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We present a simple model of the bimolecular charge carrier recombination in polar amorphous organic semiconductors where the dominant part of the energetic disorder is provided by permanent dipoles and show that the recombination rate…

Disordered Systems and Neural Networks · Physics 2020-02-21 S. V. Novikov

We consider the bimolecular charge carrier recombination in amorphous organic semiconductors having a special kind of energetic disorder where energy levels for electrons and holes at a given transport site move in the same direction with…

Materials Science · Physics 2020-02-21 S. V. Novikov

The original Shockley-Read-Hall recombination statistics is extended to include recombination of localized excitations. The recombination is treated as a bimolecular process rather than a monomolecular recombination of excitons. The…

Materials Science · Physics 2019-04-16 Oleg Rubel

Understanding how the complex intermolecular- and nano-structure present in organic semiconductor donor-acceptor blends impacts charge carrier motion, interactions, and recombination behavior is a critical fundamental issue with a…

Materials Science · Physics 2016-06-08 Michael C. Heiber , Thuc-Quyen Nguyen , Carsten Deibel

We report numerical and analytical studies of the donor-acceptor recombination in compensated semiconductors. Our calculations take into account random electric fields of charged impurities which are important in non zero compensation case.…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 N. A. Bogoslovskiy , P. V. Petrov , Yu. L. Ivanov K. D. Tsendin , N. S. Averkiev

A self-consistent model of bipolar charge-carrier injection and transport processes in a semiconductor/insulator/conductor system is developed which incorporates space-charge effects in the description of the injection process. The amount…

Materials Science · Physics 2008-11-27 S. V. Yampolskii , Yu. A. Genenko , C. Melzer , K. Stegmaier , H. von Seggern

The theoretical effects of phase separation on encounter-limited charge carrier recombination in organic semiconductor blends are investigated using kinetic Monte Carlo (KMC) simulations of pump-probe experiments. Using model bulk…

Materials Science · Physics 2015-04-06 Michael C. Heiber , Christoph Baumbach , Vladimir Dyakonov , Carsten Deibel

A method for determination of the bimolecular recombination constant in working double-injection diodes such as organic light-emitting diodes (OLEDs) and organic photovoltaics (OPVs) using impedance spectroscopy is proposed. The proposed…

Applied Physics · Physics 2019-03-27 Makoto Takada , Takahiro Mayumi , Takashi Nagase , Takashi Kobayashi , Hiroyoshi Naito

Carrier recombination is a process that significantly influences the performance of semiconductor devices such as solar cells, photodiodes, and light-emitting diodes (LEDs). Therefore, a model that can accurately describe and quantify the…

Applied Physics · Physics 2022-04-11 M. L. Inche Ibrahim , Anvar A. Zakhidov

The kinetics of the charge carrier recombination in dye molecule-doped multilayer organic light-emitting diodes (OLEDs) was quantified by transient electroluminescence (EL). Three sets of dye molecules, such as derivatives of naphthalimide…

Materials Science · Physics 2014-11-13 Shengwei Shi , Feng Gao , Zhengyi Sun , Yiqiang Zhan , Mats Fahlman , Dongge Ma

We propose a model to explain the reduced bimolecular recombination rate found in state-of-the-art bulk heterojunction solar cells. When compared to the Langevin recombination, the experimentally observed rate is one to four orders of…

Materials Science · Physics 2009-08-09 C. Deibel , A. Wagenpfahl , V. Dyakonov

The photoluminescence in amorphous semiconductors decays according to power law $t^{-delta}$ at long times. The photoluminescence is controlled by dispersive transport of electrons. The latter is usually characterized by the power $alpha$…

Statistical Mechanics · Physics 2009-11-11 Kazuhiko Seki , Mariusz Wojcik , M. Tachiya

The dimer-atom-atom recombination process in the system of four identical bosons with resonant interactions is studied. The description uses the exact Alt, Grassberger and Sandhas equations for the four-particle transition operators that…

Atomic Physics · Physics 2015-06-05 A. Deltuva

Apparent recombination orders exceeding the value of two expected for bimolecular recombination have been reported for organic solar cells in various publications. Two prominent explanations are bimolecular losses with a carrier…

Soft Condensed Matter · Physics 2012-08-23 D. Rauh , C. Deibel , V. Dyakonov

The geometry-dependent energy transfer rate from an electrically pumped inorganic semiconductor quantum well into an organic molecular layer is studied theoretically. We focus on F\"orster-type nonradiative excitation transfer between the…

Mesoscale and Nanoscale Physics · Physics 2018-04-20 Judith Specht , Eike Verdenhalven , Björn Bieniek , Patrick Rinke , Andreas Knorr , Marten Richter

Metal/semiconductor interfaces govern the operation of semiconductor devices through the formation of charge injection barriers that can be controlled by tuning the metal work function. However, the controlling ability is typically limited…

Materials Science · Physics 2014-01-14 Ryo Nouchi , Masanori Shigeno , Nao Yamada , Tomoaki Nishino , Katsumi Tanigaki , Masahiko Yamaguchi

Two-dimensional (2D) crystalline semiconductors hold promise for next-generation electronic devices due to its atomical thickness and consequent properties. Despite years of search, literature-reported 2D semiconductors commonly suffered…

Materials Science · Physics 2024-04-15 Chenmu Zhang , Yuanyue Liu

The ABC model has been widely used to describe the carrier recombination rate, in which the rate of non-radiative recombination assisted by deep-level defects is assumed to depend linearly on excess carrier density $\Delta n$, leading to a…

Materials Science · Physics 2025-02-25 Shanshan Wang , Menglin Huang , Su-Huai Wei , Xin-Gao Gong , Shiyou Chen

We report on the non-trivial field dependence of charge carrier recombination in an organic blend at low temperatures. A new microwave resonance technique for monitoring charge recombination in organic semiconductors at low temperatures is…

Mesoscale and Nanoscale Physics · Physics 2015-09-09 S. Athanasopoulos , N. C. Greenham , R. H. Friend , A. D. Chepelianskii

Organic semiconductors are indispensable for today's display technologies in form of organic light emitting diodes (OLEDs) and further optoelectronic applications. However, organic materials do not reach the same charge carrier mobility as…

Soft Condensed Matter · Physics 2023-10-12 Patrick Reiser , Manuel Konrad , Artem Fediai , Salvador Léon , Wolfgang Wenzel , Pascal Friederich
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