Related papers: Photon-mediated charge-exchange reactions between …
We present a mass spectrometric technique for identifying the masses and relative abundances of Coulomb-crystallized ions held in a linear Paul trap. A digital radiofrequency waveform is employed to generate the trapping potential, as this…
Nanophotonic traps for cold atoms typically have trap volumes that are orders of magnitude smaller than, e.g., free-space optical tweezers. This makes efficient loading of these traps challenging, thereby limiting the total number of atoms…
Understanding the interaction between metal ions and their aqueous environment is fundamental in many areas of chemistry, biology, and environmental science. In this study, we investigate the electronic structure of hydrated calcium ions,…
We present a versatile and compact electron beam driven source for alkali metal atoms, which can be implemented in cryostats. With a heat load of less than 10mW, the heat dissipation normalized to the atoms loaded into the magneto-optical…
We present first indications of sympathetic cooling between two neutral, optically trapped atomic species. Lithium and cesium atoms are simultaneously stored in an optical dipole trap formed by the focus of a CO$_2$ laser, and allowed to…
We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that…
We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of…
It is challenging to parameterize the force field for calcium ions (Ca2+) in calcium-binding proteins because of their unique coordination chemistry that involves the surrounding atoms required for stability. In this work, we observed wide…
We report on reaching sub-Doppler temperatures of $^{40}$K in a single-chamber setup using a dispenser-based potassium source with natural (0.012$\%$ of $^{40}$K) isotopic composition. With gray molasses cooling on the $D_1$-line following…
We study theoretically the behavior of laser-cooled calcium monofluoride (CaF) molecules in an optical molasses and magneto-optical trap (MOT), and compare our results to recent experiments. We use multi-level optical Bloch equations to…
The lifetime of Ba$^+$ ions confined in a Paul trap is found, under typical conditions, to be limited by chemical reactions with residual background gas. An integrated ion trap and time-of-flight mass spectrometer are used to analyze the…
We present an experimental and theoretical study of atom-molecule collisions in a mixture of cold, trapped atomic nitrogen and NH molecules at a temperature of $\sim 600$~mK. We measure a small N+NH trap loss rate coefficient of…
We report the laser cooling of a single $^{40}\text{Ca}^+$ ion in a Penning trap to the motional ground state in one dimension. Cooling is performed in the strong binding limit on the 729-nm electric quadrupole $S_{1/2}\leftrightarrow…
Photoionization spectroscopy of cold cesium dimers obtained by photoassociation of cold atoms in a magneto-optical trap is reported here. In particular, we report on the observation and on the spectroscopic analysis of all the excited…
Using the ab initio computed Potential Energy Surface (PES) for the electronic interaction of the MgH$^+$ ($^1\Sigma$) ion with the He($^1$S) atom, we calculate the relevant state-changing rotationally inelastic collision cross sections…
The empirical coupled-channel (ECC) model and the universal fusion function (UFF) prescription are used to analyse the data of capture cross sections for reactions ${}^{39}$K$+{}^{181}$Ta and ${}^{46}$K$+{}^{181}$Ta reported recently by A.…
State-selected Coulomb-crystallized molecular ions were employed for the first time in ion-molecule reaction studies using the prototypical charge-transfer process $\mathrm{N_2^++N_2\rightarrow N_2+N_2^+}$ as an example. By preparing the…
We investigate the intermolecular interactions between laser-cooled CaF and Ca, in their ground and excited electronic states, aiming to understand atom-exchange reaction pathways. Using state-of-the-art \textit{ab initio} quantum chemistry…
We study optical gain in a gas of cold 39K atoms. The gain is observed during operation of a conventional magneto-optical trap without the need for additional fields. Measurements of transmission spectra from a weak probe show that the gain…
We present state-selected measurements of rotational cooling and excitation rates of CH$^+$ molecular ions by inelastic electron collisions. The experiments are carried out at the Cryogenic Storage Ring, making use of a monoenergetic…