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Light offers a route to engineer new phases of matter far from equilibrium, including transient states suggestive of superconducting, charge-ordered, and excitonic ordering behavior. Yet it remains unclear how optical excitation can…

Superconductivity · Physics 2025-09-09 Mattia Moroder , Sebastian Paeckel , Matteo Mitrano , John Sous

In pursuit of rational control of orbital polarization, we present a combined experimental and theoretical study of single unit cell superlattices of the correlated metal LaNiO$_3$ and the band insulator LaAlO$_3$. Polarized x-ray…

Strongly Correlated Electrons · Physics 2012-01-23 J. W. Freeland , Jian Liu , M. Kareev , B. Gray , J. W. Kim , P. Ryan , R. Pentcheva , J. Chakhalian

We explore the tunability of the phonon polarization in suspended uniaxially strained graphene by magneto-phonon resonances. The uniaxial strain lifts the degeneracy of the LO and TO phonons, yielding two cross-linearly polarized phonon…

Mesoscale and Nanoscale Physics · Physics 2021-04-15 Jens Sonntag , Sven Reichardt , Bernd Beschoten , Christoph Stampfer

We utilize ultrafast photoexcitation to drive coherent lattice oscillations in the layered ferrimagnetic crystal Mn3Si2Te6, which significantly stiffen below the magnetic ordering temperature. We suggest that this is due to an…

Nonlinear phononics provides a route to control crystal structures through light-induced phonon excitation. In this study, we apply nonlinear phononics to an iron-based superconductor, LaFeAsO, with the aim of tuning its crystal structure…

Superconductivity · Physics 2026-04-09 Shu Kamiyama , Tatsuya Kaneko , Kazuhiko Kuroki , Masayuki Ochi

Driving materials using light with more than one frequency component is an emerging technique, enabled by advanced pulse-shaping capabilities in recent years. Here, we translate this technique to lattice vibrations, by exciting multicolor…

Materials Science · Physics 2025-04-07 Omer Yaniv , Dominik M. Juraschek

In this paper we present a novel scheme for the controlled generation of of tunable narrowband gamma-ray radiation by ultra-relativistic positron beams inside acoustically driven periodically bent crystals. A novel acoustic crystalline…

We investigate coherent lattice dynamics in optimally doped YBa$_2$Cu$_3$O$_{7-\delta}$ driven by ultrashort ($\sim$ 12 fs) near infrared (NIR) and near ultraviolet (NUV) pulses. Transient reflectivity experiments, performed at room…

Materials Science · Physics 2023-05-08 Kunie Ishioka , Alexej Pashkin , Christian Bernhard , Hrvoje Petek , Xin Yao , Jure Demsar

The phonon dynamics in a one dimensional Heisenberg spin chain coupled to finite-frequency bond phonons is studied. We present the first detailed phonon spectra for these systems using Quantum Monte Carlo. The quantum phase transition is…

Strongly Correlated Electrons · Physics 2007-05-23 Franz Michel , Hans-Gerd Evertz

The dominant phonon wavevectors $q^{*}$ probed by the 2D Raman mode of graphene are highly anisotropic and rotate with the orientation of the polarizer:analyzer direction relative to the lattice. The corresponding electronic transitions…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Rohit Narula , Nicola Bonini , Nicola Marzari , Stephanie Reich

Optical systems are scalable under low-intensity illumination since their governing equations are linearly dependent of the optical signal strength. Nonetheless, in high-intensity regimes, the induced polarization becomes nonlinear,…

Coherent excitation of shear phonons in van der Waals layered materials is a non-destructive mechanism to fine-tune the electronic state of the system. We develop a diagrammatic theory for the displacive Raman force and apply it to the…

Mesoscale and Nanoscale Physics · Physics 2022-10-19 Habib Rostami

Nonlinear processes involving frequency-mixing of light fields set the basis for ultrafast coherent spectroscopy of collective modes in solids. In certain semimetals and semiconductors, generation of coherent phonon modes can occur by a…

In bilayer CrI3, experimental and theoretical studies suggest that the magnetic order is closely related to the layer staking configuration. In this work, we study the effect of dynamical lattice distortions, induced by non-linear phonon…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. Rodriguez-Vega , Ze-Xun Lin , A. Leonardo , A. Ernst , G. Chaudhary , M. G. Vergniory , Gregory A. Fiete

Recent advances in nanowire synthesis have enabled the realization of crystal phases that in bulk are attainable only under extreme conditions, i.e. high temperature and/or high pressure. For group IV semiconductors this means access to…

Rotational excitation of polar molecules trapped in an optical lattice gives rise to rotational excitons. Here we show that non-linear interactions of such excitons can be controlled by an electric field. The exciton--exciton interactions…

Mesoscale and Nanoscale Physics · Physics 2012-06-20 Ping Xiang , Marina Litinskaya , Roman V. Krems

Lattice vibration in solids may carry angular momentum. But unlike the intrinsic spin of electrons, the lattice vibration is rarely rotational. To induce angular momentum, one needs to find a material that can accommodate a twisted normal…

Materials Science · Physics 2021-09-29 G. P. Zhang , Y. H. Bai , Thomas F. George

We present a Raman scattering study of Ca$_2$RuO$_4$, in which we investigate the temperature-dependence of the lattice dynamics and the electron-phonon interaction below the metal-insulator transition temperature ({\it T}$_{\rm MI}$).…

Strongly Correlated Electrons · Physics 2009-11-11 H. Rho , S. L. Cooper , S. Nakatsuji , H. Fukazawa , Y. Maeno

Lattice vibrations carrying angular momentum, known as chiral phonons, have emerged as a promising route to control and understand complex material properties, yet their deterministic manipulation remains largely unexplored. Here we…

The multi-order Raman scattering is studied up to a fourth order for a detwinned LaMnO_3 crystal. Based on a comprehensive data analysis of the polarisation-dependent Raman spectra, we show that the anomalous features in the multi-order…

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