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An efficient low-order scaling method is presented for large-scale electronic structure calculations based on the density functional theory using localized basis functions, which directly computes selected elements of the density matrix by…

Strongly Correlated Electrons · Physics 2010-05-04 Taisuke Ozaki

The split-charge equilibration method is extended to describe dissipative charge transfer similarly as the Drude model, whereby the generic frequency-dependent dielectric permitivitties or conductivities of dielectrics and metals can be…

Materials Science · Physics 2024-10-02 Martin H. Müser

The three-particle operator in a second quantized form is studied. The operator is transformed into irreducible tensor form. Possible coupling schemes, distinguished by the classes of symmetric group \mathrm{S_{6}}, are presented.…

Atomic Physics · Physics 2018-02-14 Rytis Jursenas , Gintaras Merkelis

We illustrate the main features of a recently proposed method based on ensemble density functional theory to divide rigorously a complex molecular system into its parts [M.H. Cohen and A. Wasserman, J. Phys. Chem. A 111, 2229 (2007)]. The…

Other Condensed Matter · Physics 2016-09-28 Morrel H. Cohen , Adam Wasserman , Kieron Burke

We describe a macroscopic beam splitter for polar neutral molecules. A complex electrode structure is required for the beam splitter which would be very difficult to produce with traditional manufacturing methods. Instead, we make use of a…

Chemical Physics · Physics 2017-05-03 Sean D. S. Gordon , Andreas Osterwalder

The ability of having a sparse representation for a certain class of signals has many applications in data analysis, image processing, and other research fields. Among sparse representations, the cosparse analysis model has recently gained…

Machine Learning · Computer Science 2014-06-09 Matthias Seibert , Julian Wörmann , Rémi Gribonval , Martin Kleinsteuber

This paper proposes a component-based dual decomposition of the nonconvex AC optimal power flow (OPF) problem, where the modified dual function is solved in a distributed fashion. The main contribution of this work is that is demonstrates…

Distributed, Parallel, and Cluster Computing · Computer Science 2017-08-23 Sleiman Mhanna , Gregor Verbic , Archie Chapman

We analyze the convergence of compressive sensing based sampling techniques for the efficient evaluation of functionals of solutions for a class of high-dimensional, affine-parametric, linear operator equations which depend on possibly…

Numerical Analysis · Mathematics 2015-09-22 Holger Rauhut , Christoph Schwab

In this article we address the general approach for calculating dynamical dipole polarizabilities of small quantum systems, based on a sum-over-states formula involving in principle the entire energy spectrum of the system. We complement…

Quantum Physics · Physics 2017-07-10 R. Vexiau , D. Borsalino , M. Lepers , A. Orbán , M. Aymar , O. Dulieu , N. Bouloufa-Maafa

The reliability of the approximations commonly adopted in the calculation of static optical (hyper)polarizabilities is tested against exact results obtained for an interesting toy-model. The model accounts for the principal features of…

Chemical Physics · Physics 2009-11-07 Luca Del Freo , Francesca Terenziani , Anna Painelli

Numerical heating in particle-in-cell (PIC) codes currently precludes the accurate simulation of cold, relativistic plasma over long periods, severely limiting their applications in astrophysical environments. We present a spatially…

We present a new multi-fluid, multi-temperature plasma solver with adaptive Cartesian mesh (ACM) based on a full-Newton (non-linear, implicit) scheme for collisional low-temperature plasma. The particle transport is described using the…

Computational Physics · Physics 2020-08-19 Robert Arslanbekov , Vladimir Kolobov

Operator splitting methods solve composite optimization problems by breaking them into smaller sub-problems that can be solved sequentially or in parallel. In this paper, we propose a unified framework for certifying both linear and…

Optimization and Control · Mathematics 2019-10-25 Han Wang , Mahyar Fazlyab , Shaoru Chen , Victor M. Preciado

The impact of the operator-valued commutator on nonclassical properties of continuous polarization variables is discussed. The definition of polarization squeezing is clarified to exclude those squeezed states which do not contain any new…

Quantum Physics · Physics 2007-05-23 N. Korolkova , R. Loudon

We give a constant-factor approximation algorithm for the asymmetric traveling salesman problem (ATSP). Our approximation guarantee is analyzed with respect to the standard LP relaxation, and thus our result confirms the conjectured…

Data Structures and Algorithms · Computer Science 2020-09-17 Ola Svensson , Jakub Tarnawski , László A. Végh

Splitting algorithms for finding a zero of sum of operators often involve multiple steps which are referred to as forward or backward steps. Forward steps are the explicit use of the operators and backward steps involve the operators…

Optimization and Control · Mathematics 2021-04-13 Minh N. Dao , Hung M. Phan

General formulas of the two-electron operator representing either atomic or effective interactions are given in a coupled tensorial form in relativistic approximation. The alternatives of using uncoupled, coupled and antisymmetric…

Atomic Physics · Physics 2010-04-30 Rytis Jursenas , Gintaras Merkelis

We introduce a coefficient-decoupled matrix product operator (MPO) representation for Pauli-sum operators that separates reusable symbolic operator support from a tunable coefficient bridge across a fixed bipartition. This representation…

Quantum Physics · Physics 2026-03-27 Younes Javanmard

Intramolecular symmetry-adapted perturbation theory (ISAPT) is a method to compute and decompose the noncovalent interaction energy between two molecular fragments A and B connected via a linker C. The existing ISAPT algorithm displays…

Chemical Physics · Physics 2022-09-13 Du Luu , Konrad Patkowski

A new method for implementing the kinetic energy operator for real-space, grid-based electronic structure codes is developed. It is based on multi-order Adaptive Finite Differencing (AFD) and uses atomic pseudo orbitals produced by the…

Computational Physics · Physics 2023-05-23 E. L. Briggs , Wenchang Lu , J. Bernholc