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We examine the archetype of an interference experiment for Auger electrons: two electron wave packets are launched by inner-shell ionizing a krypton atom using two attosecond light pulses with a variable time delay. This setting is an…

Atomic Physics · Physics 2015-03-13 Christian Buth , Kenneth J. Schafer

We demonstrate the generation of a train of attosecond XUV pulses that are in a superposition of wavefront states. Such superposition yields a high precision, self-referencing, common path XUV interferometer setup to produce pairs of…

Intense X-ray free-electron lasers (XFELs) can rapidly excite matter, leaving it in inherently unstable states that decay on femtosecond timescales. As the relaxation occurs primarily via Auger emission, excited state observations are…

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

Extreme ultraviolet (XUV) attosecond pulses, generated by a process known as laser-induced electron recollision, are a key ingredient for attosecond metrology, providing a tool to precisely initiate and probe sub-femtosecond dynamics in the…

Atomic Physics · Physics 2016-02-24 Yunpei Deng , Zhinan Zeng , Zhengmao Jia , Pavel Komm , Yinhui Zheng , Xiaochun Ge , Ruxin Li , Gilad Marcus

Attosecond x-ray pulses play a crucial role in the study of ultrafast phenomena occurring within inner and valence electrons. To achieve attosecond time-resolution studies and gain control over electronic wavefunctions, it is crucial to…

Accelerator Physics · Physics 2024-01-30 Hao Sun , Xiaofan Wang , Weiqing Zhang

Electrons photoemitted by extreme ultraviolet attosecond pulses derive spatially from the first few atomic surface layers and energetically from the valence band and highest atomic orbitals. As a result, it is possible to probe the emission…

Time-Delay Interferometry (TDI) is the data processing technique that cancels the large laser phase fluctuations affecting the one-way Doppler measurements made by unequal-arm space-based gravitational wave interferometers. By taking finite…

General Relativity and Quantum Cosmology · Physics 2022-05-11 Sanjeev Dhurandhar , Prasanna Joshi , Massimo Tinto

We calculate the transient absorption of an isolated attosecond pulse by helium atoms subject to a delayed infrared (\ir) laser pulse. With the central frequency of the broad attosecond spectrum near the ionization threshold, the absorption…

Atomic Physics · Physics 2015-06-12 Shaohao Chen , Mengxi Wu , Mette B. Gaarde , Kenneth J. Schafer

Time-resolved electronic processes on the attosecond scale have recently become experimentally accessible through the development of laser-based pump-probe interrogation techniques such as the attosecond streak camera, the reconstruction of…

Atomic Physics · Physics 2022-06-02 Hongcheng Ni , Stefan Donsa , Xiaochun Gong , Kiyoshi Ueda , Jian Wu , Joachim Burgdörfer

Attosecond x-ray pulse with known spectro-temporal information is an essential tool for the investigation of ultrafast electron dynamics in quantum systems. Ultrafast free-electron lasers (FELs) have the unique advantage on unprecedented…

Accelerator Physics · Physics 2023-04-17 Yaozong Xiao , Hao Sun , Bo Liu , Zhentang Zhao , Chao Feng

We study theoretically the reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) in strongly polar molecules. The time-dependent energy of a polar molecule in the infrared (IR) field gives rise to an…

Atomic Physics · Physics 2024-01-30 Jakub Benda , Zdeněk Mašín

First time-resolved photoemission experiments employing attosecond streaking of electrons emitted by an XUV pump pulse and probed by a few-cycle NIR pulse found a time delay of about 100 attoseconds between photoelectrons from the…

Other Condensed Matter · Physics 2015-05-13 C. Lemell , B. Solleder , K. Tokesi , J. Burgdoerfer

We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a…

Atomic Physics · Physics 2015-01-14 Álvaro J. Galán , Luca Argenti , Fernando Martín

Measuring the time it takes to remove an electron from an atom or molecule during photoionization using newly developed attosecond spectroscopies has been a focus of many recent experiments. However, the outcome of such measurement depends…

Atomic Physics · Physics 2017-03-08 Lisa Torlina , Olga Smirnova

Tunnelling, one of the key features of quantum mechanics, ignited an ongoing debate about the value, meaning and interpretation of 'tunnelling time'. Until recently the debate was purely theoretical, with the process considered to be…

Time-delay interferometry (TDI) is a post-processing technique used to reduce laser noise in heterodyne interferometric measurements with unequal armlengths, a situation characteristic of space gravitational detectors such as Laser…

General Relativity and Quantum Cosmology · Physics 2021-07-14 Jean-Baptiste Bayle , Olaf Hartwig , Martin Staab

Photoelectron interferometry with femto- and atto-second light pulses is a powerful probe of the fast electron wavepacket dynamics, albeit it has practical limitations on the energy resolution. We show that one can simultaneously obtain…

Atomic Physics · Physics 2022-02-24 A. Plunkett , M. A. Alarcon , J. K. Wood , C. H. Greene , A. Sandhu

We study experimentally the influence of the intensity of the infrared (IR) probe field on attosecond pulse train (APT) phase measurements performed with the RABITT method (Reconstruction of Attosecond Beating by Interference in Two-Photon…

Atomic Physics · Physics 2009-07-22 M. Swoboda , J. M. Dahlstrom , T. Ruchon , P. Johnsson , J. Mauritsson , K. J. Schafer , A. L'Huillier

We report measurements of energy-dependent attosecond photoionization delays between the two outer-most valence shells of N$_2$O and H$_2$O. The combination of single-shot signal referencing with the use of different metal foils to filter…

Atomic Physics · Physics 2016-09-21 Martin Huppert , Inga Jordan , Denitsa Baykusheva , Aaron von Conta , Hans Jakob Wörner