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Recent experiments on the dipolar-octupolar pyrochlore compound Ce$_2$Zr$_2$O$_7$ indicate that it may realize a three-dimensional quantum spin liquid (QSL). In particular, the analyses of available data suggest that the system is in a…

Strongly Correlated Electrons · Physics 2022-06-30 Félix Desrochers , Li Ern Chern , Yong Baek Kim

The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…

The dipolar-octupolar (DO) pyrochlores, R$_2$M$_2$O$_7$ (R = Ce, Sm, Nd), are key players in the search for realizable novel quantum spin liquid (QSL) states as a large parameter space within the DO pyrochlore phase diagram is theorized to…

Symmetry plays a fundamental role in our understanding of both conventional symmetry breaking phases and the more exotic quantum and topological phases of matter. We explore the experimental signatures of symmetry enriched U(1) quantum spin…

Strongly Correlated Electrons · Physics 2017-01-25 Yao Dong Li , Gang Chen

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

We point out the experimental relevance and the detection scheme of symmetry enriched U(1) quantum spin liquids (QSLs) outside the perturbative spin-ice regime. Recent experiments on Ce-based pyrochlore QSL materials suggest that the…

Strongly Correlated Electrons · Physics 2020-03-25 Xu-Ping Yao , Yao Dong Li , Gang Chen

Quantum spin liquids (QSLs) are exotic phases of matter exhibiting long-range entanglement and supporting emergent gauge fields. A vigorous search for experimental realizations of these states has identified several materials with…

Strongly Correlated Electrons · Physics 2018-07-24 Owen Benton

Motivated by recent experimental and theoretical progress on the Er2Ti2O7 pyrochlore XY antiferromagnet, we study the problem of quantum order-by-disorder in pyrochlore XY systems. We consider the most general nearest-neighbor pseudo…

Strongly Correlated Electrons · Physics 2013-11-15 Anson W. C. Wong , Zhihao Hao , Michel J. P. Gingras

A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…

Quantum spin liquid (QSL) is a disordered state of quantum-mechanically entangled spins commonly arising from frustrated magnetic dipolar interactions. However, QSL in some pyrochlore magnets can also come from frustrated magnetic octupolar…

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

Dipolar-octupolar (DO) pyrochlore systems Ce$_2$(Zr,Sn,Hf)$_2$O$_7$ have garnered much attention as recent investigations suggest that they may stabilize a novel quantum spin ice (QSI), a quantum spin liquid (QSL) with an emergent $U(1)$…

Strongly Correlated Electrons · Physics 2025-12-10 Zhengbang Zhou , Félix Desrochers , Yong Baek Kim

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

We study the uniform $U(1)$ quantum spin liquid (QSL) with low-energy fermionic quasiparticles for pyrochlore magnets with dipolar-octupolar symmetry, employing a fermionic parton mean field theory approach. Self-consistent calculations…

Strongly Correlated Electrons · Physics 2023-12-07 Krushna Chandra Sahu , Sambuddha Sanyal

Magnetic heat capacity measurements of a high-quality single crystal of the dipole-octupole pyrochlore Ce$_2$Hf$_2$O$_7$ down to a temperature of $T = 0.02$ K are reported. These show a two-peaked structure, with a Schottky-like peak at…

We study the zero-temperature ground-state (GS) properties of the spin-$\frac{1}{2}$ anisotropic planar pyrochlore, using the coupled cluster method (CCM) implemented to high orders of approximation. The system comprises a $J_{1}$--$J_{2}$…

Strongly Correlated Electrons · Physics 2015-09-09 P. H. Y. Li , R. F. Bishop

Dipolar-octupolar pyrochlore magnets in a strong external magnet field applied in the [110] direction are known to form a `chain' state, with subextensive degeneracy. Magnetic moments are correlated along one-dimensional chains carrying…

Strongly Correlated Electrons · Physics 2020-12-08 Benedikt Placke , Roderich Moessner , Owen Benton

Motivated by recent experiments on Ce$_2$Zr$_2$O$_7$ that reveal a dynamic, liquid-like ground state, we study the nearest neighbor XYZ Hamiltonian of dipolar-octupolar pyrochlore magnets with the pseudofermion functional renormalization…

Strongly Correlated Electrons · Physics 2024-05-21 Li Ern Chern , Félix Desrochers , Yong Baek Kim , Claudio Castelnovo

The quantum pyrochlore antiferromagnet is studied by perturbative expansions and exact diagonalization of small clusters. We find that the ground state is a spin-liquid state: The spin-spin correlation functions decay exponentially with…

Strongly Correlated Electrons · Physics 2009-10-31 Benjamin Canals , Claudine Lacroix
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