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Using a Langmuir-Blodgett (LB) synthesis method, novel two-dimensional (2D) mixed-spin magnetic systems, in which each magnetic layer is both structurally and magnetically isolated, have been generated. Specifically, a 2D Fe-Ni…

Strongly Correlated Electrons · Physics 2009-11-07 J. -H. Park , J. T. Culp , D. W. Hall , D. R. Talham , M. W. Meisel

We report the magnetic properties of newly synthesized, single crystals of $\mathrm{TbTi_3Bi_4}$ whose crystal structure is highlighted by the stacking of terbium-based zigzag chains and titanium-based kagome lattices. This compound…

Strongly Correlated Electrons · Physics 2024-05-16 Kaizhen Guo , Zeyu Ma , Hongxiong Liu , Ziyang Wu , Junfeng Wang , Youguo Shi , Yuan Li , Shuang Jia

The high-field ground state of the competing-spin-chain compound Cs2Cu2Mo3O12 with the ferromagnetic first-nearest-neighbor J1=-93 K and the antiferromagnetic second-nearest-neighbor J2 = +33 K was investigated by 133Cs-NMR. A divergence of…

Statistical Mechanics · Physics 2013-09-24 Yukihiro Hoshino , Soichiro Atarashi , Takayuki Goto , Masashi Hase , Takahiko Sasaki

We derive a quantum spin Hamiltonian of the spin-1/2 zigzag chain realized in a rare earth ytterbium-based magnetic insulator, YbCuS2. This material undergoes a transition at 0.95K to an incommensurate magnetic phase with small moments,…

Strongly Correlated Electrons · Physics 2024-08-02 Hidehiro Saito , Hiroki Nakai , Chisa Hotta

We synthesize homogeneous compositions of NaLu$_x$Yb$_{1-x}$Se$_2$, connecting non-magnetic NaLuSe$_2$ to the triangular lattice spin liquid candidate NaYbSe$_2$. Thermal and magnetic properties are studied as the system evolves from one…

Quantum spin liquid (QSL) phases exist in theory, but real candidate QSL materials are often extraordinarily sensitive to structural defects which disrupt the ground state. Here, we investigate candidate triangular QSL material…

Low dimensional quantum magnets are interesting because of the emerging collective behavior arising from strong quantum fluctuations. The one-dimensional (1D) S = 1/2 Heisenberg antiferromagnet is a paradigmatic example, whose low-energy…

Magnetic moments arranged at the corners of a honeycomb lattice are predicted to form a novel state of matter, Kitaev quantum spin liquid, under the influence of frustration effects between bond-dependent Ising interactions. Some layered…

Strongly Correlated Electrons · Physics 2022-03-09 Sean K. Takahashi , Jiaming Wang , Alexandre Arsenault , Mykola Abramchuk , Fazel Tafti , Philip M. Singer , Takashi Imai

We present local probe results on the honeycomb lattice antiferromagnet Ba3CuSb2O9. Muon spin relaxation measurements in zero field down to 20 mK show unequivocally that there is a total absence of spin freezing in the ground state. Sb NMR…

Strongly Correlated Electrons · Physics 2015-06-05 J. A. Quilliam , F. Bert , E. Kermarrec , C. Payen , C. Guillot-Deudon , P. Bonville , C. Baines , H. Luetkens , P. Mendels

We present the dynamical spin structure factor of the antiferromagnetic spin-$\frac{1}{2}$ $J_1-J_2$ Heisenberg model on a triangular lattice obtained from large-scale matrix-product state simulations. The high frustration due to the…

Strongly Correlated Electrons · Physics 2023-12-11 Markus Drescher , Laurens Vanderstraeten , Roderich Moessner , Frank Pollmann

Magnetic, thermodynamic, neutron diffraction and inelastic neutron scattering are used to study spin correlations in the easy-axis XXZ triangular lattice magnet K2Co(SeO3)2. Despite the presence of quasi-2D "supersolid" magnetic order, the…

Strongly Correlated Electrons · Physics 2024-11-04 M. Zhu , V. Romerio , N. Steiger , S. D. Nabi , N. Murai , S. Ohira-Kawamura , K. Yu. Povarov , Y. Skourski , R. Sibille , L. Keller , Z. Yan , S. Gvasaliya , A. Zheludev

The topologically-protected, chiral soliton lattice is a unique state of matter offering intriguing functionality and it may serve as a robust platform for storing and transporting information in future spintronics devices. While the…

Strongly Correlated Electrons · Physics 2019-04-12 A. A. Aczel , L. M. DeBeer-Schmitt , T. J. Williams , M. A. McGuire , N. J. Ghimire , L. Li , D. Mandrus

Competing magnetic interactions in low-dimensional quantum magnets can lead to the exotic ground state with fractionalized excitations. Herein, we present our results on an S = 5/2 quasi-one-dimensional spin system Bi3FeMo2O12. The…

We apply moderate-high-energy inelastic neutron scattering (INS) measurements to investigate Yb$^{3+}$ crystalline electric field (CEF) levels in the triangular spin-liquid candidate YbMgGaO$_4$. Three CEF excitations from the ground-state…

A primary goal at the interface of theoretical and experimental quantum magnetism is the investigation of exotic spin states, most notably quantum spin liquids (QSLs). Magnetic rare-earth ions go beyond the straightforward paradigm of…

Strongly Correlated Electrons · Physics 2022-01-11 Christopher A. Pocs , Peter E. Siegfried , Jie Xing , Athena S. Sefat , Michael Hermele , Bruce Normand , Minhyea Lee

We report 7Li NMR, magnetic susceptibility, and heat capacity measurements on the triangular lattice Heisenberg antiferromagnet compound LiCrO2. We find that in contrast to NaCrO2, magnetic properties of LiCrO2 have a more pronounced three…

Strongly Correlated Electrons · Physics 2007-05-23 L. K. Alexander , N. Buettgen , R. Nath , A. V. Mahajan , A. Loidl

Here, we report both ac and dc magnetization, thermodynamic and electric properties of hexagonal Ba$_3$NiIr$_2$O$_9$. The Ni$^{2+}$ (spin-1) forms layered triangular-lattice and interacts antiferromagnetically while Ir$^{5+}$ is believed to…

Strongly Correlated Electrons · Physics 2021-07-14 Shobha Gondh , Manju Mishra Patidar , Kranti Kumar , M. P. Saravanan , V. Ganesan , A. K. Pramanik

Motivated by recent experiments on the material Ba_3NiSb_2O_9 we consider a spin-one quantum antiferromagnet on a triangular lattice with the Heisenberg bilinear and biquadratic exchange interactions and a single-ion anisotropy. Using a…

Strongly Correlated Electrons · Physics 2012-08-30 Maksym Serbyn , T. Senthil , Patrick A. Lee

The cradle of quantum spin liquids, triangular antiferromagnets show strong proclivity to magnetic order and require deliberate tuning to stabilize a spin-liquid state. In this brief review, we juxtapose recent theoretical developments that…

Strongly Correlated Electrons · Physics 2020-03-13 Yuesheng Li , Philipp Gegenwart , Alexander A. Tsirlin

We report on high-field electron spin resonance (ESR) studies of magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs$_2$CuBr$_4$. Frequency-field diagrams of ESR excitations are measured for different orientations of…

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