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On a lattice composed of triangular plaquettes where antiferromagnetic exchange interactions between localized spins cannot be simultaneously satisfied, the system becomes geometrically frustrated with magnetically disordered phases…

The physics of spin-orbit entangled magnetic moments of $4d$ and $5d$ transition metal ions on a honeycomb lattice has been much explored in search for unconventional magnetic orders or quantum spin liquids expected for compass spin models,…

Strongly Correlated Electrons · Physics 2024-10-15 Ryutaro Okuma , Kylie MacFarquharson , Roger D. Johnson , David Voneshen , Pascal Manuel , Radu Coldea

Quantum spin liquids (QSLs) are an exotic state of matter that is subject to extensive research. However, the relationship between the ubiquitous disorder and the QSL behaviors is still unclear. Here, by performing comparative experimental…

We have performed high resolution neutron diffraction and inelastic neutron scattering experiments in the frustrated multiferroic hexagonal compounds RMnO3 (R=Ho, Yb, Sc, Y), which provide evidence of a strong magneto-elastic coupling in…

Strongly Correlated Electrons · Physics 2009-06-01 X. Fabreges , S. Petit , I. Mirebeau , S. Pailhes , L. Pinsard , A. Forget , M. T. Fernandez-Diaz , F. Porcher

MgV$_{2}$O$_{4}$ is a spinel based on magnetic V$^{3+}$ ions which host both spin ($S=1$) and orbital ($l_{eff}=1$) moments. Owing to the underlying pyrochlore coordination of the magnetic sites, the spins in MgV$_{2}$O$_{4}$ only…

A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For…

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…

Magnetic spins and charges interact strongly in high-temperature superconductors. New physics emerges as layers of copper oxide are tuned towards the boundary of the superconducting phase. As the pseudogap increases the characteristic spin…

The Yb based triangular lattice delafossites $A$Yb$X_2$ ($A$ = alkali metal, $X$ = O, S, Se) have recently been studied as quantum spin liquid candidates. We report the synthesis of powders and single crystals of CuYbSe$_2$ with a perfect…

Strongly Correlated Electrons · Physics 2025-09-23 Barkha Khattar , Anzar Ali , Masahiko Isobe , Yogesh Singh

Recent experiments on the Ba$_3$XSb$_2$O$_9$ family have revealed materials that potentially realise spin- and spin-orbital liquid physics. However, the lattice structure of these materials is complicated due to the presence of charged…

Strongly Correlated Electrons · Physics 2015-10-06 Andrew Smerald , Frederic Mila

The temperature-magnetic-field phase diagram of the mixed honeycomb triangular lattice system K$_{2}$Mn$_{3}$(VO$_{4}$)$_{2}$CO$_{3}$ is investigated by means of magnetization, heat capacity and neutron scattering measurements. The results…

The search for new quantum phases, especially in frustrated magnets, is central to modern condensed matter physics. One of the most promising places to look is in rare-earth pyrochlore magnets with highly-anisotropic exchange interactions,…

Strongly Correlated Electrons · Physics 2017-03-29 Han Yan , Owen Benton , Ludovic D. C. Jaubert , Nic Shannon

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

Strongly Correlated Electrons · Physics 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome

In this paper we present a comprehensive study of magnetic dynamics in the rare-earth orthoferrite YbFeO$_3$ at temperatures below and above the spin-reorientation (SR) transition $T_{\mathrm{SR}}=7.6$ K, in magnetic fields applied along…

We study the effective spin-orbital model for honeycomb-layered transition metal compounds, applying the second-order perturbation theory to the three-orbital Hubbard model with the anisotropic hoppings. This model is reduced to the Kitaev…

Strongly Correlated Electrons · Physics 2018-04-04 Akihisa Koga , Shiryu Nakauchi , Joji Nasu

We performed high-field magnetization, magnetocaloric effect (MCE), and NMR measurements on the Ising triangular-lattice antiferromagnet Rb$_2$Co(SeO$_3$)$_2$. The observations of the 1/3-magnetization plateau, the split NMR lines, and the…

Motivated by the recent activities on the Ni-based diamond lattice antiferromagnet NiRh$_2$O$_4$, we theoretically explore on a general ground the unique spin and orbital physics for the Ni$^{2+}$ ions with a $3d^8$ electron configuration…

Strongly Correlated Electrons · Physics 2019-07-10 Fei-Ye Li , Gang Chen

Co$^{2+}$ ions in an octahedral crystal field, stabilise a j$_{eff}$ = 1/2 ground state with an orbital degree of freedom and have been recently put forward for realising Kitaev interactions, a prediction we have tested by investigating…

Rare-earth delafossites were recently proposed as promising candidates for the realization of an effective $S$=1/2 quantum spin liquid (QSL) on the triangular lattice. In contrast to the most actively studied triangular-lattice…

Strongly Correlated Electrons · Physics 2020-01-08 R. Sarkar , Ph. Schlender , V. Grinenko , E. Haeussler , Peter J. Baker , Th. Doert , H. -H. Klauss