objects repel, and (ii) they do so regardless of the sign of their electrical charge.…

Soft Condensed Matter · Physics 2022-12-27 Sida Wang , Rowan Walker-Gibbons , Bethany Watkins , Melissa Flynn , Madhavi Krishnan

Responsive poly-N-isopropylacrylamide-based microgels are commonly used as model colloids with soft repulsive interactions. It has been shown that the microgel-microgel interaction in solution can be easily adjusted by varying the…

Soft Condensed Matter · Physics 2021-09-06 Steffen Bochenek , Cathy E. McNamee , Michael Kappl , Hans Juergen Butt , Walter Richtering

Charged colloidal particles trapped at an air--water interface are well known to form an ordered crystal, stabilized by a long ranged repulsion, the details of this repulsion remain something of a mystery, but all experiments performed to…

Soft Condensed Matter · Physics 2016-12-22 Duck-Gyu Lee , Pietro Cicuta , Dominic Vella

The electrostatic interaction between colloidal particles trapped at the interface between two immiscible electrolyte solutions is studied in the limit of small inter-particle distances. Within an appropriate model exact analytic…

Soft Condensed Matter · Physics 2014-05-07 Arghya Majee , Markus Bier , S. Dietrich

The description of forces across confined complex fluids still holds many challenges due to the possible overlap of different contributions. Here, an attempt is made to untangle the interaction between charged surfaces across nanoparticle…

Soft Condensed Matter · Physics 2021-01-06 Michael Ludwig , Regine von Klitzing

Previous experimental reports of long-range interactions in ionic liquids (ILs) stand in contradiction with theoretical predictions and numerical simulations. To provide insights into the literature discrepancies regarding the experimental…

Soft Condensed Matter · Physics 2026-03-24 Benjamin Cross , Léo Garcia , Elisabeth Charlaix , Patrick Kékicheff
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