Related papers: Complete phase retrieval of photoelectron wavepack…
We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…
Tracking the coupled motion of electrons and nuclei on their intrinsic timescales is essential to understanding and controlling photochemical transformations. While attosecond techniques have provided unprecedented insight into electronic…
Numerical simulations are presented to validate the possible use of cutting-edge attosecond time- resolved photoelectron spectroscopy to observe in real time the creation of an electronic wavepacket and subsequent electronic motion in a…
The classical problem of phase retrieval has found a wide array of applications in optics, imaging and signal processing. In this paper, we consider the phase retrieval problem in a one-bit setting, where the signals are sampled using…
We investigate the possibility to use transient absorption of a coherent bound electron wave packet in hydrogen as an attosecond pulse characterization technique. In recent work we have shown that photoionization of such a coherent bound…
We investigate the photoionization spectrum of helium by attosecond XUV pulses both in the spectral region of doubly excited resonances as well as above the double ionization threshold. In order to probe for convergence, we compare three…
Attosecond streaking of photoelectrons emitted by extreme ultraviolet light has begun to reveal how electrons behave during their transport within simple crystalline solids. Many sample types within nanoplasmonics, thin-film physics, and…
Phase retrieval approaches based on DL provide a framework to obtain phase information from an intensity hologram or diffraction pattern in a robust manner and in real time. However, current DL architectures applied to the phase problem…
If matter absorbs a photon of sufficient energy it emits an electron. The question of the duration of the emission process has intrigued scientists for decades. With the advent of attosecond metrology, experiments addressing such ultrashort…
Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…
Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…
Previously reported crystalline structures obtained by an iterative phase retrieval reconstruction of their diffraction patterns seem to be free from displaying any irregularities or defects in the lattice, which appears to be unrealistic.…
Laser-assisted photoemission from a solid is considered within a numerically exactly solvable one-dimensional model of a crystal. The effect of the inelastic scattering and of the finite duration of the pump pulse on the photoelectron…
The recent development of Homochromatic Attosecond Streaking (HAS) has enabled a novel, highly precise method for ultrafast metrology of attosecond electron pulses as well as for real-time sampling of the instantaneous field waveforms of…
We introduce a phase imaging mechanism for scanning transmission electron microscopy that exploits the complementary intensity changes of transmitted disks at different scattering angles. For scanning transmission electron microscopy, this…
In this paper we consider the nonlinear inverse problem of phase retrieval in the context of dynamical sampling. Where phase retrieval deals with the recovery of signals & images from phaseless measurements, dynamical sampling was…
We demonstrate the complete reconstruction of the electric field of visible-infrared pulses with energy as low as a few tens of nanojoules. The technique allows for the reconstruction of the instantaneous electric field vector direction and…
Strongly laser-driven semiconductor crystals offer substantial advantages for the study of many-body physics and ultrafast optoelectronics via the high harmonic generation process. While this phenomenon has been employed to investigate the…
Attosecond science has been transforming our understanding of electron dynamics in atoms, molecules and solids. However, to date almost all of the attoscience experiments have been based on spectroscopic measurements because attosecond…
We propose a protocol to probe the ultrafast evolution and dephasing of coherent electronic excitation in molecules in the time domain by the intrinsic streaking field generated by the molecule itself. Coherent electronic motion in the…