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We have developed an extreme ultraviolet (XUV) frequency comb for performing ultra-high precision spectroscopy on the many XUV transitions found in highly charged ions (HCI). Femtosecond pulses from a 100 MHz phase-stabilized near-infrared…

The remarkable precision of frequency comb (FC) lasers is transferred to the extreme ultraviolet (XUV, wavelengths shorter than 100 nm), a frequency region previously not accessable to these devices. A frequency comb at XUV wavelengths near…

We review the current state of tabletop extreme ultraviolet (XUV) sources based on high harmonic generation (HHG) in femtosecond enhancement cavities (fsEC). Recent developments have enabled generation of high photon flux (1014 photons/sec)…

Optics · Physics 2015-06-05 Arthur K Mills , TJ Hammond , Matthew HC Lam , David J Jones

A chirped-pulse electro-optic (EO) dual comb system operating near 821 nm is used to generate cavity enhanced dual combs in the ultraviolet (UV) region near 323 nm with an optical bandwidth of up to 90 GHz. The UV combs result from…

Optics · Physics 2026-03-10 Jasper R. Stroud , David F. Plusquellic

We report on the realization of a solid-state-based vacuum ultraviolet frequency comb, using multi-harmonic generation in an external enhancement cavity. Optical conversions in such arrangements were so-far reported only using gaseous…

Optics · Physics 2019-03-27 J. Seres , E. Seres , C. Serrat , Erin C. Young , James S. Speck , T. Schumm

Extreme ultraviolet frequency combs are a versatile tool with applications including precision measurement, strong-field physics, and solid-state physics. Here we report on an application of extreme ultraviolet frequency combs and their…

Optics · Physics 2016-01-26 Craig Benko , Linqiang Hua , Thomas K. Allison , François Labaye , Jun Ye

Development of the optical frequency comb has revolutionised metrology and precision spectroscopy due to its ability to provide a precise and direct link between microwave and optical frequencies. A novel application of frequency comb…

External passive femtosecond enhancement cavities (fsECs) are widely used to increase the efficiency of non-linear conversion processes like high harmonic generation (HHG) at high repetition rates. Their performance is often limited by beam…

Ultraviolet frequency combs enable applications ranging from precision spectroscopy to atomic clocks by addressing the electronic transitions of atoms and molecules. Access to ultraviolet light via integrated nonlinear optics is usually…

Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

We present a high efficiency source of picosecond pulses derived from a dual cavity optical frequency comb generator. This approach overcomes the limitations of single cavity comb generators that are restricted to efficiencies of a few…

Optics · Physics 2023-07-28 Mateusz P. Mrozowski , Jonathan D. Pritchard , J. Jeffers

Many atomic and molecular systems of fundamental interest possess resonance frequencies in the extreme ultraviolet (XUV) where laser technology is limited and radiation sources have traditionally lacked long-term phase coherence. Recent…

We demonstrate a novel technique for coupling XUV harmonic radiation out of a femtosecond enhancement cavity. We use a small-period diffraction grating etched directly into the surface of a dielectric mirror. For the fundamental light, this…

Optics · Physics 2009-11-13 D. C. Yost , T. R. Schibli , Jun Ye

Vacuum ultraviolet (VUV) light is critical for the study of molecules and materials, but the generation of femtosecond pulses in the VUV region at high repetition rates has proven difficult. Here, we demonstrate the efficient generation of…

Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…

Atomic Physics · Physics 2015-05-27 P. Tzallas , E. Skantzakis , L. A. A. Nikolopoulos , G. D. Tsakiris , D. Charalambidis

Novel table-top sources of extreme-ultraviolet light based on high-harmonic generation yield unique insight into the fundamental properties of molecules, nanomaterials, or correlated solids, and enable advanced applications in imaging or…

The operation of a frequency comb at extreme ultraviolet (XUV) wavelengths based on pair-wise amplification and nonlinear upconversion to the 15th harmonic of pulses from a frequency comb laser in the near-infrared range is reported.…

We report the generation of the 5th harmonic of Ti:sapphire, at 160 nm, with more than 4~$\mu$J of pulse energy, and a pulse length of 37 fs with a 1 kHz repetition rate. The VUV pulses are produced using Four-Wave Difference Frequency…

Optics · Physics 2024-04-01 Ruaridh Forbes , Paul Hockett , Quentin Leterrier , Rune Lausten

In the present work we report on the current progress of the recently constructed GW attosecond extreme ultraviolet (XUV) source developed at the Institute of Electronic Structure and Laser of the Foundation for Research and…

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