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Nanomaterials are anticipated to be promising storage media, owing to their high surface-to-mass ratio. The high hydrogen capacity achieved by using graphene has reinforced this opinion and motivated investigations of the possibility to use…

Materials Science · Physics 2013-11-26 Yuanyue Liu , Vasilii I. Artyukhov , Mingjie Liu , Avetik R. Harutyunyan , Boris I. Yakobson

Li$_6$PS$_5$Cl is a promising candidate for the solid electrolyte in all-solid-state Li-ion batteries. In applications, this material is in a polycrystalline state with grain boundaries (GBs) that can affect ionic conductivity. While…

Materials Science · Physics 2024-12-02 Yongliang Ou , Yuji Ikeda , Lena Scholz , Sergiy Divinski , Felix Fritzen , Blazej Grabowski

In this study, we address the challenge of electrolyte degradation in all-solid-state humidified Li-$O_2$ batteries, which offer high theoretical energy density and potential cost advantages over conventional lithium-ion batteries.…

The effect of increased electron-density (from adsorbed Li atoms) in polyacenes and in nano-ribbons with zig-zag edge is discussed in terms of resonance theoretical considerations and in terms edge-localized frontier molecular orbitals. The…

Chemical Physics · Physics 2025-11-10 Yenni P. Ortiz , Douglas J. Klein , Thomas H. Seligman

We study the effect of long-range disorder created by charge impurities on the carrier density distribution of graphene-based heterostructures. We consider heterostructures formed by two graphenic sheets (either single layer graphene, SLG,…

Mesoscale and Nanoscale Physics · Physics 2014-07-10 Martin Rodriguez-Vega , Jonathan Fischer , S. Das Sarma , E. Rossi

Based on density functional theory (DFT) calculations including an on-site Hubbard $U$ term we investigate the effect of substrate-induced strain on the properties of ferrimagnetic Fe$_2$O$_3$-FeTiO$_3$ solid solutions and heterostructures.…

Materials Science · Physics 2009-10-13 Hasan Sadat Nabi , Rossitza Pentcheva

Electron transport in bilayer graphene is studied by using a first principles analysis and theMonte Carlo simulation under conditions relevant to potential applications. While the intrinsic properties are found to be much less desirable in…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 X. Li , K. M. Borysenko , M. Buongiorno Nardelli , K. W. Kim

We present a theoretical study of the local optical conductivity, plasmon spectra, and thermoelectric properties of twisted bilayer graphene (TBG) at different filling factors and twist angles $\theta$. Our calculations are based on the…

Mesoscale and Nanoscale Physics · Physics 2020-09-04 Pietro Novelli , Iacopo Torre , Frank H. L. Koppens , Fabio Taddei , Marco Polini

We show that the propagation of spin polarized carriers may be dramatically affected by {\em inhomogeneous} electric fields. Surprisingly, the spin diffusion length is found to strongly depend on the sign and magnitude of electric field…

Materials Science · Physics 2009-11-11 Dan Csontos , Sergio E. Ulloa

By combining {\it ab initio} calculations and experiments we demonstrate how the band gap of the transition metal tri-chalcogenide TiS$_3$ can be modified by inducing tensile or compressive strain. We show by numerical calculations that the…

Flexoelectricity, a coupling between strain gradients and electric polarization, has attracted significant interest due to its critical role in enhanced effects at small scales and its applicability across a diverse range of materials.…

Computational Physics · Physics 2025-02-28 Arash Kazemi , Kshiteej J Deshmukh , Susan Trolier-McKinstry , Shad Roundy

We formulate the continuum field equations and constitutive equations that govern deformation, stress, and electric current flow in a Li-ion half-cell. The model considers mass transport through the system, deformation and stress in the…

Computational Physics · Physics 2011-08-01 Allan F. Bower , Pradeep R. Guduru , Vijay A. Sethuraman

Moving to larger cell formats in lithium-ion batteries increases overall useable energy but introduces inhomogeneities that influence aging. This study investigates degradation in 21700-type cells with NCM cathodes and graphite/SiOx anodes…

Recently, considerable efforts have been made on research and improvement for Ni-rich lithium-ion batteries to meet the demand from vehicles and grid-level large-scale energy storage. Development of next-generation high-performance…

The chemical modification of graphene with adatoms is of importance for nanoelectronics applications. Based on first-principles density-functional theory calculations with including van der Waals interactions, we present a comparative study…

Materials Science · Physics 2017-04-26 Seho Yi , Hyun-Jung Kim , Jin-Ho Choi , Jun-Hyung Cho

Surface stresses, in nano-sized anode particles undergoing chemomechanical interactions, have a relaxing effect on the diffusion-induced stresses thus improving the mechanical endurance of the particles, whereas, the compressive effect of…

Soft Condensed Matter · Physics 2021-02-23 Amrita Sengupta , Jeevanjyoti Chakraborty

We perform molecular dynamics simulations to study lithium dynamics in a model of LiPO$_3$ glass at temperatures below the glass transition. A straightforward analysis of the ionic trajectories shows that lithium diffusion results from…

Soft Condensed Matter · Physics 2009-11-10 Michael Vogel

All solid state Li-ion batteries employing metallic lithium as an anode offer higher energy densities while also being safer than conventional liquid electrolyte based Li-ion batteries. However, the growth of tiny filaments of lithium…

Applied Physics · Physics 2020-01-20 Vikalp Raj , Varun R Kankanallu , Bibhatsu Kuiri , Naga Phani B Aetukuri

We calculate the \tco{polarization}-controlled Rayleigh scattering response of twisted bilayer graphene (tBLG) based on the continuum electronic band model developed by Bistritzer and MacDonald while considering its refinements which…

Mesoscale and Nanoscale Physics · Physics 2023-06-01 Disha Arora , Deepanshu Aggarwal , Sankalpa Ghosh , Rohit Narula

We report measurements of the diffusion rate of isolated ion-implanted $^{8}$Li$^{+}$ within $\sim$120 nm of the surface of oriented single-crystal rutile TiO$_2$ using a radiotracer technique. The $\alpha$-particles from the $^{8}$Li decay…

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