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We generalize the one electron attosecond streaking camera to time-resolve the correlated two-electron escape dynamics during a collision process involving a deep core electron. The collision process is triggered by an XUV attosecond pulse…

Atomic Physics · Physics 2010-03-09 A. Emmanouilidou , A. Staudte , P. B. Corkum

Ultrafast processes in matter, such as the electron emission following light absorption, can now be studied using ultrashort light pulses of attosecond duration ($10^{-18}$s) in the extreme ultraviolet spectral range. The lack of spectral…

Phase retrieval is a prevalent problem in digital signal processing and experimental physics that consists of estimating a complex signal from magnitude measurements. This paper expands the classical phase retrieval framework to electric…

Signal Processing · Electrical Eng. & Systems 2023-05-17 Samuel Talkington , Santiago Grijalva

The development of schemes for coherent nonlinear time-domain spectroscopy in the extreme-ultraviolet regime (XUV) has so far been impeded by experimental difficulties that arise at these short wavelengths. In this work we present a novel…

Conventional methods of wavefront reconstruction from the raw data of the Shack-Hartmann sensor use the focal spot shifts and discard the high-frequency information about the wavefront. Phase-retrieval-based methods treat the Hartmann…

We develop and exactly solve a model for electrons driven by pulsed or continuous ac fields. The theory includes both the photoexcitation process as well as the subsequent acceleration of the electrons. In the case of an ac response, we…

Strongly Correlated Electrons · Physics 2015-01-12 W. S. Shen , T. P. Devereaux , J. K. Freericks

We report attosecond-scale probing of the laser-induced dynamics in molecules. We apply the method of high-harmonic spectroscopy, where laser-driven recolliding electrons on various trajec- tories record the motion of their parent ion.…

The attoclock is a powerful tool for probing ultrafast electron dynamics with attosecond precision.Here, we demonstrate an all-optical terahertz (THz) attoclock that reconstructs photoionization dynamics by detecting the THz radiation…

Attosecond streaking camera is an ex situ technique in which a linearly polarized (LP) XUV attopulse produces an electron wavepacket by photoionization in the presence of an IR femtopulse. By moving the two synchronous oppositely circularly…

Atomic Physics · Physics 2025-11-27 M. A. H. B. Md Yusoff , H. B. Ambalampitiya , J. M. Ngoko Djiokap

Photoelectron holography constitutes a powerful tool for the ultrafast imaging of matter, as it combines high electron currents with subfemtosecond resolution, and gives information about transition amplitudes and phase shifts. Similarly to…

Atomic Physics · Physics 2020-02-19 C. Figueira de Morisson Faria , A. S. Maxwell

In a recent publication, Dalen, and Selst{\o}, Phys. Rev. A {\bf 111}, 033116 (2025), it was demonstrated how converged photo electron spectra could be determined using a complex absorbing potential on a truncated numerical domain…

Quantum Physics · Physics 2025-10-14 Selstø Sølve , Bendik Steinsvåg Dalen

Half of wavefunction information is undetected by conventional transmission electron microscopy (CTEM) as only the intensity, and not the phase, of an image is recorded. Following successful applications of deep learning to optical hologram…

Image and Video Processing · Electrical Eng. & Systems 2020-01-31 Jeffrey M. Ede , Jonathan J. P. Peters , Jeremy Sloan , Richard Beanland

Action-detected two-dimensional electronic spectroscopy (A-2DES) provides valuable insights into ultrafast dynamics within functional materials and devices by measuring incoherent signals like photocurrent. This work details the…

Chemical Physics · Physics 2025-06-04 E. Amarotti , L. Bolzonello , S. -H. Lee , D. Zigmantas , N. -G. Park , N. van Hulst , T. Pullerits

Studies of ultrafast dynamics along with femtosecond-pulse metrology rely on non-linear processes, induced solely by the exciting/probing pulses or the pulses to be characterized. Extension of these approaches to the extreme-ultraviolet…

Atomic Physics · Physics 2015-05-27 P. Tzallas , E. Skantzakis , L. A. A. Nikolopoulos , G. D. Tsakiris , D. Charalambidis

The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…

Atomic Physics · Physics 2008-02-27 J. Mauritsson , P. Johnsson , E. Gustafsson , M. Swoboda , T. Ruchon , A. LHuillier , K. J. Schafer

Tremendous advances in laser pump-probe techniques open the door for the observation in real time of ultrafast \textit{electronic} processes. Particularly attractive is the visualization of interatomic processes where one can follow the…

Atomic and Molecular Clusters · Physics 2007-05-23 Alexander I. Kuleff , Lorenz S. Cederbaum

A novel and universal interference structure is found in the photoelectron momentum distribution of atoms in intense infrared laser field. Theoretical analysis shows that this structure can be attributed to a new form of…

We analyze the time delay between emission of photoelectrons from the outer valence $ns$ and $np$ sub-shells in noble gas atoms following absorption of an attosecond XUV pulse. By solving the time dependent Schr\"odinger equation and…

Atomic Physics · Physics 2010-12-07 A. S. Kheifets , I. A. Ivanov

Recollision physics and attosecond pulse generation meld the precision of optics with collision physics. As a follow-up to our previous work, we reveal a new direction for the study of electronic structure and multielectron dynamics by…

Atomic Physics · Physics 2023-06-06 Chunmei Zhang , Graham G. Brown , Dong Hyuk Ko , Paul B. Corkum

The well-known phase problem which means image reconstruction from only spectrum magnitude without using any spectrum phase information is considered basically in application to VLBI mapping of compact extragalactic radio sources (active…

Instrumentation and Methods for Astrophysics · Physics 2012-11-13 A. T. Bajkova
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