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We report magnetic resonance spectroscopy measurements of individual nuclear spins in a crystal coupled to a neighbouring paramagnetic center, detected using microwave fluorescence at millikelvin temperatures. We observe real-time quantum…

Single-cell analysis can unravel functional heterogeneity within cell populations otherwise obscured by ensemble measurements. However, non-invasive techniques that probe chemical entities and their dynamics are still lacking. This…

Applied Physics · Physics 2023-06-14 Nick Ruben Neuling , Robin Derek Allert , Dominik Benjamin Bucher

Single-molecule detection with chemical specificity is a powerful and much desired tool for biology, chemistry, physics, and sensing technologies. Surface-enhanced spectroscopies enable single molecule studies, yet reliable substrates of…

Mesoscale and Nanoscale Physics · Physics 2008-02-22 D. R. Ward , N. K. Grady , C. S. Levin , N. J. Halas , Y. Wu , P. Nordlander , D. Natelson

We present a scheme of surface-sensitive nuclear magnetic resonance in optically pumped semiconductors, where an NMR signal from a part of the surface of a bulk compound semiconductor is detected apart from the bulk signal. It utilizes…

Mesoscale and Nanoscale Physics · Physics 2008-09-12 Atsushi Goto , Tadashi Shimizu , Kenjiro Hashi , Shinobu Ohki

Understanding light-matter interaction at the nanoscale requires probing the optical properties of matter at the individual nano-absorber level. To this end, we have developed a nanomechanical photothermal sensing platform that can be used…

Optics · Physics 2024-06-07 Kostas Kanellopulos , Robert G. West , Silvan Schmid

Mechanical resonators operating in the megahertz range have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also appealing for force…

Mesoscale and Nanoscale Physics · Physics 2026-04-20 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

On chip exciting electric modes in individual plasmonic nanostructures are realized widely; nevertheless, the excitation of their magnetic counterparts is seldom reported. Here, we propose a highly efficient on chip excitation approach of…

Optics · Physics 2021-12-15 Yingke Ji , Binbin Wang , Liang Fang , Qiang Zhao , Fajun Xiao , Xuetao Gan

A series of test experiments on three different Si-based neutron detectors, namely a 1-d 128 channel, 0.5 mm space resolution Si microstrip sensor coupled to natural Gd converter, a medium size ? 1 cm2 PIN diode coupled to nGd2O3 or…

Instrumentation and Detectors · Physics 2018-05-04 G. Mauri , M. Mariotti , F. Casinini , F. Sacchetti , C. Petrillo

Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial,…

Low thermal polarization of nuclear spins is a primary sensitivity limitation for nuclear magnetic resonance. Here we demonstrate optically pumped (microwave-free) nuclear spin polarization of $^{13}\mathrm{C}$ and $^{15}\mathrm{N}$ in…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Ben L. Green , Ben G. Breeze , Gregory J. Rees , John V. Hanna , Jyh-Pin Chou , Viktor Ivády , Adam Gali , Mark E. Newton

We describe how a local non-equilibrium nuclear polarisation can be generated and detected by electrical means in a semiconductor quantum point contact device. We show that measurements of the nuclear spin relaxation rate will provide clear…

Mesoscale and Nanoscale Physics · Physics 2008-06-26 N. R. Cooper , V. Tripathi

Performing nanoscale scanning electron paramagnetic resonance (EPR) requires three essential ingredients. First, a static magnetic field together to field gradients to Zeeman split the electronic energy levels with spatial resolution.…

Mesoscale and Nanoscale Physics · Physics 2024-01-16 Carlos A. González-Gutiérrez , David García-Pons , David Zueco , María José Martínez-Pérez

The possibility that strongly correlated many-electron systems may exhibit spin-charge separation has generated great excitement, particularly in the light of recent experiments on low dimensional conductors and high temperature…

Strongly Correlated Electrons · Physics 2007-05-23 Nic Shannon

Tunneling spectroscopy measurements have been carried out on a single molecule device formed by two Pd nanocrystals (dia, $\sim$5 nm) electronically coupled by a conducting molecule, dimercaptodiphenylacetylene. The I-V data, obtained by…

Materials Science · Physics 2007-05-23 Ved Varun Agrawal , Reji Thomas , G. U. Kulkarni , C. N. R. Rao

We report bulk, room-temperature hyperpolarization of 13C nuclear spins observed via high-field nuclear magnetic resonance (NMR). The hyperpolarization is achieved by optical pumping (OP) of nitrogen vacancy defect centers in diamond…

We demonstrate an experimental method to separately test the optical response of a single sub-wavelength nano-structure to tailored electric and magnetic field distributions in the optical domain. For this purpose a highly focused…

Optics · Physics 2015-05-18 P. Banzer , U. Peschel , S. Quabis , G. Leuchs

Fundamental weak interactions have been shown to violate parity in both nuclear and atomic systems. However, observation of parity violation in a molecular system has proven an elusive target. Nuclear spin dependent contributions of the…

Magnetic media remain a key in information storage and processing. The continuous increase of storage densities and the desire for quantum memories and computers pushes the limits of magnetic characterisation techniques. Ultimately, a tool…

Magnetic-field and microwave-frequency modulated DNP experiments have been shown to yield improved enhancements over conventional DNP techniques, and even to shorten polarization build-up times. The resulting increase in signal-to-noise…

Instrumentation and Detectors · Physics 2015-12-23 Mallory L. Guy , Lihuang Zhu , Chandrasekhar Ramanathan