Related papers: Attosecond Transient Absorption Spectroscopy witho…
Extreme ultraviolet (XUV) transient absorption (TA) and transient reflectivity (TR) spectroscopies enable element-specific insights into attosecond-timescale processes in solids. XUV transient grating spectroscopy (TGS) is an emerging tool…
We numerically demonstrate inhibition of absorption, optical transparency, and anomalous momentum states of phase locked harmonic pulses in semiconductors, at UV and extreme UV frequencies, in spectral regions where the dielectric constant…
Time-domain sampling of arbitrary electric fields with sub-cycle resolution enables a complete time-frequency analysis of a system's response to electromagnetic illumination. This provides access to dynamic information that is not provided…
The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…
We demonstrate time-resolved nonlinear extreme-ultraviolet absorption spectroscopy on multiply charged ions, here applied to the doubly charged neon ion, driven by a phase-locked sequence of two intense free-electron laser pulses.…
We present an experimental approach to detect the saturated absorption spectroscopy different from conventional scheme. Using this approach, crossovers are removed to avoid their overlap with other peaks in the spectrum and sensitivity of…
Shaping electron beams with the cycles of light provides femtosecond and attosecond time resolution in electron microscopy and enables fundamental quantum-coherent measurements. However, efficient light-electron control requires a prolonged…
The transient-absorption spectrum of a $V$-type three-level system is investigated, when this is periodically excited by a train of equally spaced, $\delta$-like pump pulses as, e.g., from an optical-frequency-comb laser. We show that, even…
We present a theoretical study of transient absorption and reshaping of extreme ultraviolet (XUV) pulses by helium atoms dressed with a moderately strong infrared (IR) laser field. We formulate the atomic response using both the…
Coherent light beams composed of ultrashort pulses are now increasingly used in different fields of Science, from time-resolved spectroscopy to plasma physics. Under the effect of even simple optical components, the spatial properties of…
Recent advances in the field of attosecond science hold the promise of tracking electronic processes at the shortest space and time scales. Imaging methods that combine attosecond temporal with nanometer spatial resolution are currently out…
We have calculated the resonant and nonresonant contributions to attosecond impulsive stimulated electronic Raman scattering (SERS) in regions of autoionizing transitions. Comparison with Multiconfiguration Time-Dependent Hartree-Fock…
The generation of the shortest isolated attosecond pulses requires both broad spectral bandwidth and control of the spectral phase. Rapid progress has been made in both aspects, leading to the generation of the world-record-shortest 67 as…
Two decades after its introduction, laser-assisted Atom Probe Tomography (La-APT) has demonstrated a unique potential for the study of the 3D distribution of atomic species in semiconductor materials and devices, and in a growing list of…
Phase transitions of solids and structural transformations of molecules are canonical examples of important photo-induced processes, whose underlying mechanisms largely elude our comprehension due to our inability to correlate electronic…
In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…
We develop an analytical model for ultraintense attosecond pulse emission in the highly relativistic laser-plasma interaction. In this model, the attosecond pulse is emitted by a strongly compressed electron layer around the instant when…
Based on the work done by an electromagnetic field on an atomic or molecular electronic system, a general gauge invariant formulation of transient absorption spectroscopy is presented within the semi-classical approximation. Avoiding…
Linear off-resonant X-ray Raman techniques are capable of detecting the ultrafast electronic coherences generated when a photoexcited wave packet passes through a conical intersection. A hybrid femtosecond or attosecond probe pulse is…
High-repetition-rate attosecond pulse sources are indispensable tools of time-resolved studies of electron dynamics, such as coincidence spectroscopy and experiments with high demands on statistics or signal-to-noise ratio, especially in…