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We analyze the effects on the structural and electronic properties of vanadium dioxide (VO$_2$) of adding an empirical inter-atomic potential within the density-functional theory$+V$ (DFT$+V$) framework. We use the DFT$+V$ machinery founded…

Materials Science · Physics 2025-04-15 Lea Haas , Peter Mlkvik , Nicola A. Spaldin , Claude Ederer

The interactions between different layers in van der Waals heterostructures have a significant impact on the electronic and optical characteristics. By utilizing the intrinsic dipole moment of Janus transition metal dichalcogenides (TMDs),…

Materials Science · Physics 2024-01-18 Ö. C. Yelgel

We report the existence of metallic two-dimensional electron gases (2DEGs) at the (001) and (101) surfaces of bulk-insulating TiO2 anatase due to local chemical doping by oxygen vacancies in the near-surface region. Using angle-resolved…

Materials Science · Physics 2015-07-15 T. C. Rödel , F. Fortuna , F. Bertran , M. Gabay , M. J. Rozenberg , A. F. Santander-Syro , P. Le Fèvre

We studied the oxygen vacancies($V_{O}$) in rutile TiO2 by using $G_0W_0$ approximation on top of GGA+$U$ as a method of choice to improve the gap. Since there is no extensive agreement regarding the characteristic of electron localization…

Strongly Correlated Electrons · Physics 2010-12-30 Ali Kazempour , Seyed Javad Hashemifar , Hadi Akbarzadeh

Phosphorene is emerging as a promising 2D semiconducting material with a direct band gap and high carrier mobility. In this paper, we examine the role of the extrinsic point defects including surface adatoms in modifying the electronic…

Chemical Physics · Physics 2015-05-20 Gaoxue Wang , Ravindra Pandey , Shashi P. Karna

In this study we report on the results from emission $^{57}$Fe M${\"o}$ssbauer Spectroscopy experiments, using dilute $^{57}$Mn implantation into pristine (TiO$_2$) and hydrogenated anatase held at temperatures between 300-700 K. Results of…

Studying the atomic structure of intrinsic defects in two-dimensional transition metal dichalcogenides is difficult since they damage quickly under the intense electron irradiation in transmission electron microscopy (TEM). However, this…

Achieving efficient and stable ultraviolet emission is a challenging goal in optoelectronic devices. Herein, we investigate the UV luminescence of zinc germanate Zn2GeO4 microwires by means of photoluminescence measurements as a function of…

The strain effect on electronic structure and thermoelectric properties of Higher Manganese Silicides (HMSs) Mn4Si7 was studied using Density Functional Theory (DFT) and through solving Boltzman Transport Equation (BTE). We found that the…

Materials Science · Physics 2016-09-21 Do Duc Cuong , JinSik Park , S. H. Rhim , Soon Cheol Hong

Interfacial water on transition metal oxides such as TiO$_2$ has been widely studied because of their structural complexity and scientific relevance in e.g. photocatalysis and ice growth. Using ab initio molecular dynamics, we find that…

Materials Science · Physics 2021-11-02 Keyang Liu , Jianqing Guo , Weizhong Fu , Ji Chen

Ab initio density functional theory (DFT) and DFT plus coherent potential approximation (DFT+CPA) are employed to reveal, respectively, the effect of in-plane strain and site-diagonal disorder on the electronic structure of cubic boron…

Materials Science · Physics 2022-12-20 L. Craco , S. S. Carara , E. da Silva Barboza , T. A. S. Pereira , M. V. Milosevic

The study of zinc oxide, within the homogeneous electron gas approximation, results in overhybridization of zinc $3d$ shell with oxygen $2p$ shell, a problem shown for most transition metal chalcogenides. This problem can be partially…

Chalcogen vacancies are considered to be the most abundant point defects in two-dimensional (2D) transition-metal dichalcogenide (TMD) semiconductors, and predicted to result in deep in-gap states (IGS). As a result, important features in…

Topological insulators (TIs) have been considered as promising candidates for next generation of electronic devices due to their topologically protected quantum transport phenomena. In this work, a scheme for atomic-scale field effect…

Mesoscale and Nanoscale Physics · Physics 2025-10-02 Cunyuan Jiang

Lattice defects such as stacking faults may obscure electronic topological features of real materials. In fact, defects are a source of disorder that can enhance the density of states and conductivity of the bulk of the system and they…

Mesoscale and Nanoscale Physics · Physics 2022-10-05 Gabriele Naselli , Viktor Könye , Sanjib Kumar Das , G. G. N. Angilella , Anna Isaeva , Jeroen van den Brink , Cosma Fulga

Defects in cuprous oxide (Cu$_2$O) strongly influence its performance in applications ranging from photovoltaics to emerging quantum technologies based on Rydberg excitons where microscopic crystal purity is essential. Photoluminescence…

Materials Science · Physics 2026-03-19 Alistair Brewin , Matthew P A Jones , Stewart J Clark

Td-WTe2 is a topological Weyl semimetal. WTe2 in the orthorhombic structure is stable at room temperature. Elastic, electronic, bonding, and optoelectronic properties of WTe2 have been investigated in detail in this work using the density…

Materials Science · Physics 2020-12-01 B. Rahman Rano , Ishtiaque M. Syed , S. H. Naqib

We present a microscopic investigation of frequently observed impurity-induced states in stoichiometric LiFeAs using low temperature scanning tunneling microscopy and spectroscopy (STM/STS). Our data reveal seven distinct well defined…

Superconductivity · Physics 2018-06-12 R. Schlegel , P. K. Nag , D. Baumann , R. Beck , S. Wurmehl , B. Büchner , C. Hess

Using first-principles calculations, we show that Fe2VAl is an indirect band gap semiconductor. Our calculations reveal that its, sometimes assigned, semimetallic character is not an intrinsic property but originates from the antisite…

Materials Science · Physics 2015-05-27 Daniel I. Bilc , Philippe Ghosez

An underestimation of the fundamental band gap values by the density functional theory within the local density approximation and associated approaches is a well-known challenge of ab-initio electronic structure computations. Motivated by…

Strongly Correlated Electrons · Physics 2023-08-24 Giuseppe Cuono , Raghottam M. Sattigeri , Carmine Autieri , Tomasz Dietl