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Among the 'beyond Li-ion' battery chemistries, nonaqueous Li-O$_2$ batteries have the highest theoretical specific energy and as a result have attracted significant research attention over the past decade. A critical scientific challenge…

Using dielectric spectroscopy and differential scanning calorimetry, we have performed a detailed investigation of the influence of water uptake on the translational and reorientational glassy dynamics in the typical ionic liquid…

Materials Science · Physics 2017-01-23 P. Sippel , V. Dietrich , D. Reuter , M. Aumüller , P. Lunkenheimer , A. Loidl , S. Krohns

We determine the phase diagram of liquid supercooled water by extensive computer simulations using the TIP5P-E model [J. Chem. Phys. {\bf 120}, 6085 (2004)]. We find that the transformation of water into a low density liquid in the…

Statistical Mechanics · Physics 2007-05-23 Dietmar Paschek

In the present work, we study an electrolyte solution confined between planar surfaces with nonopatterned charged domains, which has been connected to a bulk ionic reservoir. The system is investigated through an improved Monte Carlo (MC)…

Soft Condensed Matter · Physics 2020-09-29 Amin Bakhshandeh , Maximiliano Segala , Thiago Colla

Controlling the charge density in low-dimensional materials with an electrostatic potential is a powerful tool to explore and influence their electronic and optical properties. Conventional solid gates impose strict geometrical constraints…

Using molecular dynamics simulations we examine the effective interactions between two like-charged rods as a function of angle and separation. In particular, we determine how the competing electrostatic repulsions and…

Soft Condensed Matter · Physics 2009-11-10 Kun-Chun Lee , Itamar Borukhov , William M. Gelbart , Andrea J. Liu , Mark J. Stevens

The hydrodynamic behavior of electron fluids in a certain range of temperatures and densities is well established in graphene and in 2D semiconductor heterostructures. The hydrodynamic regime is intrinsically based on electron-electron…

Mesoscale and Nanoscale Physics · Physics 2023-12-12 Jack N. Engdahl , Aydin Cem Keser , Oleg P. Sushkov

Wetting of a charged substrate by an electrolyte solution is investigated by means of classical density functional theory applied to a lattice model. Within the present model the pure, i.e., salt-free solvent, for which all interactions are…

Soft Condensed Matter · Physics 2013-06-06 Ingrid Ibagon , Markus Bier , S. Dietrich

Intermolecular correlations in liquid water at ambient conditions have generally been characterized through short range density fluctuations described through the atomic pair distribution functions (PDF). Recent numerical and experimental…

Soft Condensed Matter · Physics 2016-03-23 Upayan Baul , J. Maruthi Pradeep Kanth , Ramesh Anishetty , Satyavani Vemparala

Polymer translocation experiments typically involve anionic polyelectrolytes such as DNA molecules driven through negatively charged nanopores. Quantitative modelling of polymer capture to the nanopore followed by translocation therefore…

Soft Condensed Matter · Physics 2017-10-11 Sahin Buyukdagli , Tapio Ala-Nissila

Rejuvenation of hydrodynamic transport in solids provides a new window to study collective motion of electrons, where electrons behave like a viscous fluid akin to classical liquids. Experimental observations of such exotic states have not…

Quantum Physics · Physics 2022-09-13 Weiwei Chen , W. Zhu

Electrochemistry experiments have established that the capacitance of electrode-electrolyte interfaces is much larger for good metals such as gold and platinum than for carbon-based materials. Despite the development of elaborate electrode…

Materials Science · Physics 2021-09-03 Alessandra Serva , Laura Scalfi , Benjamin Rotenberg , Mathieu Salanne

Hydroxide ion transport in anion-exchange membranes fundamentally limits the efficiency of alkaline water electrolysis for green hydrogen production, yet the atomic-scale transport mechanisms remain poorly understood due to the…

We demonstrate a general non--Derjaguin-Landau-Verwey-Overbeek method to stabilize colloids in liquids. By this method, colloidal particles that initially form unstable suspension and sediment from the liquid are stabilized by the addition…

Soft Condensed Matter · Physics 2014-09-12 Sela Samin , Manuela Hod , Eitan Melamed , Moshe Gottlieb , Yoav Tsori

Metal hydrides are critical materials in numerous technologies including hydrogen storage, gas separation, and electrocatalysis. Here, using Pd-H as a model metal hydride, we perform electrochemical insertion studies of hydrogen via liquid…

Materials Science · Physics 2018-08-07 Jesse D. Benck , Ariel Jackson , David Young , Daniel Rettenwander , Yet-Ming Chiang

The striking anomalies in physical properties of supercooled water that were discovered in the 1960-70s, remain incompletely understood and so provide both a source of controversy amongst theoreticians, and a stimulus to experimentalists…

Chemical Physics · Physics 2016-05-31 Sander Woutersen , Michiel Hilbers , Zuofeng Zhao , C. Austen Angell

Using the Taylor--Couette geometry we experimentally investigate the effect of salt on drag reduction caused by bubbles present in the flow. We combine torque measurements with optical high-speed imaging to relate the bubble size to the…

Fluid Dynamics · Physics 2023-02-15 Luuk J. Blaauw , Detlef Lohse , Sander G. Huisman

Ionic liquids (ILs) are salts that are liquid close to room temperature. Their possible applications are numerous, e.g., as solvents for green chemistry in various electrochemical devices, and even for such "exotic" purposes as…

Materials Science · Physics 2015-09-16 P. Sippel , P. Lunkenheimer , S. Krohns , E. Thoms , A. Loidl

We present results from extensive molecular dynamics simulations of collapse transitions of hydrophobic polymers in explicit water focused on understanding effects of lengthscale of the hydrophobic surface and of attractive interactions on…

Statistical Mechanics · Physics 2007-05-23 Manoj V. Athawale , Gaurav Goel , Tuhin Ghosh , Thomas M. Truskett , Shekhar Garde

Using a solid electrolyte to tune the carrier density in thin-film materials is an emerging technique that has potential applications in both basic and applied research. Until now, only materials containing small ions, such as protons and…

Materials Science · Physics 2017-06-16 Jialin Zhao , Meng Wang , Xuefu Zhang , Yue Lv , Tianru Wu , Shan Qiao , Shufeng Song , Bo Gao